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Revolutionizing photothermal CO_(2)hydrogenation with ceria-based catalysts

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摘要 In the context of achieving carbon neutrality,CO_(2)catalytic conversion technologies are effective in reducing atmospheric CO_(2)concentrations while simultaneously producing renewable products.This approach is seen as a viable method for constructing a new carbon cycle,thereby effectively addressing the issue of global warming.Photothermal CO_(2)conversion has recently emerged as a promising research focus due to its high energy utilization efficiency,superior CO_(2)conversion,excellent product selectivity,mild operating conditions,low energy consumption and minimal operating costs.Cerium oxide(CeO_(2))has been widely used in photothermal catalysis due to its unique chemical properties,particularly when used as a support material with supported metals,creating distinctive interfacial sites for catalytic reactions.As an emerging star support in photothermal CO_(2)conversion,its contributions are equally significant and should not be overlooked.However,to our knowledge,there has been no comprehensive review of CeO_(2)applications in catalytic hydrogenation of CO_(2).In this paper,we summarize and discuss CeO_(2)-based materials for photothermal CO_(2)conversion to value-added products.This research particularly focuses on the synthesis methods of CeO_(2)-supported catalysts,the history of CeO_(2)in photothermal catalysis,types of photothermal catalytic reactors,unique characterization methods for the photothermal catalysts and the photothermal CO_(2)hydrogenation reactions by CeO_(2)-based catalysts.Perspectives related to further challenges and future directions for photothermal CO_(2)hydrogenation are also provided.
出处 《Nano Research》 SCIE EI 2025年第1期30-49,共20页 纳米研究(英文版)
基金 supported by the National Natural Science Foundation of China(Nos.22172069 and 22106085).
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