期刊文献+

Thermodynamic Study on the Catalytic Partial Oxidation of Methane to Syngas 被引量:5

Thermodynamic Study on the Catalytic Partial Oxidation of Methane to Syngas
下载PDF
导出
摘要 The catalytic partial oxidation of methane to syngas (CO+H2) has been simulated thermodynamically with the advanced process simulator PRO/Ⅱ. The influences of temperature,pressure,CH4/O2 ratio and steam addition in feed gas on the conversion of CH4 selectively to syngas and heat duty required were investigated, and their effects on carbon formation were also discussed. The simulation results were in good agreement with the literature data taken from a spouted bed reactor. the catalytic partial oxidation of methane to syngas (CO + H_2)has been simulated thermodynamically with the advanced processsimulator PRO/II. The influences of temperature, pressure, CH_4/O_2ratio and steam addition in feed gas on the conversion of CH_4selectively to syngas and eat duty required were investigated, andtheir effects on carbon formation were also discussed. The simulationresults were in good agreement with the literature data taken from aspouted bed reactor.
出处 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2002年第1期56-62,共7页 中国化学工程学报(英文版)
基金 the China National Petroleum Co. (CNPC).
关键词 热力学 部分氧化催化 甲烷 合成气 methane partial oxidation syngas thermodynamic simulation
  • 相关文献

参考文献16

  • 1Haggin, J., "Direct conversionof methane to fuels: chemicals still intensively sought", Oil Gas J., 70 (17),33-35(1992).
  • 2Rostrup-Nielsen, J. R., "Production of synthesis gas",Catal. Today, 18(4), 305-324 (1993).
  • 3Lange, L. P., Tijm, P. J. A., "Processes for converting methane to liquidfuels: Economic screening through energy management", Chem. Eng. Sci., 51 (10),2379-2387(1996).
  • 4Tindall, B. M., Crews, M. A., "Alternative technologies to steam-methanereforming", Hydrocarbon Processing, 74(11), 75-80 (1995).
  • 5Farina, G. L., Supp, E., "Produce syngas for methanol",HydrocarbonProcessing, 77 (3), 77-79 (1992).
  • 6Foulds, G. A., Lapszewicz, J. A., "Catalytic partial oxidation of methane tosynthesis gas (syngas)", Catalysis, 11,412-440 (1994).
  • 7Vermeiren, W. J. M., Blomsma, E., Jacobs. P. A., "Catalytic and thermodynamicapproach of the oxyreforming reaction of methane", Catal. Today, 13 (2-3),427-436(1992).
  • 8Tang, S. C., Claridge, J. B., Green, M. L. H., "Recent advances in theconversion of methane to synthesis gas",Catal. Today, 23 (1), 3-15 (1995).
  • 9Marschall, K. J., Mleczko, L., "Short-contact-time reactor for catalyticpartial oxidation of methane", Ind. Eng.Chem. Res., 38 (5), 1813-1821 (1999).
  • 10Marnasidou, K. G., Voutetakis, S. S., Tjatjopoulos, G. J.,Vasalos, Ⅰ. A.,"Catalytic partial oxidation of methane to synthesis gas in a pilot-plant-scalespouted-bed reactor",Chem. Eng. Sci., 54 (15-16), 3691-3699 (1999).

同被引文献46

引证文献5

二级引证文献17

相关作者

内容加载中请稍等...

相关机构

内容加载中请稍等...

相关主题

内容加载中请稍等...

浏览历史

内容加载中请稍等...
;
使用帮助 返回顶部