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Natural Radioactivity and Excess Lifetime Cancer Risk Associated with Soil in Kargi Area, Marsabit-Kenya

Natural Radioactivity and Excess Lifetime Cancer Risk Associated with Soil in Kargi Area, Marsabit-Kenya
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摘要 The main aim of investigating activity concentrations together with distribution of radionuclides naturally in soil from Kargi was to evaluate radiological health hazard together with environmental radioactivity. Research shows radionuclides as one source of exposure due to radiation with detrimental effects health wise for populations found in areas considered high background radiation. After collecting 117 soil samples from the area, analysis was done in order to measure their natural radioactivities due to <sup>40</sup>K, <sup>232</sup>Th and <sup>226</sup>Ra radionuclides. Measurements method of gamma spectrometry employing a high purity germanium (HPGe) detector was employed basically to evaluate the radiological hazard of radioactivities. For <sup>40</sup>K, <sup>232</sup>Th and <sup>226</sup>Ra, mean calculated activities were 353.19 ± 110.07, 7.98 ± 3.98 and 7.37 ± 2.60 Bq<span style="white-space:nowrap;">·</span>kg <sup>-1</sup> respectively. Mean values of absorbed and effective dose rates, external and internal hazard indices together with radium equivalent activity were 23.82 ± 6.59 nGy<span style="white-space:nowrap;">·</span>h <sup>-1</sup> and 0.14 ± 0.04 mSv<span style="white-space:nowrap;">·</span>y <sup>-1</sup>, 0.12 ± 0.03 and 0.14 ± 0.04 and 45.90 ± 12.65 Bq<span style="white-space:nowrap;">·</span>kg <sup>-1</sup> respectively. Comparing with approved global values, the values were found to be below the given global limits. Evidence of involvement of metasomatic activity of the radioelements or fractionation during weathering is seen as calculations give a higher value Th/U. Excess cancer risk, calculated from the samples showed lower values as compared to global standard values hence minimal chance of getting cancer disease. The area is safe from cancer causing radionuclides. The main aim of investigating activity concentrations together with distribution of radionuclides naturally in soil from Kargi was to evaluate radiological health hazard together with environmental radioactivity. Research shows radionuclides as one source of exposure due to radiation with detrimental effects health wise for populations found in areas considered high background radiation. After collecting 117 soil samples from the area, analysis was done in order to measure their natural radioactivities due to <sup>40</sup>K, <sup>232</sup>Th and <sup>226</sup>Ra radionuclides. Measurements method of gamma spectrometry employing a high purity germanium (HPGe) detector was employed basically to evaluate the radiological hazard of radioactivities. For <sup>40</sup>K, <sup>232</sup>Th and <sup>226</sup>Ra, mean calculated activities were 353.19 ± 110.07, 7.98 ± 3.98 and 7.37 ± 2.60 Bq<span style="white-space:nowrap;">·</span>kg <sup>-1</sup> respectively. Mean values of absorbed and effective dose rates, external and internal hazard indices together with radium equivalent activity were 23.82 ± 6.59 nGy<span style="white-space:nowrap;">·</span>h <sup>-1</sup> and 0.14 ± 0.04 mSv<span style="white-space:nowrap;">·</span>y <sup>-1</sup>, 0.12 ± 0.03 and 0.14 ± 0.04 and 45.90 ± 12.65 Bq<span style="white-space:nowrap;">·</span>kg <sup>-1</sup> respectively. Comparing with approved global values, the values were found to be below the given global limits. Evidence of involvement of metasomatic activity of the radioelements or fractionation during weathering is seen as calculations give a higher value Th/U. Excess cancer risk, calculated from the samples showed lower values as compared to global standard values hence minimal chance of getting cancer disease. The area is safe from cancer causing radionuclides.
作者 Willis Ougo Aguko Robert Kinyua John Gitonga Githiri Willis Ougo Aguko;Robert Kinyua;John Gitonga Githiri(Physics Department, School of Physical Sciences, College of Pure & Applied Sciences, Jomo Kenyatta University of Agriculture and Technology, Nairobi, Kenya)
机构地区 Physics Department
出处 《Journal of Geoscience and Environment Protection》 2020年第12期127-143,共17页 地球科学和环境保护期刊(英文)
关键词 Kargi-Marsabit Nuclear Science Gamma-Ray Spectrometry Lifetime Cancer Risk ACTIVITY Kargi-Marsabit Nuclear Science Gamma-Ray Spectrometry Lifetime Cancer Risk Activity
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