We report a systematic study on layered metal SrCu_(4-x)P_(2) single crystals via transport, magnetization, thermodynamic measurements and structural characterization. We find that the crystals show large linear magne...We report a systematic study on layered metal SrCu_(4-x)P_(2) single crystals via transport, magnetization, thermodynamic measurements and structural characterization. We find that the crystals show large linear magnetoresistance without any sign of saturation with a magnetic field up to 30T. We also observe a phase transition with significant anomalies in resistivity and heat capacity at T_(p)~140 K. Thermal expansion measurement reveals a subtle lattice parameter variation near Tp, i.e.,?L_(c)/L_(c)~0.062%. The structural characterization confines that there is no structure transition below and above T_(p). All these results suggest that the nonmagnetic transition of SrCu_(4-x)P_(2) could be associated with structural distortion.展开更多
Recent experimental and theoretical work has focused on two-dimensional van der Waals(2D vdW)magnets due to their potential applications in sensing and spintronics devises.In measurements of these emerging materials,c...Recent experimental and theoretical work has focused on two-dimensional van der Waals(2D vdW)magnets due to their potential applications in sensing and spintronics devises.In measurements of these emerging materials,conventional magnetometry often encounters challenges in characterizing the magnetic properties of small-sized vdW materials,especially for antiferromagnets with nearly compensated magnetic moments.Here,we investigate the magnetism of 2D antiferromagnet CrPS_(4)with a thickness of 8nm by using dynamic cantilever magnetometry(DCM).展开更多
We report a systematic investigation on c-axis point-contact Andreev reflection (PCAR) in BaFe2-xNixAs2 superconducting single crystals from underdoped to overdoped regions (0.075≤ x ≤0.15). At low temperatures,...We report a systematic investigation on c-axis point-contact Andreev reflection (PCAR) in BaFe2-xNixAs2 superconducting single crystals from underdoped to overdoped regions (0.075≤ x ≤0.15). At low temperatures, an in-gap sharp peak at low-bias voltage is observed in PCAR for overdoped samples, in contrast to the case of underdoped junctions, in which an in-gap plateau is observed. The variety of the conductance spectra with doping can be well described by using a generalized Blonder-Tinkham-Klapwijk formalism with an angle-dependent gap. This gap shows a clear crossover from a nodeless in the underdoped side to a nodal feature in the overdoped region. This result provides evidence of the doping-induced evolution of the superconducting order parameter when the inter-pocket and intra-pocket scattering are tuned through doping, as expected in the s± scenario.展开更多
The electronic and superconducting properties of Fe_(1-δ)Se single-crystal flakes grown hydrothermally are studied by the transport measurements under zero and high magnetic fields up to 38.5 T.The results contrast s...The electronic and superconducting properties of Fe_(1-δ)Se single-crystal flakes grown hydrothermally are studied by the transport measurements under zero and high magnetic fields up to 38.5 T.The results contrast sharply with those previously reported for nematically ordered Fe Se by chemical-vapor-transport(CVT)growth.No signature of the electronic nematicity,but an evident metal-to-nonmetal crossover with increasing temperature,is detected in the normal state of the present hydrothermal samples.Interestingly,a higher superconducting critical temperature T_c of 13.2 K is observed compared to a suppressed T_c of 9 K in the presence of the nematicity in the CVT Fe Se.Moreover,the upper critical field in the zero-temperature limit is found to be isotropic with respect to the field direction and to reach a higher value of-42 T,which breaks the Pauli limit by a factor of 1.8.展开更多
