Motivated by recent realizations of spin-1 NaRb mixtures in the experiments[Phys.Rev.Lett.114,255301(2015);Phys.Rev.Lett.128,223201(2022)],we investigate heteronuclear magnetism in the Mott-insulating regime.Different...Motivated by recent realizations of spin-1 NaRb mixtures in the experiments[Phys.Rev.Lett.114,255301(2015);Phys.Rev.Lett.128,223201(2022)],we investigate heteronuclear magnetism in the Mott-insulating regime.Different from the identical mixtures where the boson statistics only admits even parity states from angular momentum composition,for heteronuclear atoms in principle all angular momentum states are allowed,which can give rise to new magnetic phases.While various magnetic phases can be developed over these degenerate spaces,the concrete symmetry breaking phases depend on not only the degree of degeneracy but also the competitions from many-body interactions.We unveil these rich phases using the bosonic dynamical mean-field theory approach.These phases are characterized by various orders,including spontaneous magnetization order,spin magnitude order,singlet pairing order,and nematic order,which may coexist specially in the regime with odd parity.Finally we address the possible parameter regimes for observing these spin-ordered Mott phases.展开更多
The flexible superhydrophobic thermoplastic polyurethane(TPU)porous material was prepared by heat-induced phase separation method with two cooling steps.The influence of the preparation process on the microstructure o...The flexible superhydrophobic thermoplastic polyurethane(TPU)porous material was prepared by heat-induced phase separation method with two cooling steps.The influence of the preparation process on the microstructure of the material was discussed in depth.The microstructure,hydrophobicity and specific surface area of porous TPU materials were analyzed in detail.The surface wettability,separation selectivity,saturated adsorption capacity and adsorption rate,mechanical properties,environmental adaptability and cyclic properties of porous TPU materials were studied.The results show that the TPU-8%porous monolithic material prepared by heat-induced phase separation method shows good performance when the polymer concentration is 8%,the phase separation temperature is 0℃,the phase separation time is 30min,and the mixing solvent ratio is 9:1.展开更多
As a potential candidate for quantum computation and metrology,the nitrogen vacancy(NV)center in diamond presents both challenges and opportunities resulting from charge-state conversion.By utilizing different lasers ...As a potential candidate for quantum computation and metrology,the nitrogen vacancy(NV)center in diamond presents both challenges and opportunities resulting from charge-state conversion.By utilizing different lasers for the photon-induced charge-state conversion,we achieved subdiffraction charge-state manipulation.The charge-state depletion(CSD)microscopy resolution was improved to 4.1 nm by optimizing the laser pulse sequences.Subsequently,the electron spin-state dynamics of adjacent NV centers were selectively detected via the CSD.The experimental results demonstrated that the CSD can improve the spatial resolution of the measurement of NV centers for nanoscale sensing and quantum information.展开更多
This paper discusses the developement and investigation of a silica microbubble resonator(MBR) that is optimized to cancel mode dispersion with material dispersion, at a wavelength of approximately 1550 nm and maintai...This paper discusses the developement and investigation of a silica microbubble resonator(MBR) that is optimized to cancel mode dispersion with material dispersion, at a wavelength of approximately 1550 nm and maintain a quality factor of an optical mode as large as 5.4 × 10~7. Benefitting from the near-zero dispersion and high quality factor, a primary optical comb is generated in the MBR using cascaded four-wave mixing processes, which span over 300 nm with several tens of teeth. Furthermore, the frequency comb could be gradually tuned by mechanically stretching the MBR. This tunable Kerr comb has multiple potential applications in precision measurements and sensing applications, such as molecular spectroscopy and ranging.展开更多
Metasurfaces have proven themselves an exotic ability to harness light at nano-scale,being important not only for classical but also for quantum optics.Dynamic manipulation of the quantum states is at the heart of qua...Metasurfaces have proven themselves an exotic ability to harness light at nano-scale,being important not only for classical but also for quantum optics.Dynamic manipulation of the quantum states is at the heart of quantum information processing;however,such function has been rarely realized with metasurfaces so far.Here,we report an all-optical dynamic modulation of the photonic quantum states using the nonlinear metasurface.The metasurface consists of a metallic nanostructure combined with a photoisomerizable azo layer.By tuning the plasmonic resonance through optically switching the azo molecules between their binary isomeric states,we have realized dynamic control of transmission efficiencies of orthogonally polarized photons and also the phase delay between them,thereby an entangled state was efficiently controlled.As an illustration,a quantum state distillation has been demonstrated to recover a Bell state from a non-maximally entangled one to that with fidelities higher than 98%.Our work would enrich the functions of the metasurface in the quantum world,from static to dynamic modulation,making the quantum metasurface going practical.展开更多
