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Recent advances in core-shell organic framework-based photocatalysts for energy conversion and environmental remediation
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作者 Qibing Dong Ximing Li +9 位作者 Yanyan Duan Qingyun Tian Xinxin Liang Yiyin Zhu Lin Tian Junjun Wang atif sial Yongqian Cui Ke Zhao Chuanyi Wang 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第8期168-199,I0004,共33页
Direct conversion of solar energy into chemical energy in an environmentally friendly manner is one of the most promising strategies to deal with the environmental pollution and energy crisis.Among a variety of materi... Direct conversion of solar energy into chemical energy in an environmentally friendly manner is one of the most promising strategies to deal with the environmental pollution and energy crisis.Among a variety of materials developed as photocatalysts,the core-shell metal/covalent-organic framework(MOF or COF)photocatalysts have garnered significant attention due to their highly porous structure and the adjustability in both structure and functionality.The existing reviews on core-shell organic framework photocatalytic materials have mainly focused on core-shell MOF materials.However,there is still a lack of indepth reviews specifically addressing the photocatalytic performance of core-shell COFs and MOFs@COFs.Simultaneously,there is an urgent need for a comprehensive review encompassing these three types of core-shell structures.Based on this,this review aims to provide a comprehensive understanding and useful guidelines for the exploration of suitable core-shell organic framework photocatalysts towards appropriate photocatalytic energy conversion and environmental governance.Firstly,the classification,synthesis,formation mechanisms,and reasonable regulation of core-shell organic framework were summarized.Then,the photocatalytic applications of these three kinds of core-shell structures in different areas,such as H_(2)evolution,CO_(2)reduction,and pollutants degradation are emphasized.Finally,the main challenges and development prospects of core-shell organic framework photocatalysts were introduced.This review aims to provide insights into the development of a novel generation of efficient and stable core-shell organic framework materials for energy conversion and environmental remediation. 展开更多
关键词 Organic framework Core-shell structure PHOTOCATALYSIS Energy conversion Environmental remediation
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不同营养环境下棕鞭藻共栖细菌的群落结构比较 被引量:3
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作者 张波 刘珂轶 +3 位作者 张安龙 陈佳琛 高俊玲 atif sial 《环境科学学报》 CAS CSCD 北大核心 2020年第8期2812-2818,共7页
微藻富含油脂,可以用作合成生物柴油的原料,被认为是最具发展前景的生物质能源.微藻的光合培养体系往往是非纯培养体系,现有研究更多地关注微藻生物量的积累及其对废水环境的净化效果,而对体系中广泛存在的共栖细菌缺乏全面深入的认知.... 微藻富含油脂,可以用作合成生物柴油的原料,被认为是最具发展前景的生物质能源.微藻的光合培养体系往往是非纯培养体系,现有研究更多地关注微藻生物量的积累及其对废水环境的净化效果,而对体系中广泛存在的共栖细菌缺乏全面深入的认知.本文通过对棕鞭藻共栖细菌的16S rDNA基因进行高通量测序分析,研究棕鞭藻(Ochromonas)在生活废水、BG11及Glu+BG11(BG11中添加10 g·L^-1葡萄糖)3种不同营养环境中共栖细菌的群落结构差异,进而阐明有机物及复杂废水环境对微藻共栖细菌群落结构的影响效果.结果表明,生活废水、BG11及Glu+BG11 3种营养环境中共栖细菌群落结构存在显著差异,生活废水体系中生物多样性显著高于BG11及Glu+BG11体系,生活废水中共栖细菌香浓(Shannon)多样性指数高达4.32,其次是BG11及Glu+BG11,Shannon指数分别为2.13、1.54.从共栖细菌群落的组成上看,3种营养环境中优势菌属差异显著,生活废水中优势菌属有芽殖杆菌属(Gemmobacter)、鞘脂单胞菌属(Sphingomonas)及玫瑰球菌属(Roseococcus),相对丰度分别为14.46%、14.9%、14.54%,其中,芽殖杆菌属只在生活废水中有较高丰度.BG11中寡养单胞菌属(Stenotrophomonas)与玫瑰球菌属的丰度分别高达26.86%、51.03%.Glu+BG11中寡养单胞菌属较BG11中显著增加,达到82.41%,而玫瑰球菌属较生活废水及BG11中则明显降低,菌群丰度仅为6.2%.对比3种营养环境,玫瑰球菌属均具有较高丰度,是棕鞭藻良好的共生菌. 展开更多
关键词 棕鞭藻 共栖细菌 高通量测序 群落结构
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