摘要
In this work,we reported a new strategy to improve the nonlinear saturable absorption performance of magnetite(Fe_(3)O_(4))nanoparticles(FONPs)via the compositional engineering with the Ti_(3)C_(2) MXene in the near-infrared(NIR)region.Based on the DFT simulation,the band structures and work function were significantly modified by the Ti_(3)C_(2) MXene doping.By using the open-aperture Z-scan technology,the nonlinear optical features of the FONPs@Ti_(3)C_(2) nanocomposite were significantly improved,showing the great potential as the saturable absorber in the pulsed laser.With the nanocomposite as the saturable absorber,the passively Q-switched Nd:GdVO4 lasers emitted much shorter pulse durations when compared with the pristine FONP saturable absorber.These findings indicated that FONPs@Ti_(3)C_(2) heterostructure was a promising saturable absorber for the short pulse generation in the NIR region.
基金
This work was finically supported by the National Natural Science Foundation of China(NSFC)(Nos.12004213 and 21872084)
the Fundamental Research Fund of Shandong University(No.2018TB044)
the financial support from the Young Scholar Program of Shandong University。