Quantum teleportation can transfer an unknown quantum state between distant quantum nodes,which holds great promise in enabling large-scale quantum networks.To advance the full potential of quantum teleportation,quant...Quantum teleportation can transfer an unknown quantum state between distant quantum nodes,which holds great promise in enabling large-scale quantum networks.To advance the full potential of quantum teleportation,quantum states must be faithfully transferred at a high rate over long distance.Despite recent impressive advances,a high-rate quantum teleportation system across metropolitan fiber networks is extremely desired.Here,we demonstrate a quantum teleportation system which transfers quantum states carried by independent photons at a rate of 7.1±0.4 Hz over 64-km-long fiber channel.An average single-photon fidelity of≥90.6±2.6%is achieved,which exceeds the maximum fidelity of 2/3 in classical regime.Our result marks an important milestone towards quantum networks and opens the door to exploring quantum entanglement based informatic applications for the future quantum internet.展开更多
We develop a new spectroscopic method to quickly and intuitively characterize the coupling of two microwave-photon-coupled semiconductor qubits via a high-impedance resonator.Highly distinctive and unique geometric pa...We develop a new spectroscopic method to quickly and intuitively characterize the coupling of two microwave-photon-coupled semiconductor qubits via a high-impedance resonator.Highly distinctive and unique geometric patterns are revealed as we tune the qubit tunnel couplings relative to the frequency of the mediating photons.These patterns are in excellent agreement with a simulation using the Tavis-Cummings model,and allow us to readily identify different parameter regimes for both qubits in the detuning space.This method could potentially be an important component in the overall spectroscopic toolbox for quickly characterizing certain collective properties of multiple cavity quantum electrodynamics(QED)coupled qubits.展开更多
The ultracold molecule is a promising candidate for versatile quantum tasks due to its long-range interaction and rich internal rovibrational states.With the help of the cavity quantum electrodynamics(QED)effects,an o...The ultracold molecule is a promising candidate for versatile quantum tasks due to its long-range interaction and rich internal rovibrational states.With the help of the cavity quantum electrodynamics(QED)effects,an optical cavity can be employed to increase the efficiency of the formation of the photoassociated molecules and offers a non-demolition detection of the internal states of molecules.Here,we demonstrate the production of the high-finesse optical fiber microcavity for the Rb_(2) molecule cavity QED experiment,which includes the fabrication of fiber-based cavity mirrors,testing,and the assembly of ultra-high vacuum-compatible optical fiber microcavity.The optical fiber microcavity offers high cooperativity between cavity mode and ultracold molecule and paves the way for the study of molecule cavity QED experimental research.展开更多
Microwave sensing offers important applications in areas such as data communication and remote sensing.It has thus received much attention from academia,industry,and governments.Atomic wireless sensing uses the strong...Microwave sensing offers important applications in areas such as data communication and remote sensing.It has thus received much attention from academia,industry,and governments.Atomic wireless sensing uses the strong response of the large electric dipole moment of a Rydberg atom in response to an external field to achieve precise measurement of a radio frequency(RF)signal.This method offers advantages over traditional wireless sensing including ultrawide energy level transitions,which makes it responsive to RF electric fields over a wide bandwidth.Here,we briefly review the progress of electric field measurement based on Rydberg atoms.We discuss the properties of Rydberg atoms,measurement using Rydberg atoms,experimental progress in electric field measurement of different bands,and different methods for detecting electric fields(such as atomic superheterodyne,machine learning,and critically enhanced measurement).The development of Rydberg atomic measurement focuses on the advantages of Rydberg atomic sensing,especially when compared to conventional microwave receivers.This work is of major significance to developing Rydberg-based measurements in astronomy,remote sensing,and other fields.展开更多
