Two-dimensional material has been widely investigated for potential applications in sensor and flexible electronics.In this work,a self-powered flexible humidity sensing device based on poly(vinyl alcohol)/Ti_(3)C_(2)...Two-dimensional material has been widely investigated for potential applications in sensor and flexible electronics.In this work,a self-powered flexible humidity sensing device based on poly(vinyl alcohol)/Ti_(3)C_(2)Tx(PVA/MXene)nanofibers film and monolayer molybdenum diselenide(MoSe2)piezoelectric nanogenerator(PENG)was reported for the first time.The monolayer MoSe_(2)-based PENG was fabricated by atmospheric pressure chemical vapor deposition techniques,which can generate a peak output of 35 mV and a power density of42 mW m^(-2).The flexible PENG integrated on polyethylene terephthalate(PET)substrate can harvest energy generated by different parts of human body and exhibit great application prospects in wearable devices.The electrospinned PVA/MXene nanofiber-based humidity sensor with flexible PET substrate under the driven of monolayer MoSe_(2) PENG,shows high response of~40,fast response/recovery time of 0.9/6.3 s,low hysteresis of 1.8%and excellent repeatability.The self-powered flexible humidity sensor yields the capability of detecting human skin moisture and ambient humidity.This work provides a pathway to explore the high-performance humidity sensor integrated with PENG for the self-powered flexible electronic devices.展开更多
Two-dimensional(2D)nanomaterials have been widely used in gas sensing due to their large specific surface area,high surface reactivity,and excellent gas adsorption properties.This paper reviews the typical synthesis m...Two-dimensional(2D)nanomaterials have been widely used in gas sensing due to their large specific surface area,high surface reactivity,and excellent gas adsorption properties.This paper reviews the typical synthesis methods of various types of 2D nanomaterials and summarizes the recent progress in gas sensors based on 2D materials,such as noble metal nanoparticles(NPs),metal oxides(MOS),conductive polymers,other new 2D materials.The methods of doping,modification,and photoexcitation can effectively improve the gas-sensing properties of 2D materials.The sensitive mechanisms of heterojunction,Schottky junction,and photoexcitation in 2D material sensors are discussed in detail.This paper discusses the application prospects of 2D materials in wearable gas sensors,food safety,and self-powered sensing,and provides ideas for further applications in environmental quality monitoring and disease diagnosis.In addition,the opportunities and challenges for gas sensors based on 2D materials are also discussed.展开更多
基金supported by the National Natural Science Foundation of China(51777215)National Natural Science Foundation of China(51775306)+1 种基金Beijing Municipal Natural Science Foundation(4192027)the Graduate Innovation Fund of China University of Petroleum(YCX2020097)。
文摘Two-dimensional material has been widely investigated for potential applications in sensor and flexible electronics.In this work,a self-powered flexible humidity sensing device based on poly(vinyl alcohol)/Ti_(3)C_(2)Tx(PVA/MXene)nanofibers film and monolayer molybdenum diselenide(MoSe2)piezoelectric nanogenerator(PENG)was reported for the first time.The monolayer MoSe_(2)-based PENG was fabricated by atmospheric pressure chemical vapor deposition techniques,which can generate a peak output of 35 mV and a power density of42 mW m^(-2).The flexible PENG integrated on polyethylene terephthalate(PET)substrate can harvest energy generated by different parts of human body and exhibit great application prospects in wearable devices.The electrospinned PVA/MXene nanofiber-based humidity sensor with flexible PET substrate under the driven of monolayer MoSe_(2) PENG,shows high response of~40,fast response/recovery time of 0.9/6.3 s,low hysteresis of 1.8%and excellent repeatability.The self-powered flexible humidity sensor yields the capability of detecting human skin moisture and ambient humidity.This work provides a pathway to explore the high-performance humidity sensor integrated with PENG for the self-powered flexible electronic devices.
基金the National Natural Science Foundation of China(No.51777215)the Original Innovation Special Project of Science and Technology Plan of Qingdao West Coast New Area(No.2020-85)the Special Foundation of the Taishan Scholar Project.
文摘Two-dimensional(2D)nanomaterials have been widely used in gas sensing due to their large specific surface area,high surface reactivity,and excellent gas adsorption properties.This paper reviews the typical synthesis methods of various types of 2D nanomaterials and summarizes the recent progress in gas sensors based on 2D materials,such as noble metal nanoparticles(NPs),metal oxides(MOS),conductive polymers,other new 2D materials.The methods of doping,modification,and photoexcitation can effectively improve the gas-sensing properties of 2D materials.The sensitive mechanisms of heterojunction,Schottky junction,and photoexcitation in 2D material sensors are discussed in detail.This paper discusses the application prospects of 2D materials in wearable gas sensors,food safety,and self-powered sensing,and provides ideas for further applications in environmental quality monitoring and disease diagnosis.In addition,the opportunities and challenges for gas sensors based on 2D materials are also discussed.