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Recent advances in metal-free CDs/g-C_(3)N_(4) photocatalysts:Synthetic strategies,mechanism insight,and applications 被引量:1

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摘要 Carbon dots/graphite carbon nitride(CDs/g-C_(3)N_(4)),a novel composite photocatalyst,has shown great po-tential for applications in energy regeneration and environmental remediation owing to its following advantages:metal-free,low cost,easily tunable,and excellent photocatalytic performance.Hence,we reviewed the development of synthetic strategies,photocatalytic enhancement mechanisms,and pho-tocatalytic applications of CDs/g-C_(3)N_(4) in this study.First,the three composite strategies of CDs and g-C_(3)N_(4)-self-assembly,solvothermal,and calcination polymerization are outlined,and their advantages and disadvantages are described in detail.Moreover,the photocatalytic enhancement mechanism of the com-posite strategies was elucidated according to the variation trends of CDs/g-C_(3)N_(4) band structure,electronic properties,light absorption range,and interfacial charge transfer.Then,the applications of CDs/g-C_(3)N_(4) in hydrogen evolution,pollutant degradation,CO_(2) reduction,and bacterial disinfection in recent years are reviewed systematically.Finally,the current obstacles and future research directions of CDs/g-C_(3)N_(4) are discussed from the perspective of preparation technology and practical applications,respectively.
出处 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2023年第19期11-26,共16页 材料科学技术(英文版)
基金 supported by the National Key Research and Development Program of China (No.2022YFF1100705) the Key Research and Development Program of Yunnan Province (No.202202AE090007) the Science and Technology Project of Jiangsu Provincial Bureau of Market Supervision and Administra-tion (No.KJ2022054) the Fundamental Research Funds for the Central Universities (No.JUSRP222001) the Collaborative In-novation Center of Food Safety and Quality Control Jiangsu in Province,Jiangnan University.
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