液态水辐射源产生太赫兹波的研究进展

Research Progress on Terahertz Wave Generation from Liquid Water

作为生活中最常见的液体,液态水在学术研究中具有重要的地位。但由于水对太赫兹辐射具有极大的吸收系数,长期以来它并不被视为一种合适的太赫兹辐射源。不过近年来已经有研究团队在实验上证实了飞秒激光激励液态水产生太赫兹波的可行性,并且针对这一现象机制的相关理论模型也已被提出。由此可见,对该领域的现有研究成果进行总结,对水乃至其他液体作为辐射源产生太赫兹波的研究是具有重要意义的。对液态水中太赫兹波产生这一研究领域近些年的发展进行概述,包括两种不同的液态水辐射源系统方案的实验设计、与产生的太赫兹波能量有关的因素、相关理论模型的设计思路。最后结合自身理解与当前的研究成果,对这一领域的未来发展方向进行展望。

Significance Terahertz(THz)wave,whose frequency range lying between the infrared wave and microwave,is a section of the electromagnetic spectrum with unique features.Broadly,the THz frequency range covers the spectral region from 0.1 to 30 THz,but researchers universally define 0.1-10 THz as the THz band.Owing to the lack of suitable THz radiation sources and detectors,THz wave,once known as"THz Gap"for ages,became the last segment of the entire electromagnetic spectrum to be fully explored.Nevertheless,the ultrafast optoelectronics technology and microscale semiconductor technology,which received rapid development in the 1980 s,made emerging from the previous dilemma possible for researchers in this field.Since then,THz technology has been widely used in scientific research and practical application,such as medical treatment,nondestructive testing,national defense,safety inspection,and communication.Among various branches of THz technologies,THz photonics undoubtedly earns a place in the current hotspots of the field.However,recently,studies on THz photonics focused more on the linear response of material rather than the nonlinear response,and the absence of suitable THz radiation sources with strong field strength might be to blame for this study status.In China,the 973 Program and several other projects associated with fundamental study supported the study of THz photonics well,unfortunately,the related study work is still focused on linear THz systems.Thus,exploiting the technology for building a more suitable THz radiation source system with stronger THz field strength,along with its optimization,is an essential prerequisite for further expanding the practical area of THz waves.As the most common liquid in life,water plays an important role in academic research.However,water has not been considered an appropriate THz radiation source for a long time owing to its strong absorption in the THz frequency range.While recently,some groups have experimentally confirmed the feasibility of THz wave generation from water under the excitation of a femtosecond laser,and several theoretical models are proposed for the mechanism of the generation processes.Thus,summarizing the current research progress in this field for the study of THz wave generation from water and other liquids is significant.Progress Under the efforts of professor Zhang Xicheng and his team,a thin water film(~170μm)under femtosecond laser\s excitation was historically used for THz wave generation in 2017(Fig.1).This water film,which has a gravity-driven free-flowing structure,can be better for mitigating the inevitable absorption of THz waves caused by water.Under the identical experimental condition,the electric field of THz wave generated from the thin water film is 1.8 times stronger than the case of the air plasma.Besides,compared with air plasma,agreat difference in THz generation is that liquid water prefers a laser pulse with a longer pulse duration(~600 fs)rather than a traditional femtosecond pulse(~50 fs)(Fig.3).Further,the improvement of the THz electric field with a dual-color laser scheme in water is not able to be as high as that in air.The different photoionization mechanisms between water and air might be responsible for these discrepancies.To weaken the total internal reflection at the flat water-air interface in water film,a water line was used for solving this problem.In 2018,strong THz radiation generated from a water line of 200-μm diameter under the femtosecond laser\s excitation was first reported in the experiment(Fig.8).Strong THz radiation can be detected only when the pump laser propagation axis deviates from the center of the waterline owing to the ponderomotive force-induced photocurrent with the symmetry broken at the air-water interface.As for its preference,just like the results of water film,subpicosecond laser pulses behave better in water lines when compared with a short temporal laser pulse.Notably,the overall distribution of THz radiation generated by water lines with different diameters may not be different in space,so the optimal radiation angle for THz generation from a water line is all about 60°(Fig.10).Although the phenomenon is similar to air,the explanation for the mechanism of THz generation from water is still under study.While other kinds of nonlinear effects existed during the photoionization process in water and the different ionization mechanisms of these two matters may partially account for this mystery.Currently,the theoretical models to explain the phenomenon of THz generation from water include the dipole array model,ponderomotive-force-induced photocurrent model,unidirectional pulse propagation equation model,and radiation field dynamics model.Conclusions and Prospect The study on THz generation from liquid water would be beneficial for researchers to better understand the interaction between water and intense lasers,and it serves a significant role in the further study of potential THz radiation sources.Based on these reasons,research progresses on THz generation from liquid water recently,are reviewed in this article,which includes experimental schemes for two liquid water sources,the factors related to the improvement of the generated THz energy,as well as the design ideas for relevant theoretical models.Finally,the prospect of this field based on our understanding and the current study achievements is proposed.