Loss is inevitable for the optical system due to the absorption of materials, scattering caused by the defects, and surface roughness. In quantum optical circuits, the loss can not only reduce the intensity of the sig...Loss is inevitable for the optical system due to the absorption of materials, scattering caused by the defects, and surface roughness. In quantum optical circuits, the loss can not only reduce the intensity of the signal, but also affect the performance of quantum operations. In this work, we divide losses into unbalanced linear losses and shared common losses, and provide a detailed analysis on how loss affects the integrated linear optical quantum gates. It is found that the orthogonality of eigenmodes and the unitary phase relation of the coupled waveguide modes are destroyed by the loss. As a result, the fidelity of single-and two-qubit operations decreases significantly as the shared loss becomes comparable to the coupling strength. Our results are important for the investigation of large-scale photonic integrated quantum information processes.展开更多
The Kibble-Zurek(KZ)mechanism has played a fundamental role in defect formation with universal scaling laws in nonequilibrium phase transitions.However,this theory may not accurately predict the scaling laws in inhomo...The Kibble-Zurek(KZ)mechanism has played a fundamental role in defect formation with universal scaling laws in nonequilibrium phase transitions.However,this theory may not accurately predict the scaling laws in inhomogeneous systems and slow quenching processes.Here,we present a generalized KZ mechanism for the defect formation in trapped ions with the freeze-out condition gt=b0τ(t),where g is a universal quenching velocity function and b0 is a constant.We derived a differential equationφ(x,t)to account for the frozen correlation length of a kink in an inhomogeneous system and demonstrated a smooth crossover from a fast quenching process to a slow quenching process,which agrees well with the experiments performed by Ulm et al.[Nat.Commun.4,2290(2013)]and Pyka et al.[Nat.Commun.4,2291(2013)].Furthermore,we confirmed our theoretical model using molecular dynamics simulation by solving the stochastic differential equation,showing excellent agreement with the results from the differential equation.Our theory provides a general theoretical framework for studying KZ physics in inhomogeneous systems,which has applications in other nonequilibrium platforms studied experimentally.展开更多
With high integration density and excellent optical properties, silicon photonics is becoming a promising platform for complete integration and large-scale optical quantum information processing. Scalable quantum info...With high integration density and excellent optical properties, silicon photonics is becoming a promising platform for complete integration and large-scale optical quantum information processing. Scalable quantum information applications need photon generation and detection to be integrated on the same chip, and we have seen that various devices on the silicon photonic chip have been developed for this goal. This paper reviews the relevant research results and state-of-the-art technologies on the silicon photonic chip for scalable quantum applications. Despite the shortcomings, the properties of some components have already met the requirements for further expansion. Furthermore, we point out the challenges ahead and future research directions for on-chip scalable quantum information applications.展开更多
基金supported by the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB0500000)the Innovation Program for Quantum Science and Technology(Grant No.2021ZD0301200)+1 种基金the National Natural Science Foundation of China(Grant Nos.12074431,12274384,and 12374252)the Excellent Youth Foundation of Hunan Scientific Committee(Grant No.2021JJ10044).
文摘Motivated by recent realizations of spin-1 NaRb mixtures in the experiments[Phys.Rev.Lett.114,255301(2015);Phys.Rev.Lett.128,223201(2022)],we investigate heteronuclear magnetism in the Mott-insulating regime.Different from the identical mixtures where the boson statistics only admits even parity states from angular momentum composition,for heteronuclear atoms in principle all angular momentum states are allowed,which can give rise to new magnetic phases.While various magnetic phases can be developed over these degenerate spaces,the concrete symmetry breaking phases depend on not only the degree of degeneracy but also the competitions from many-body interactions.We unveil these rich phases using the bosonic dynamical mean-field theory approach.These phases are characterized by various orders,including spontaneous magnetization order,spin magnitude order,singlet pairing order,and nematic order,which may coexist specially in the regime with odd parity.Finally we address the possible parameter regimes for observing these spin-ordered Mott phases.
基金We acknowledge the fnancial support from the Research Project of Keyi College of Zhejiang Sci-Tech University(KY2021001)the National Natural Science Foundation of Zhejiang Province China(LY15B030002).
