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Synthesis of Chiral Schiff Base Metal Complex Inducing CD and Elucidation of Structure of Adsorption on Surface of Gold Nanoparticles 被引量：1

Synthesis of Chiral Schiff Base Metal Complex Inducing CD and Elucidation of Structure of Adsorption on Surface of Gold Nanoparticles
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摘要 We have prepared supramolecular systems of chiral Schiff base Ni(II), Cu(II), Zn(II) complexes and colloidal gold nanoparticles (AuNP) of 10 nm diameters. They demonstrated that direct adsorption of chiral Schiff base metal complex on the surface of AuNP owing to observation of clear induced CD spectra for the first time. We observed and discussed induced CD bands on AuNP from chiral Schiff base Ni(II), Cu(II), Zn(II) complexes. We have prepared supramolecular systems of chiral Schiff base Ni(II), Cu(II), Zn(II) complexes and colloidal gold nanoparticles (AuNP) of 10 nm diameters. They demonstrated that direct adsorption of chiral Schiff base metal complex on the surface of AuNP owing to observation of clear induced CD spectra for the first time. We observed and discussed induced CD bands on AuNP from chiral Schiff base Ni(II), Cu(II), Zn(II) complexes.
作者 Minako Oshima Minoru Matsuno Tsutsumi Yuki Sunaga Nobumitsu Tomoyuki Haraguchi Takashiro Akitsu
机构地区 Department of Chemistry
出处 《International Journal of Organic Chemistry》 2017年第2期153-170,共18页 有机化学国际期刊（英文）
关键词 CHIRAL SCHIFF Base Metal Complex Gold Nanoparticle Chiral Schiff Base Metal Complex Gold Nanoparticle
分类号 O6 [理学—化学]
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  • 1Humbury, G. A.; Borovkov, V. V.; Inoue, Y. Chirality-Sensing Supramolecular Systems. Chem. Soc. Rev. 2008, 108, 1-72.
  • 2Crassous, J. Chiral Transfer in Coordination Complexes: Towards Molecular Materials. Chem. Soc. Rev. 2009, 38, 830-845.
  • 3Slocik, J. M.; Govorov, A. O.; Naik, R. R. Plasmonic Circular Dichroism of Peptide-Functionalized Gold Nanoparticles. Nano Lett. 2011, 11, 701-705.
  • 4Schipper, P. E. Use of Dispersion-lnduced Circular Dichroism (DICD) in Spectroscopic Assignment: Applications to Copper(II) Complexes. J. Am. Chem. Soc. 1976, 98, 7938-7944.
  • 5Akitsu, T.; Ishioka, C.; Itoh, T. Polarized Spectroscopy of Hybrid Materials of Mn2 Single-Molecule Magnet and Azobenzene or Disperse Red 1 in PMMA Films. Cent. Eur. J. Chem. 2009, 7, 690-696.
  • 6Akitsu, T.; Itoh, T. Polarized Spectroscopy of Hybrid Materials of Chiral Schiff Base Cobalt(II), Nickel(II), Copper(II), and Zinc(II) Complexes and Photochromic Azobenzenes in PMMA Films. Polyhedron. 2010, 29, 477-487.
  • 7Aritake, Y.; Takanashi, T.; Polarized Spectroscopy and Yamazaki, A.; Akitsu, T. Hybrid Materials of Chiral Schiff Base Ni(II), Cu(II), Zn(II) Complexes with Included or Separated Azo-Groups. Polyhedron. 2011, 30 886-894.
  • 8Aritake, Y.; Akitsu, T. The Role of Chiral Dopants in Organic/Inorganic Hybrid Materials Containing Chiral Schiff Base Ni(II), Cu(II), and Zn(II) Complexes. Polyhedron. 2012, 31, 278-284.
  • 9Yamazaki, A.; Akitsu, T. Polarized Spectroscopy and Polarized UV Light-Induced Molecular Orientation of Chiral Diphenyl Schiff Base Ni(II) and Cu(II) Complexes and Azobenzene in a PMMA Film. RSC Advances. 2012, 2. 2975-2980.
  • 10Akitsu, T.; Uchida, N.; Aritake, Y.; Yamaguchi, J. Induced D-D Bands in CD Spectra due to Chiral Transfer from Chiral Nickel(II) Complexes to Achiral Copper(II) Complexes and Application for Structural Estimation. Trends in Inorg. Chem. 2008, 10, 41-49.

引证文献1

International Journal of Organic Chemistry
2017年 第2期

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