摘要
Biology systems harvest solar energy to regulate ions and molecules precisely across cell membrane that is essential to maintain their life sustainability.Recently,artificial light-driven directional ion transport through graphene oxide membranes has been established,where the membrane converts light power into a transmembrane motive force.Herein,we report a silver nanoparticles decorated graphene oxide membranes for enhanced photo-driven ionic transport.Asymmetric light stimulated charge carrier dynamics,such as advanced light absorption efficiency,extended lifetime and efficient separation of photo-excited charge carriers,are account for the ion-driven force enhancement.Based on metal nanoparticles decoration,the concept of the guest-interactions of plasmon-enhanced photo-driven ion transport in two-dimentional layered membranes will stimulate broad researches in sensing,energy storage and conversion and water treatment.
基金
the National Natural Science Foundation of China(No.51603211)
the 111 Project(No.B14009).