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甲烷预混火焰中芳香烃及多环芳烃形成的数值模拟 被引量：4

Numerical Simulation of Aromatic and Polycyclic Aromatic Hydrocarbon Formation in Premixed Methane Flame
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摘要 利用一种详细的化学动力学模型,模拟了甲烷层流预混火焰中芳香烃及多环芳烃(PAHs)的形成.结果表明,数值模拟与实验数据吻合得较好,可以用于预测同类型火焰中芳香烃及PAHs的形成.对不同工况条件下火焰的数值模拟结果显示,火焰当量比、压力对芳香烃及PAHs形成都有影响. Detailed chemical kinetic modeling was performed to investigate aromatic and polycyclic aromatic hydrocarbons (PAHs) formation in a rich, sooting, methane premixed flame. By comparing modeling results with the experimental data, the model shows its perfect validity in simulating this type of flames. Employing this model, the impacts of pressure and oxygen concentration were investigated.
作者 刘晓飞 钟北京 傅维标
机构地区 清华大学工程力学系
出处 《燃烧科学与技术》 EI CAS CSCD 2003年第3期214-218,共5页 Journal of Combustion Science and Technology
基金 国家重点基础研究发展规划(973)资助项目(2002CB211602).
关键词 预混火焰 多环芳烃 数值模拟 Computer simulation Mathematical models Polycyclic aromatic hydrocarbons Reaction kinetics
分类号 TK223.21 [动力工程及工程热物理—动力机械及工程] O643.12 [理学—物理化学]
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参考文献12

  • 1Kennedy I M. Models of soot formation and oxidation [ J ]. Progress in Energy and Combustion Science, 1997,23:95-132.
  • 2Richter H, Howard J B. Formation of polycyclic aromatic hydrocarbons and their growth to soot-a review of chemical reaction pathways [ J ].Progress in Energy and Combustion Science,2000,26:565-608.
  • 3Frenklach M,Clary D W, Gardiner J et al. Detailed kinetic modeling of soot formation on shock-tube pyrolysis of acetylene [ A ]. Twentieth Symposium ( International ) on Combustion [ C ]. Pittsburgh, PA : Combustion Institute, 1985. 887-901.
  • 4Frenklach M,Warnatz J. Detailed modeling of PAH profiles in a sooting low-pressure acetylene flame [ J ]. Combustion Science and Technology, 1987,51:265-283.
  • 5Frenklach M, Wang H. Detailed mechanism and modeling of soot particle formation [ A ]. In: Beckhorn H. Soot Formation in Combustion[ C]. Springer-Verlag, Berlin, 1994. 162-190.
  • 6Wang H, Frenklach M. A detailed kinetic modeling study of aromatics formation in laminar premixed acetylene and ethylene flames [ J ].Combustion and Flame, 1997,110 : 173-221.
  • 7Appel J, Bockhom H, Frenklach M. Kinetic modeling of soot formation with detailed chemistry and physics :laminar premixed flames of C2 hydrocarbons[ J]. Combustion and Flame ,2000,121 : 122-136.
  • 8Marinov N M, Pitz W J, Westbrook C K et al. Modeling of aromatic and polycyclic aromatic hydrocarbon formation in premixed methane and ethane flames [ J]. Combustion Science and Technology, 1996:116-117 ;211-287.
  • 9Xu F, Lin K C, Faeth G M. Soot formation in laminar premixed methane/oxygen flames at atmospheric pressure [ J ]. Combustion and Flame, 1998,115 : 195-209.
  • 10Frenklach M, Wang H, Goldenberg Met al. GRI-Mech-An Optimized Detailed Chemical Reaction Mechanism for Methane Combustion[ R]. Gas Research Institute Report GRI-95/0058, Chicago: IL,1995.

同被引文献64

  • 1曹玉春,严建华,李晓东,池涌,岑可法.乙烷预混火焰多环芳烃生成动力学模拟[J].中国电机工程学报,2005,25(16):84-89. 被引量：2
  • 2尹雪峰,李晓东,陆胜勇,尤孝方,谷月玲,严建华,倪明江,岑可法.大型电站燃煤锅炉多环芳烃排放特性[J].中国电机工程学报,2007,27(5):1-6. 被引量：8
  • 3Richter H,Howard J B,Frank P.Computationalinvestigation of PAH and soot formation in premixedethylene flames[C]//Proceedings of the EuropeanCombustion Meeting,Louvain-la-Neuve,Belgien,2005.
  • 4Lee S M,Yoon S S,Chung S H,et al.Synergistic effecton soot formation in counterflow diffusion flames ofethylene–propane mixtures with benzene addition[J].Combustion and Flame,2004,136(4):493-494.
  • 5Litzinger T,Santoro R,Linevsky M,et al.Reduction ofPAH and soot in premixed ethylene-air flames by additionof ethanol[J].Combustion and Flames,2006,144(4):675-687.
  • 6Healy D,Donato N S,Aul C J,et al.n-Butane:Ignitiondelay measurements at high pressure and detailedchemical kinetic simulations[J].Combustion and Flame,2010,157(8):1526-1539.
  • 7Marinov N M,Pitz W J,Westbrook C K,et al.Aromaticand polycyclic aromatic hydrocarbon formation in alaminar premixed n-butane flame[J].Combustion andFlame,1998,114(1-2):192-213.
  • 8Simmie J M.Detailed chemical kinetic models for thecombustion of hydrocarbon fuels[J].Progress in Energyand Combustion Science,2003,29(6):599-634.
  • 9Smith G P,Golden D M,Frenklach M,et al.GRI-MECH3.0[EB/OL].Available from:http://www.me.Berkeley.edu/gri_mech/version30/.
  • 10Anna A D,Sirignano M,Commodo M,et al.Anexperimental and modeling study of particulate formationin premixed flames burning methane[J].CombustionScience and Technology,2008,180(5):950-958.

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燃烧科学与技术
2003年 第3期

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