An experiment for studying the effects of sediment dredging on denitrification in sediments was carried out through a one-year incubation of undredged (control) and dredged cores in laboratory. Dredging the upper 30...An experiment for studying the effects of sediment dredging on denitrification in sediments was carried out through a one-year incubation of undredged (control) and dredged cores in laboratory. Dredging the upper 30 cm of sediment can significantly affect physico-chemical characteristics of sediments. Less degradation of organic matter in the dredged sediments was found during the experiment. Denitrification rates in the sediments were estimated by the acetylene blockage technique, and ranged from 21.6 to 102.7 nmol N2/(g dry weight (dw)-hr) for the undredged sediment and from 6.9 to 26.9 nmol N2/(g dw-hr) for dredged sediments. The denitrification rates in the undredged sediments were markedly higher (p 〈 0.05) than those in the dredged sediments throughout the incubation, with the exception of February 2006. The importance of various environmental factors on denitrification was assessed, which indicated that denitrification was regulated by temperature. Nitrate was probably the key factor limiting denitrification in both undredged and dredged sediments. Organic carbon played some role in determining the denitrification rates in the dredged sediments, but not in the undredged sediments. Sediment dredging influenced the mineralization of organic matter and denitrification in the sediment; and therefore changed the pattern of inherent cycling of nitrogen.展开更多
Due to the increasing power consumption of whole society and widely using of new non-linear and asymmetric electrical equipment,power quality assessment problem in the new period has attracted more and more attention....Due to the increasing power consumption of whole society and widely using of new non-linear and asymmetric electrical equipment,power quality assessment problem in the new period has attracted more and more attention.The mathematical essence of comprehensive assessment of power quality is a multiattribute optimal decision-making problem.In order to solve the key problem of determining the indicator weight in the process of power quality assessment,a rough analytic hierarchy process(AHP)is proposed to aggregate the judgment opinions of multiple experts and eliminate the subjective effects of single expert judgment.Based on the advantage of extension analysis for solving the incompatibility problem,extension analysis method is adopted to assess the power quality.The assessment grades of both total power quality and each assessment indicator are obtained by correlation function.Through a case of 110 kV bus of a converting station in a wind farm of China,the feasibility and effectiveness of the propose method are demonstrated.The result shows that the proposed method can determine the overall power quality of power grid,as well as compare the differences among the performance of assessment indicators and provide the basis for further improving of power quality.展开更多
Tea(Camellia sinensis[L.]O.Kuntze.)is an important cash crop,which mainly uses tender shoots and young leaves for manufacturing.Due to the marketing characteristic that earlier made tea has higher price,the time of th...Tea(Camellia sinensis[L.]O.Kuntze.)is an important cash crop,which mainly uses tender shoots and young leaves for manufacturing.Due to the marketing characteristic that earlier made tea has higher price,the time of the breaking of winter dormancy buds in spring is extremely important in tea industry.Strigolactones are a group of carotenoids-derived metabolites which regulates bud outgrowth,shoot branching,tiller angle and environmental stress responses.The role of strigolactones in tea plant was briefly summarized in the current review,with an emphasis of the association of strigolactones on bud ecodormancy and shoot branching.The involvement of strigolactones on the biosynthesis of the tea characteristic metabolites flavonoids,caffeine and theanine were also discussed.Moreover,recent advances on the biosynthesis of strigolactones and its regulation by microRNAs and environmental stresses were also presented.This review provides a basis for future investigations underlying the mechanisms of strigolactones on bud winter dormancy and tea secondary metabolism.展开更多
The main aim of this present note is to establish three new Hermite-Hadamard type integral inequalities for r-convex functions. The three new Hermite-Hadamard type integral inequalities for r-convex functions improve ...The main aim of this present note is to establish three new Hermite-Hadamard type integral inequalities for r-convex functions. The three new Hermite-Hadamard type integral inequalities for r-convex functions improve the result of original one by H?lder’s integral inequality, Stolarsky mean and convexity of function.展开更多
Residual magnetic error remains after standard levelling process.The weak non-geological effect,manifesting itself as streaky noise along flight lines,creates a challenge for airborne geophysical data processing and i...Residual magnetic error remains after standard levelling process.The weak non-geological effect,manifesting itself as streaky noise along flight lines,creates a challenge for airborne geophysical data processing and interpretation.Microleveling is the process to eliminate this residual noise and is now a standard areogeophysical data processing step.In this paper,we propose a two-step procedure for single aerogeophysical data microleveling:a deep convolutional network is first adopted as approximator to map the original data into a low-level part with nature geological structures and a corrugated residual which still contains high-level detail geological structures;second,the mixture of Gaussian robust principal component analysis(MoG-RPCA)is then used to separate the weak energy fine structures from the residual.The final microleveling result is the addition of low-level structures from deep convolutional network and fine structures from MoG-RPCA.The deep convolutional network does not need dataset for training and the handcrafted network serves as prior(deep image prior)to capture the low-level nature geological structures in the areogeophysical data.Experiments on synthetic data and field data demonstrate that the combination of deep convolutional network and MoG-RPCA is an effective framework for single areogeophysical data microleveling.展开更多