Low-temperature specific heat Cp is measured on Ba(Fe1-xCox)2As2 single crystals in a wide doping region. A sizeable residual specific heat coefficient γo is observed in the low temperature limit of all samples. Th...Low-temperature specific heat Cp is measured on Ba(Fe1-xCox)2As2 single crystals in a wide doping region. A sizeable residual specific heat coefficient γo is observed in the low temperature limit of all samples. The specific heat jump near Tc, i.e. ΔCp/T/T_c, is also determined. It is found that -γo, ΔCp/T/T_c and Tc all share a similar evolution with doping. These can be well understood within the model of S± pairing symmetry when accounting for the cobalt-dopants as unitary scattering centers in the FeAs planes. Our results reveal a non-trivial impact of impurity scattering in FeAs-based.展开更多
The compounds composed of transition metal cations and pnictide anions provide a rich platform for studying novel physical phenomena.Here we report on the observation of a phase transition at~70 K and 145 K in layered...The compounds composed of transition metal cations and pnictide anions provide a rich platform for studying novel physical phenomena.Here we report on the observation of a phase transition at~70 K and 145 K in layered compound EuCu_(4)As_(2)and SrCu_(4)As_(2),respectively.from both the transport and heat capacity.The thermal expansion measurements show that the variation of the lattice parameters(△L_(b)/L_(ab))around T_(P) is much less than that for a typical crystalline phase transition.Our experimental results reveal that the transition in EuCu_(4)As_(2)and SrCu_(4)As_(2)should be driven by subtle structural-distortion.展开更多
基金Project supported by the National Key Research and Development Program of China (Grant Nos.2023YFA1607403,2021YFA1600201,and 2022YFA1602603)the Natural Science Foundation of China (Grant Nos.U19A2093,U2032214,and U2032163)+5 种基金the Collaborative Innovation Program of Hefei Science Center,CAS (Grant No.2019HSC-CIP 001)the Youth Innovation Promotion Association of CAS (Grant No.2021117)the Natural Science Foundation of Anhui Province (No.1908085QA15)the HFIPS Director’s Fund (Grant No.YZJJQY202304)the CASHIPS Director’s Fund (Grant No.YZJJ2022QN36)supported by the High Magnetic Field Laboratory of Anhui Province。
文摘We report a systematic study on layered metal SrCu_(4-x)P_(2) single crystals via transport, magnetization, thermodynamic measurements and structural characterization. We find that the crystals show large linear magnetoresistance without any sign of saturation with a magnetic field up to 30T. We also observe a phase transition with significant anomalies in resistivity and heat capacity at T_(p)~140 K. Thermal expansion measurement reveals a subtle lattice parameter variation near Tp, i.e.,?L_(c)/L_(c)~0.062%. The structural characterization confines that there is no structure transition below and above T_(p). All these results suggest that the nonmagnetic transition of SrCu_(4-x)P_(2) could be associated with structural distortion.
基金supported by the National Key R&D Program of China(Grant No.2022YFA1602602)the National Natural Science Foundation of China(Grant Nos.12122411 and 12474053)+4 种基金CAS Project for Young Scientists in Basic Research(Grant No.YSBR-084)HFIPS Director’s Fund(Grant Nos.2023BR,YZJJ-GGZX-2022-03,and YZJJ202403TS)HFIPS Director’s Fud(Grant No.BJPY2021B05)the Basic Research Program of the Chinese Academy of Sciences Based on Major Scientific Infrastructures(Grant No.JZHKYPT-2021-08)the High Magnetic Field Laboratory of Anhui Province(Grant No.AHHM-FX2020-02)。
文摘Recent experimental and theoretical work has focused on two-dimensional van der Waals(2D vdW)magnets due to their potential applications in sensing and spintronics devises.In measurements of these emerging materials,conventional magnetometry often encounters challenges in characterizing the magnetic properties of small-sized vdW materials,especially for antiferromagnets with nearly compensated magnetic moments.Here,we investigate the magnetism of 2D antiferromagnet CrPS_(4)with a thickness of 8nm by using dynamic cantilever magnetometry(DCM).
