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Thermo-electro-mechanical microstructural interdependences in conductive thermoplastics

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摘要 Additive manufacturing has enabled the design of thermoplastic components that provide structural support,electrical conductivity and heat generation modulated by mechanical deformation.The mechanisms and interplays that govern the material response at the microstructural level remain,however,elusive.Here,we develop an experimental method to characterise conductive filaments from a combined mechanical,electrical and thermal perspective.This approach is used to unravel exciting material interplays of conductive polylactic acid.To overcome experimental limitations that prevent a complete microstructural analysis of the problem,we develop a full-field homogenisation framework and implement it for finite elements.The framework accounts for viscoplasticity,electrical and thermal conduction,convection and heat generation via Joule effect,as well as for the interdependences between them.After experimental validation,the framework is applied to virtually optimise fabrication requirements to obtain desired properties in final products,i.e.,stiffer products,filaments with higher conductivities or with better sensing capabilities.
出处 《npj Computational Materials》 SCIE EI CSCD 2023年第1期955-965,共11页 计算材料学(英文)
基金 The authors acknowledge support from the European Research Council(ERC)under the European Union’s Horizon 2020 research and innovation programme(grant agreement No.947723,project:4D-BIOMAP) from the Ministerio de Ciencia,Innovacion y Universidades under the Plan Nacional 2018(RTI2018-094318-B-I00) the Plan Nacional 2021(PID2021-123294OB-I00) J.C.M.acknowledges support from the Ministerio de Ciencia,Innovacion y Universidades,Spain(PRE2019-089276) S.L.was funded by the Marie Skłodowska-Curie Individual Fellowship 101031287 under the EU Horizon 2020 Framework Programme for Research and Innovation.
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