In-depth studies of hierarchical self-assembly with chirality inversion and asymmetry amplification are indispensable for understanding the chiral transfer rule in assembly systems and construction of circularly polar...In-depth studies of hierarchical self-assembly with chirality inversion and asymmetry amplification are indispensable for understanding the chiral transfer rule in assembly systems and construction of circularly polarized luminescence(CPL)active materials.Herein,a coordination-driven primary assembly of pyrene-based chiral ligand and Zn(OTf)2 was employed for the construction of homochiral metal–organic helicate with a triple helix structure,tunable emission color,and significant chirality amplification.More excitingly,the metal–organic helicate further assembled into well-ordered hierarchical nanoarchitectures with the aid of C–H⋯πinteraction andπ–πstacking,showing significant CPL enhancement and unexpected handedness inversion.Thus,the|glum|increased from 5.20×10^(−5) to 5.60×10^(−2),and the|gabs|rose from 3.80×10^(−4) to 1.04×10^(−2) over the entire hierarchical self-assembly process.The multiple supramolecular interactions not only endowed the resultant metal–organic helicate with efficient chirality transmission and tunable emission color but also guided the(supra)molecular building block of metal–organic helicate organizing into the hierarchically chiral nanoarchitecture in a directional manner.This work provides insight into the metal–organic helicate-mediated hierarchical self-assembly and aids the development of CPLactive materials with dynamic chirality modulation and enhanced chiroptical performance.展开更多
Excitation wavelength dependent(Ex-De) luminescent materials have attracted intense attention due to their great potential in multicolor bioimaging,dynamic anti-counterfeiting,and light emitting devices.However,it rem...Excitation wavelength dependent(Ex-De) luminescent materials have attracted intense attention due to their great potential in multicolor bioimaging,dynamic anti-counterfeiting,and light emitting devices.However,it remains a formidable challenge to construct an Ex-De luminescent biomaterial with green starting materials,excellent biocompatibility,good water solubility,and multiple color emission for dynamic cell imaging.In this work,nanocomposites based on the facile self-assembly strategy of bovine serum albumin(BSA) and Au(Ⅰ)-complex are rationally designed and synthesized to simultaneously present Ex-De fluorescence(429–516 nm) and decent phosphorescence(~615 nm) in a dilute aqueous solution.Combinatory analyses of spectroscopic and microscopic results reveal that the luminescent mechanism of Au(Ⅰ)-BSA nanocomposites is cluster-induced Ex-De fluorescence and metal-to-ligand charge transition(MLCT) based phosphorescence.Importantly,based on the excellent biocompatibility,water-solubility and color-tunable emission over the entire visible region(360–800 nm),the Au(Ⅰ)-BSA nanocomposites are successfully used for cell imaging with multiple and switchable colors on demand.What is more,the solid tablets of Au(Ⅰ)-BSA nanoparticles showed pressure-responsive luminescence and decent room temperature phosphorescence.This work provides an assembling-induced emission strategy for the design of water-soluble,non-cytotoxic,and color-tunable luminescent biomaterials based on the composite of protein and Au nanoparticles.展开更多
Adenosine triphosphate(ATP)is closely related to the pathogenesis of certain diseases,so the detection of trace ATP is of great significance to disease diagnosis and drug development.Graphene field-effect transistors(...Adenosine triphosphate(ATP)is closely related to the pathogenesis of certain diseases,so the detection of trace ATP is of great significance to disease diagnosis and drug development.Graphene field-effect transistors(GFETs)have been proven to be a promising platform for the rapid and accurate detection of small molecules,while the Debye shielding limits the sensitive detection in real samples.Here,a three-dimensional wrinkled graphene field-effect transistor(3D WG-FET)biosensor for ultra-sensitive detection of ATP is demonstrated.The lowest detection limit of 3D WG-FET for analyzing ATP is down to 3.01 aM,which is much lower than the reported results.In addition,the 3D WG-FET biosensor shows a good linear electrical response to ATP concentrations in a broad range of detection from 10 aM to 10 pM.Meanwhile,we achieved ultra-sensitive(LOD:10 aM)and quantitative(range from 10 aM to 100 fM)measurements of ATP in human serum.The 3D WG-FET also exhibits high specificity.This work may provide a novel approach to improve the sensitivity for the detection of ATP in complex biological matrix,showing a broad application value for early clinical diagnosis and food health monitoring.展开更多
基金supported by the National Natural Science Foundation of China (No.40730528,40901253)the Social Development Key Project and Natural Science Foundation of Jiangsu Province (No.BE2009603,BK2009333)the Knowledge Innovation Program of Chinese Academy of Sciences (No.CXNIGLAS200804)
文摘An experiment for studying the effects of sediment dredging on denitrification in sediments was carried out through a one-year incubation of undredged (control) and dredged cores in laboratory. Dredging the upper 30 cm of sediment can significantly affect physico-chemical characteristics of sediments. Less degradation of organic matter in the dredged sediments was found during the experiment. Denitrification rates in the sediments were estimated by the acetylene blockage technique, and ranged from 21.6 to 102.7 nmol N2/(g dry weight (dw)-hr) for the undredged sediment and from 6.9 to 26.9 nmol N2/(g dw-hr) for dredged sediments. The denitrification rates in the undredged sediments were markedly higher (p 〈 0.05) than those in the dredged sediments throughout the incubation, with the exception of February 2006. The importance of various environmental factors on denitrification was assessed, which indicated that denitrification was regulated by temperature. Nitrate was probably the key factor limiting denitrification in both undredged and dredged sediments. Organic carbon played some role in determining the denitrification rates in the dredged sediments, but not in the undredged sediments. Sediment dredging influenced the mineralization of organic matter and denitrification in the sediment; and therefore changed the pattern of inherent cycling of nitrogen.