基金Supported by the National Basic Research Program of China under Grant Nos 2011CBA00100 and 2012CB821404the Project of International Team on Superconductivity and Novel Electronic Materials of Chinese Academy of Sciences
文摘We report a systematic investigation on c-axis point-contact Andreev reflection (PCAR) in BaFe2-xNixAs2 superconducting single crystals from underdoped to overdoped regions (0.075≤ x ≤0.15). At low temperatures, an in-gap sharp peak at low-bias voltage is observed in PCAR for overdoped samples, in contrast to the case of underdoped junctions, in which an in-gap plateau is observed. The variety of the conductance spectra with doping can be well described by using a generalized Blonder-Tinkham-Klapwijk formalism with an angle-dependent gap. This gap shows a clear crossover from a nodeless in the underdoped side to a nodal feature in the overdoped region. This result provides evidence of the doping-induced evolution of the superconducting order parameter when the inter-pocket and intra-pocket scattering are tuned through doping, as expected in the s± scenario.
基金Supported by the National Key Research and Development Program of China (Grant Nos.2016YFA0300300 and 2017YFA0303003)the National Natural Science Foundation of China (Grant Nos.12061131005,11834016 and 11888101)+1 种基金the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No.XDB25000000)the Strategic Priority Research Program and Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (Grant Nos.QYZDY-SSW-SLH001)。
文摘The electronic and superconducting properties of Fe_(1-δ)Se single-crystal flakes grown hydrothermally are studied by the transport measurements under zero and high magnetic fields up to 38.5 T.The results contrast sharply with those previously reported for nematically ordered Fe Se by chemical-vapor-transport(CVT)growth.No signature of the electronic nematicity,but an evident metal-to-nonmetal crossover with increasing temperature,is detected in the normal state of the present hydrothermal samples.Interestingly,a higher superconducting critical temperature T_c of 13.2 K is observed compared to a suppressed T_c of 9 K in the presence of the nematicity in the CVT Fe Se.Moreover,the upper critical field in the zero-temperature limit is found to be isotropic with respect to the field direction and to reach a higher value of-42 T,which breaks the Pauli limit by a factor of 1.8.
基金Supported by the National Natural Science Foundation of China, the National Basic Research Program of China under Grant Nos 2006CB601000, 2006CB921107 and 2006CB921802, and the ITSNEM Project of Chinese Academy of Sciences.
文摘Low-temperature specific heat Cp is measured on Ba(Fe1-xCox)2As2 single crystals in a wide doping region. A sizeable residual specific heat coefficient γo is observed in the low temperature limit of all samples. The specific heat jump near Tc, i.e. ΔCp/T/T_c, is also determined. It is found that -γo, ΔCp/T/T_c and Tc all share a similar evolution with doping. These can be well understood within the model of S± pairing symmetry when accounting for the cobalt-dopants as unitary scattering centers in the FeAs planes. Our results reveal a non-trivial impact of impurity scattering in FeAs-based.
基金Project supported by the National Key Research and Development Program of China(Grant No.2021YFA1600201)the National Natural Science Foundation of China(Grant Nos.U19A2093,U2032214,U2032163,U1732274,11904002,and 11874359)+5 种基金the Collaborative Innovation Program of Hefei Science Center,Chinese Academy of Sciences(CAS)(Grant No.2019HSC-CIP 001)the Youth Innovation Promotion Association of CAS(Grant No.2021117)the Natural Science Foundation of Anhui Province,China(Grant No.1908085QA15)the Director Fund from the Hefei Institutes of Physical Science(HFIPS)(Grant No.YZJJQY202304)the Director Fund from the the Chinese Academy of Sciences and Hefei Institutes of Physical Science(CASHIPS),China(Grant No.E26MMG71131)the High Magnetic Field Laboratory of Anhui Province,China。
文摘The compounds composed of transition metal cations and pnictide anions provide a rich platform for studying novel physical phenomena.Here we report on the observation of a phase transition at~70 K and 145 K in layered compound EuCu_(4)As_(2)and SrCu_(4)As_(2),respectively.from both the transport and heat capacity.The thermal expansion measurements show that the variation of the lattice parameters(△L_(b)/L_(ab))around T_(P) is much less than that for a typical crystalline phase transition.Our experimental results reveal that the transition in EuCu_(4)As_(2)and SrCu_(4)As_(2)should be driven by subtle structural-distortion.