摘要
Taking South Lake and Jingyue Pool in Changchun as examples, we determined particulate Hg in ambient air and Hg concentration in precipitation. Results indicated that particulate Hg in air and Hg concentration in precipitation in both sites in nonheating period were lower than that in heating period, which is influenced by coal combustion. The annual particulate Hg concentrations of South Lake and Jingyue Pool were 0.254ng/m3 and 0.109ng/m3. The yearly average Hg concentrations in precipitation were 0.268μg/L(South Lake) and 0.108μg/L(Jingyue Pool). The higher particulate Hg concentration in air and Hg concentration in precipitation in South Lake than that of Jingyue Pool indicated that mercury deposition was influenced by anthropogenic sources(especially from coas combustion). Hg concentration in precipitation is related with particulate Hg in the atmosphere. Dry deposition fluxes were estimated by using dry deposition model on the base of particulate Hg concentrations in the atmosphere, they were 35.5μg/(m2.a) for South lake and 15.3μg/(m2.a) for Jingyue Pool. Combined with precipitation amount, wet deposition fluxes were estimated in these two sites, 152.2μg/(m2.a) for South Lake and 61.2μg/(m2.a) for Jingyue Pool. Atmospheric Hg deposition fluxes were 160.2g/a for South Lake and 328.62g/a for Jingyue Pool.
Taking South Lake and Jingyue Pool in Changchun as examples, we determinedparticulate Hg in ambient air and Hg concentration in precipitation. Results indicated thatparticulate Hg in air and Hg concentration in precipitation in both sites in nonheating period werelower than that in heating period, which is influenced by coal combustion. The annual particulate Hgconcentrations of South Lake and Jingyue Pool were 0. 254ng/m^3 and 0. 109ng/m^3. The yearlyaverage Hg concentrations in precipitation were 0. 268μg/L(South Lake) and 0. 108μg/L(JingyuePool). The higher particulate Hg concentration in air and Hg concentration in precipitation in SouthLake than that of Jingyue Pool indicated that mercury deposition was influenced by anthropogenicsources (especially from coas combustion). Hg concentration in precipitation is related withparticulate Hg in the atmosphere. Dry deposition fluxes were estimated by using dry deposition modelon the base of particulate Hg concentrations in the atmosphere, they were 35. 5μg/ (m^2. a) forSouth lake and 15. 3μg/(m^2. a) for Jingyue Pool. Combined with precipitation amount, wetdeposition fluxes were estimated in these two sites, 152. 2μg/(m^2. a) for South Lake and 61.2μg/(m^2. a) for Jingyue Pool. Atmospheric Hg deposition fluxes were 160. 2g/a for South Lake and328. 62g/a for Jingyue Pool.
基金
UndertheauspicesoftheNationalNaturalScienceFoundationofChina(No.40071072)
WetlandsInnovationoftheChineseAcademyofSciences(KZCX2-302)andthedirectorfundofChangchunInstituteofGeography
theChineseAcademyofSciences.