文摘Due to the increasing power consumption of whole society and widely using of new non-linear and asymmetric electrical equipment,power quality assessment problem in the new period has attracted more and more attention.The mathematical essence of comprehensive assessment of power quality is a multiattribute optimal decision-making problem.In order to solve the key problem of determining the indicator weight in the process of power quality assessment,a rough analytic hierarchy process(AHP)is proposed to aggregate the judgment opinions of multiple experts and eliminate the subjective effects of single expert judgment.Based on the advantage of extension analysis for solving the incompatibility problem,extension analysis method is adopted to assess the power quality.The assessment grades of both total power quality and each assessment indicator are obtained by correlation function.Through a case of 110 kV bus of a converting station in a wind farm of China,the feasibility and effectiveness of the propose method are demonstrated.The result shows that the proposed method can determine the overall power quality of power grid,as well as compare the differences among the performance of assessment indicators and provide the basis for further improving of power quality.
基金This work was financially supported by the China Postdoctoral Science Foundation(2018M632821)the Open Fund of State Key Laboratory of Tea Plant Biology and Utilization(SKLTOF 20180105)+3 种基金China agriculture research system(CARS-19)Hubei Natural Science Foundation Project(2019CFB178)Natural Science Foundation of Hubei Academy of Agricultural Sciences(2021NKYJJ13)the Agricultural Science and Technology Innovation Project of Hubei Province(2019-620-000-001-24).
文摘Tea(Camellia sinensis[L.]O.Kuntze.)is an important cash crop,which mainly uses tender shoots and young leaves for manufacturing.Due to the marketing characteristic that earlier made tea has higher price,the time of the breaking of winter dormancy buds in spring is extremely important in tea industry.Strigolactones are a group of carotenoids-derived metabolites which regulates bud outgrowth,shoot branching,tiller angle and environmental stress responses.The role of strigolactones in tea plant was briefly summarized in the current review,with an emphasis of the association of strigolactones on bud ecodormancy and shoot branching.The involvement of strigolactones on the biosynthesis of the tea characteristic metabolites flavonoids,caffeine and theanine were also discussed.Moreover,recent advances on the biosynthesis of strigolactones and its regulation by microRNAs and environmental stresses were also presented.This review provides a basis for future investigations underlying the mechanisms of strigolactones on bud winter dormancy and tea secondary metabolism.
文摘The main aim of this present note is to establish three new Hermite-Hadamard type integral inequalities for r-convex functions. The three new Hermite-Hadamard type integral inequalities for r-convex functions improve the result of original one by H?lder’s integral inequality, Stolarsky mean and convexity of function.
文摘Residual magnetic error remains after standard levelling process.The weak non-geological effect,manifesting itself as streaky noise along flight lines,creates a challenge for airborne geophysical data processing and interpretation.Microleveling is the process to eliminate this residual noise and is now a standard areogeophysical data processing step.In this paper,we propose a two-step procedure for single aerogeophysical data microleveling:a deep convolutional network is first adopted as approximator to map the original data into a low-level part with nature geological structures and a corrugated residual which still contains high-level detail geological structures;second,the mixture of Gaussian robust principal component analysis(MoG-RPCA)is then used to separate the weak energy fine structures from the residual.The final microleveling result is the addition of low-level structures from deep convolutional network and fine structures from MoG-RPCA.The deep convolutional network does not need dataset for training and the handcrafted network serves as prior(deep image prior)to capture the low-level nature geological structures in the areogeophysical data.Experiments on synthetic data and field data demonstrate that the combination of deep convolutional network and MoG-RPCA is an effective framework for single areogeophysical data microleveling.
