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Mixed 2D-Dion–Jacobson/3D Sn-Pb alloyed perovskites for efficient photovoltaic solar devices
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作者 Zhili Lu Chaohui Li +5 位作者 hongwei lai Xinming Zhou Chunfeng Wang Xianhu Liu Fei Guo Caofeng Pan 《Nano Research》 SCIE EI CSCD 2023年第2期3142-3148,共7页
Tin-lead(Sn-Pb)alloyed perovskites with tunable bandgaps hold great potential for constructing highly efficient single-junction and tandem photovoltaic devices.However,the efficiency and stability of Sn-Pb perovskite ... Tin-lead(Sn-Pb)alloyed perovskites with tunable bandgaps hold great potential for constructing highly efficient single-junction and tandem photovoltaic devices.However,the efficiency and stability of Sn-Pb perovskite solar cells(PSCs)are greatly hampered by severe nonradiative recombination due to the easy oxidation of Sn(II).In this work,we report the construction of mixed dimensional two-dimensional(2D)Dion–Jacobson(DJ)and three-dimensional(3D)perovskites to improve the efficiency and stability of Sn-Pb alloyed PSCs.Introducing a small amount of 1,4-butanediammonium diiodide as spacer cations of DJ perovskites into precursor,the prepared mixed dimensional Sn-Pb alloyed perovskites exhibit reduced trap-state density due to the passivation of 2D DJ perovskites.As a result,nonradiative charge recombination is greatly suppressed.The prepared Sn-Pb alloyed PSCs based on 2D-DJ/3D heterojunction deliver a power conversion efficiency of 19.02%with an impressive fill factor of 80%.As well,improved device stability is realized due to the presence of DJ perovskites which serves as a protection barrier against oxidation and water invasion. 展开更多
关键词 Sn-Pb perovskite narrow bandgap Dion–Jacobson perovskite solar cells two-dimensional(2D)/three-dimensional(3D)
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Advanced non-precious electrocatalyst of the mixed valence CoO_x nanocrystals supported on N-doped carbon nanocages for oxygen reduction 被引量:5
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作者 Sheng Chen Liwei Wang +8 位作者 Qiang Wu Xiang Li Yu Zhao hongwei lai Lijun Yang Tao Sun Yi Li Xizhang Wang Zheng Hu 《Science China Chemistry》 SCIE EI CAS CSCD 2015年第1期180-186,共7页
Taking advantage of the nitrogen(N)-participation and large surface area of N-doped carbon nanocages(NCNCs),the Co Ox nanocrystals are conveniently immobilized onto the NCNCs with high dispersion.The Co Ox/NCNCs hybri... Taking advantage of the nitrogen(N)-participation and large surface area of N-doped carbon nanocages(NCNCs),the Co Ox nanocrystals are conveniently immobilized onto the NCNCs with high dispersion.The Co Ox/NCNCs hybrid exists in the mixed valence with predominant Co O over Co3O4 and demonstrates superb oxygen reduction reaction activity and stability remaining^94%current density even after operation over 100 h.These results suggest a promising strategy to develop advanced electrocatalysts with the novel NCNCs or even beyond. 展开更多
关键词 cobalt oxide nanocrystals fuel cells non-precious electrocatalysts nitrogen doped carbon nanocages oxygen reductionreaction
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