文摘The flexible superhydrophobic thermoplastic polyurethane(TPU)porous material was prepared by heat-induced phase separation method with two cooling steps.The influence of the preparation process on the microstructure of the material was discussed in depth.The microstructure,hydrophobicity and specific surface area of porous TPU materials were analyzed in detail.The surface wettability,separation selectivity,saturated adsorption capacity and adsorption rate,mechanical properties,environmental adaptability and cyclic properties of porous TPU materials were studied.The results show that the TPU-8%porous monolithic material prepared by heat-induced phase separation method shows good performance when the polymer concentration is 8%,the phase separation temperature is 0℃,the phase separation time is 30min,and the mixing solvent ratio is 9:1.
基金This study was financially supported by the National Basic Research Program of China(Grant No.2011CB921200)the Knowledge Innovation Project of Chinese Academy of Sciences(Grant No.60921091)+3 种基金the National Natural Science Foundation of China(Grant No.11374290)the Program for New Century Excellent Talents in Universitythe Fundamental Research Funds for the Central Universitiesthe Foundation for the Author of National Excellent Doctoral Dissertation of China.
文摘As a potential candidate for quantum computation and metrology,the nitrogen vacancy(NV)center in diamond presents both challenges and opportunities resulting from charge-state conversion.By utilizing different lasers for the photon-induced charge-state conversion,we achieved subdiffraction charge-state manipulation.The charge-state depletion(CSD)microscopy resolution was improved to 4.1 nm by optimizing the laser pulse sequences.Subsequently,the electron spin-state dynamics of adjacent NV centers were selectively detected via the CSD.The experimental results demonstrated that the CSD can improve the spatial resolution of the measurement of NV centers for nanoscale sensing and quantum information.
基金supported by the National Key R&D Program of China(Grant No.2016YFA0301303)the Anhui Initiative in Quantum Information Technologies(Grant No.AHY130200)+2 种基金the National Natural Science Foundation of China(Grant Nos.11934012,61575184,and 11722436)the Fundamental Research Funds for the Central Universitiesthe Key Science and Technology Program of Henan Province,China(Grant No.182102410070)。
文摘This paper discusses the developement and investigation of a silica microbubble resonator(MBR) that is optimized to cancel mode dispersion with material dispersion, at a wavelength of approximately 1550 nm and maintain a quality factor of an optical mode as large as 5.4 × 10~7. Benefitting from the near-zero dispersion and high quality factor, a primary optical comb is generated in the MBR using cascaded four-wave mixing processes, which span over 300 nm with several tens of teeth. Furthermore, the frequency comb could be gradually tuned by mechanically stretching the MBR. This tunable Kerr comb has multiple potential applications in precision measurements and sensing applications, such as molecular spectroscopy and ranging.
基金This work was supported by Guangdong Major Project of Basic and Applied Basic Research(2020B0301030009)National Key R&D Program of China(2017YFA0305100,2017YFA0303800,2019YFA0705000)+8 种基金National Natural Science Foundation of China(92050114,12174202,11774333,91750204,62061160487,12004373,61775106,11904182,12074200,11774185)The Hong Kong Research Grant Council(AoE/P-502/20,17309021)Anhui Initiative in Quantum Information Technologies(AHY130300)The Strategic Priority Research Program of the Chinese Academy of Sciences(XDB24030601)111 Project(B07013)PCSIRT(IRT0149)Open Research Program of Key Laboratory of 3D Micro/NanoFabrication and Characterization of Zhejiang ProvinceFundamental Research Funds for the Central Universities(010-63201003,010-63201008,010-63201009,010-63211001)Tianjin Youth Talent Support Program.We thank the Nanofabrication Platform at Nankai University and USTC Center for sample fabrication.