基金supported by the National Natural Science Foundation of China(grant no.22101208)the Fundamental Research Funds for the Central Universitiesthe Program for Professors of Special Appointment(Eastern Scholar)at Shanghai Institutions of Higher Learning.
文摘In-depth studies of hierarchical self-assembly with chirality inversion and asymmetry amplification are indispensable for understanding the chiral transfer rule in assembly systems and construction of circularly polarized luminescence(CPL)active materials.Herein,a coordination-driven primary assembly of pyrene-based chiral ligand and Zn(OTf)2 was employed for the construction of homochiral metal–organic helicate with a triple helix structure,tunable emission color,and significant chirality amplification.More excitingly,the metal–organic helicate further assembled into well-ordered hierarchical nanoarchitectures with the aid of C–H⋯πinteraction andπ–πstacking,showing significant CPL enhancement and unexpected handedness inversion.Thus,the|glum|increased from 5.20×10^(−5) to 5.60×10^(−2),and the|gabs|rose from 3.80×10^(−4) to 1.04×10^(−2) over the entire hierarchical self-assembly process.The multiple supramolecular interactions not only endowed the resultant metal–organic helicate with efficient chirality transmission and tunable emission color but also guided the(supra)molecular building block of metal–organic helicate organizing into the hierarchically chiral nanoarchitecture in a directional manner.This work provides insight into the metal–organic helicate-mediated hierarchical self-assembly and aids the development of CPLactive materials with dynamic chirality modulation and enhanced chiroptical performance.
基金supported by the National Natural Science Foundation of China(22101208,22125803,22020102006)the Fundamental Research Funds for the Central Universitiesthe Program for Professors of Special Appointment(Eastern Scholar)at Shanghai Institutions of Higher Learning。
文摘Excitation wavelength dependent(Ex-De) luminescent materials have attracted intense attention due to their great potential in multicolor bioimaging,dynamic anti-counterfeiting,and light emitting devices.However,it remains a formidable challenge to construct an Ex-De luminescent biomaterial with green starting materials,excellent biocompatibility,good water solubility,and multiple color emission for dynamic cell imaging.In this work,nanocomposites based on the facile self-assembly strategy of bovine serum albumin(BSA) and Au(Ⅰ)-complex are rationally designed and synthesized to simultaneously present Ex-De fluorescence(429–516 nm) and decent phosphorescence(~615 nm) in a dilute aqueous solution.Combinatory analyses of spectroscopic and microscopic results reveal that the luminescent mechanism of Au(Ⅰ)-BSA nanocomposites is cluster-induced Ex-De fluorescence and metal-to-ligand charge transition(MLCT) based phosphorescence.Importantly,based on the excellent biocompatibility,water-solubility and color-tunable emission over the entire visible region(360–800 nm),the Au(Ⅰ)-BSA nanocomposites are successfully used for cell imaging with multiple and switchable colors on demand.What is more,the solid tablets of Au(Ⅰ)-BSA nanoparticles showed pressure-responsive luminescence and decent room temperature phosphorescence.This work provides an assembling-induced emission strategy for the design of water-soluble,non-cytotoxic,and color-tunable luminescent biomaterials based on the composite of protein and Au nanoparticles.
基金support from the National Natural Science Foundation of China(Nos.12274058 and 12104085)Taishan Scholars Program of Shandong Province(No.tsqn201812104)+2 种基金the Natural Science Foundation of Shandong Province(No.ZR2021QA008)the Qingchuang Science and Technology Plan of Shandong Province(No.2019KJJ017)the project of the Talent Introduction of Dezhou University(No.2021xjrc101).
文摘Adenosine triphosphate(ATP)is closely related to the pathogenesis of certain diseases,so the detection of trace ATP is of great significance to disease diagnosis and drug development.Graphene field-effect transistors(GFETs)have been proven to be a promising platform for the rapid and accurate detection of small molecules,while the Debye shielding limits the sensitive detection in real samples.Here,a three-dimensional wrinkled graphene field-effect transistor(3D WG-FET)biosensor for ultra-sensitive detection of ATP is demonstrated.The lowest detection limit of 3D WG-FET for analyzing ATP is down to 3.01 aM,which is much lower than the reported results.In addition,the 3D WG-FET biosensor shows a good linear electrical response to ATP concentrations in a broad range of detection from 10 aM to 10 pM.Meanwhile,we achieved ultra-sensitive(LOD:10 aM)and quantitative(range from 10 aM to 100 fM)measurements of ATP in human serum.The 3D WG-FET also exhibits high specificity.This work may provide a novel approach to improve the sensitivity for the detection of ATP in complex biological matrix,showing a broad application value for early clinical diagnosis and food health monitoring.