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含锆双金属试剂的合成与应用

Formation of the Complex Having a Zirconium-Silicon Bond or a Zirconium\|Stannum Bond and Their Applications
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摘要 　论述了锆-硅、锆-锡等含锆双金属试剂的合成方法及其在有机合成中的应用. A review with 24 references reporting the formation of the complex that has a zirconium|silicon bond or a zirconium|stannum bond and their applications.
作者 钟平 黄南平
机构地区 温州师范学院化学与材料科学学院
出处 《甘肃科学学报》 2004年第2期33-37,共5页 Journal of Gansu Sciences
基金 国家自然科学基金(20272043) 浙江省自然科学基金(201015)资助课题
关键词 锆 硅 锡 双金属试剂 合成 应用 zirconium silicon stannum metal-metal bond formation application
分类号 O627 [理学—有机化学]
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参考文献28

  • 1孙秀丽,王佰全,徐善生,周秀中,赵健,胡友良.柄型金属有机化合物(Ⅳ)——四甲基二硅桥连取代环戊二烯基钛和锆化合物的合成及催化乙烯聚合[J].高等学校化学学报,2000,21(2):222-226. 被引量：12
  • 2Takahashi T, Hasegawa M. Suzuki N. et al. Zirconium-catalyzed Highly Regioselective Hydrosilation Reaction of Alkenes and x-ray Structures of Silyl(hydrido)zirconocene Derivatives[J]. J Am Chem Soc. 1991, 113(22):8564-8566.
  • 3Ellis J E. Yuen P, Jang M. New Classes of Zerovalent Zirconium Carbonyls and Related Species. Structural Characterizations of [Zr (CO)5(SnMe3)2]2- and [Zr(CO)4(dppe)SnMe3]- , dppe=Ph2PCH2CH2PPh2[J]. J Organomet Chem, 1996, 507(1-2):283-286.
  • 4Tilley T D. Insertion of Carbon Monoxide Into a Transition metal-silicon Bond. X-ray Structure of the Silaacyl Chloro(trimethylsilylη 2-carbonyl)bis(η5-cyclopentadienyl)zirconium[J]. J Am Chem Soc. 1985, 107(13):4084-4085.
  • 5Campion B K, Falk J. Tilley T D. Reactions of Carbon Monoxide with Trimethylsilyl and Tris(trimethylsilyl)silyl Derivatives of Group 4 Metals. Synthesis. Characterization, and Reactivity of Silaacyl Complexes[J]. J Am Chem Soc, 1987, 109(7) :2049-2056.
  • 6Liu X, Wu Z, Cai H, Concolino T E, et al. Reactions of Tetrakis(dimethylamide)-Titanium, -Zirconium and -Hafnium with Silanes:Synthesis of Unusual Amide Hydride Complexes and Mechanistic Studies of Titanium-Silicon-Nitride (Ti-Si-N) Formation[J]. J Am Che
  • 7Schumann H, Zietzke K, Weimann R, et al. Synthesis, Crystal Structure and Catalytic Activity of Some New Chiral Ansa-metallocenes of Yttrium, Lanthanum, Samarium. Lutetium and of Zirconium[J]. J Organomet Chem,1999, 574(2):228-240.
  • 8Duchateau R, Cremer U, Harmsen R J, et al. Half-sandwith Group 4 Metal Siloxy and Silsesquioxane Complexes: Soluble Model Systems for Silica-grafted Olefin Polymerization Catalysts[J]. Organometallics, 1999, 18(16):5447-5459.
  • 9Mitchell T N.Wichenkamo R.Amamria A.et al.Formation and Reactions of Olefins with Vicinal Silvl and Stannvl Substituents[J].J Org Chem,1987,52(22) :4868-4874.
  • 10Joyce Y C. Janet B W. Reactions of Hydrosilanes with Transition Metal Complexes: Formation of Stable Transition-metal Silyl Compounds[J]. Chem Rev, 1999, 99(1) :175-292.

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甘肃科学学报
2004年 第2期

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