文摘Metasurfaces have proven themselves an exotic ability to harness light at nano-scale,being important not only for classical but also for quantum optics.Dynamic manipulation of the quantum states is at the heart of quantum information processing;however,such function has been rarely realized with metasurfaces so far.Here,we report an all-optical dynamic modulation of the photonic quantum states using the nonlinear metasurface.The metasurface consists of a metallic nanostructure combined with a photoisomerizable azo layer.By tuning the plasmonic resonance through optically switching the azo molecules between their binary isomeric states,we have realized dynamic control of transmission efficiencies of orthogonally polarized photons and also the phase delay between them,thereby an entangled state was efficiently controlled.As an illustration,a quantum state distillation has been demonstrated to recover a Bell state from a non-maximally entangled one to that with fidelities higher than 98%.Our work would enrich the functions of the metasurface in the quantum world,from static to dynamic modulation,making the quantum metasurface going practical.
基金This work was supported by the National Key Research and Development Program of China(Nos.2018YFA0307400,2018YFA0306102)National Natural Science Foundation of China(Nos.61775025,91836102,U19A2076,62005039)+1 种基金Innovation Program for Quantum Science and Technology(No.2021ZD0301702)Sichuan Science and Technology Program(Nos.2021YFSY0066,2021YFSY0062,2021YFSY0063,2021YFSY0064,2021YFSY0065).The authors thank X.X.H,Y.X.L and L.B.Z from the Information Center of the University of Electronic Science and Technology of China(UESTC)for providing access to the campus fiber network and for the help during the experiment.
文摘Quantum teleportation can transfer an unknown quantum state between distant quantum nodes,which holds great promise in enabling large-scale quantum networks.To advance the full potential of quantum teleportation,quantum states must be faithfully transferred at a high rate over long distance.Despite recent impressive advances,a high-rate quantum teleportation system across metropolitan fiber networks is extremely desired.Here,we demonstrate a quantum teleportation system which transfers quantum states carried by independent photons at a rate of 7.1±0.4 Hz over 64-km-long fiber channel.An average single-photon fidelity of≥90.6±2.6%is achieved,which exceeds the maximum fidelity of 2/3 in classical regime.Our result marks an important milestone towards quantum networks and opens the door to exploring quantum entanglement based informatic applications for the future quantum internet.
基金supported by the National Key Research and Development Program of China(2016YFA0301700)the National Natural Science Foundation of China(61922074,11674300,61674132,11625419 and 11804327)+2 种基金the Strategic Priority Research Program of the CAS(XDB24030601)the Anhui Initiative in Quantum Information Technologies(AHY080000)financial support by U.S.ARO through Grant No.W911NF1410346 and No.W911NF1710257。
文摘We develop a new spectroscopic method to quickly and intuitively characterize the coupling of two microwave-photon-coupled semiconductor qubits via a high-impedance resonator.Highly distinctive and unique geometric patterns are revealed as we tune the qubit tunnel couplings relative to the frequency of the mediating photons.These patterns are in excellent agreement with a simulation using the Tavis-Cummings model,and allow us to readily identify different parameter regimes for both qubits in the detuning space.This method could potentially be an important component in the overall spectroscopic toolbox for quickly characterizing certain collective properties of multiple cavity quantum electrodynamics(QED)coupled qubits.
基金supported by the National Key Research and Development Program of China(No.2017YFA0304100)National Natural Science Foundation of China(Nos.11804330 and 11821404)the Fundamental Research Funds for the Central Universities。
文摘The ultracold molecule is a promising candidate for versatile quantum tasks due to its long-range interaction and rich internal rovibrational states.With the help of the cavity quantum electrodynamics(QED)effects,an optical cavity can be employed to increase the efficiency of the formation of the photoassociated molecules and offers a non-demolition detection of the internal states of molecules.Here,we demonstrate the production of the high-finesse optical fiber microcavity for the Rb_(2) molecule cavity QED experiment,which includes the fabrication of fiber-based cavity mirrors,testing,and the assembly of ultra-high vacuum-compatible optical fiber microcavity.The optical fiber microcavity offers high cooperativity between cavity mode and ultracold molecule and paves the way for the study of molecule cavity QED experimental research.
基金supported by the National Key R&D Program of China(Grant No.2022YFA140400)the National Natural Science Foundation of China(Grant Nos.U20A20218,61525504,and 61435011)the Youth Innovation Promotion Association of the Chinese Academy of Sciences(Grant No.2018490).
