摘要
The geochemical behaviors of dissolved (<0.4 mm), low molecular weight (<10 kDa) and colloidal (10 kDa- 0.4 mm) 210Po in surface waters from the Jiulongjiang estuary were examined and the input/removal rates of different 210Po species were estimated. Both dissolved and low molecular weight 210Po were considerably removed during estuarine mixing. However, colloidal 210Po was removed only at low salinity regions (S <15) but had input behavior at high salin-ity surface waters (S >15). The input/removal rates of three species indicate that 210Po was removed rapidly in the Jiu-longjiang estuary. The discrepancy of input/removal rates between 210Po species suggests different geochemical be-havior and a dynamic transformation between 210Po species. Low molecular weight 210Po may be more appropriate for characterizing the 210Po behavior in estuary zone than the traditional dissolved 210Po.
The geochemical behaviors of dissolved (<0.4 mm), low molecular weight (<10 kDa) and colloidal (10 kDa- 0.4 mm) 210Po in surface waters from the Jiulongjiang estuary were examined and the input/removal rates of different 210Po species were estimated. Both dissolved and low molecular weight 210Po were considerably removed during estuarine mixing. However, colloidal 210Po was removed only at low salinity regions (S <15) but had input behavior at high salin-ity surface waters (S >15). The input/removal rates of three species indicate that 210Po was removed rapidly in the Jiu-longjiang estuary. The discrepancy of input/removal rates between 210Po species suggests different geochemical be-havior and a dynamic transformation between 210Po species. Low molecular weight 210Po may be more appropriate for characterizing the 210Po behavior in estuary zone than the traditional dissolved 210Po.
基金
supported by the National Natural Science Foundation of China(Grant No.40076024)
the 10th Five-Year Plan of COMRA(Grant Nos.DY 105-02-4,DY 105-02-01 and DY 105-01-04-11).