文摘Microwave sensing offers important applications in areas such as data communication and remote sensing.It has thus received much attention from academia,industry,and governments.Atomic wireless sensing uses the strong response of the large electric dipole moment of a Rydberg atom in response to an external field to achieve precise measurement of a radio frequency(RF)signal.This method offers advantages over traditional wireless sensing including ultrawide energy level transitions,which makes it responsive to RF electric fields over a wide bandwidth.Here,we briefly review the progress of electric field measurement based on Rydberg atoms.We discuss the properties of Rydberg atoms,measurement using Rydberg atoms,experimental progress in electric field measurement of different bands,and different methods for detecting electric fields(such as atomic superheterodyne,machine learning,and critically enhanced measurement).The development of Rydberg atomic measurement focuses on the advantages of Rydberg atomic sensing,especially when compared to conventional microwave receivers.This work is of major significance to developing Rydberg-based measurements in astronomy,remote sensing,and other fields.
基金supported by the National Natural Science Foundation of China(Nos.11374289,61590932,and 61505195)the National Key R&D Program(Nos.2016YFA0301700 and 2016YFA0301300)+2 种基金the Innovation Funds from the Chinese Academy of Sciences(No.60921091)the Fundamental Research Funds for the Central Universitiesthe Open Fund of the State Key Laboratory on Integrated Optoelectronics(IOSKL2015KF12)
文摘Loss is inevitable for the optical system due to the absorption of materials, scattering caused by the defects, and surface roughness. In quantum optical circuits, the loss can not only reduce the intensity of the signal, but also affect the performance of quantum operations. In this work, we divide losses into unbalanced linear losses and shared common losses, and provide a detailed analysis on how loss affects the integrated linear optical quantum gates. It is found that the orthogonality of eigenmodes and the unitary phase relation of the coupled waveguide modes are destroyed by the loss. As a result, the fidelity of single-and two-qubit operations decreases significantly as the shared loss becomes comparable to the coupling strength. Our results are important for the investigation of large-scale photonic integrated quantum information processes.
基金supported by the National Natural Science Foundation of China(Grant Nos.11904099,and 11774328)Natural Science Foundation of Hunan Province of China(Grant No.2021JJ30210)Innovation Program for Quantum Science and Technology(Grant Nos.2021ZD0301600,2021ZD0301200,and 2021ZD0301500)。
文摘The Kibble-Zurek(KZ)mechanism has played a fundamental role in defect formation with universal scaling laws in nonequilibrium phase transitions.However,this theory may not accurately predict the scaling laws in inhomogeneous systems and slow quenching processes.Here,we present a generalized KZ mechanism for the defect formation in trapped ions with the freeze-out condition gt=b0τ(t),where g is a universal quenching velocity function and b0 is a constant.We derived a differential equationφ(x,t)to account for the frozen correlation length of a kink in an inhomogeneous system and demonstrated a smooth crossover from a fast quenching process to a slow quenching process,which agrees well with the experiments performed by Ulm et al.[Nat.Commun.4,2290(2013)]and Pyka et al.[Nat.Commun.4,2291(2013)].Furthermore,we confirmed our theoretical model using molecular dynamics simulation by solving the stochastic differential equation,showing excellent agreement with the results from the differential equation.Our theory provides a general theoretical framework for studying KZ physics in inhomogeneous systems,which has applications in other nonequilibrium platforms studied experimentally.
基金National Natural Science Foundation of China(12004373,61974168,62005239,62061160487,62075243)Innovation Program for Quantum Science and Technology(2021ZD0303200)+3 种基金Natural Science Foundation of Zhejiang Province(LQ21F050006)National Key Research and Development Program of China(2017YFA0305200)Key Research and Development Program of Guangdong Province of China(2018B030325001,2018B030329001)China Postdoctoral Science Foundation(2021T140647).
文摘With high integration density and excellent optical properties, silicon photonics is becoming a promising platform for complete integration and large-scale optical quantum information processing. Scalable quantum information applications need photon generation and detection to be integrated on the same chip, and we have seen that various devices on the silicon photonic chip have been developed for this goal. This paper reviews the relevant research results and state-of-the-art technologies on the silicon photonic chip for scalable quantum applications. Despite the shortcomings, the properties of some components have already met the requirements for further expansion. Furthermore, we point out the challenges ahead and future research directions for on-chip scalable quantum information applications.