An extraordinary and unprecedented heatwave swept across western North America(i.e.,the Pacific Northwest)in late June of 2021,resulting in hundreds of deaths,a massive die-off of sea creatures off the coast,and horri...An extraordinary and unprecedented heatwave swept across western North America(i.e.,the Pacific Northwest)in late June of 2021,resulting in hundreds of deaths,a massive die-off of sea creatures off the coast,and horrific wildfires.Here,we use observational data to find the atmospheric circulation variabilities of the North Pacific and Arctic-Pacific-Canada patterns that co-occurred with the development and mature phases of the heatwave,as well as the North America pattern,which coincided with the decaying and eastward movement of the heatwave.Climate models from the Coupled Model Intercomparison Project(Phase 6)are not designed to simulate a particular heatwave event like this one.Still,models show that greenhouse gases are the main reason for the long-term increase of average daily maximum temperature in western North America in the past and future.展开更多
Formaldehyde(HCHO)has been identified as one of the most common indoor pollutions nowadays.Manganese oxides(MnO_(x))are considered to be a promising catalytic material used in indoor HCHO oxidation removal due to thei...Formaldehyde(HCHO)has been identified as one of the most common indoor pollutions nowadays.Manganese oxides(MnO_(x))are considered to be a promising catalytic material used in indoor HCHO oxidation removal due to their high catalytic activity,low-cost,and environmentally friendly.In this paper,the progress in developing MnO_(x)-based catalysts for HCHO removal is comprehensively reviewed for exploring the mechanisms of catalytic oxidation and catalytic deactivation.The catalytic oxidation mechanisms based on three typical theory models(Mars-van-Krevelen,Eley-Rideal and Langmuir-Hinshelwood)are discussed and summarized.Furthermore,the research status of catalytic deactivation,catalysts’regeneration and integrated application of MnO_(x)-based catalysts for indoor HCHO removal are detailed in the review.Finally,the technical challenges in developing MnO_(x)-based catalysts for indoor HCHO removal are analyzed and the possible research direction is also proposed for overcoming the challenges toward practical application of such catalysts.展开更多
Utilizing the Community Atmosphere Model,version 4,the influence of Arctic sea-ice concentration(SIC)on the extended-range prediction of three simulated cold events(CEs)in East Asia is investigated.Numerical results s...Utilizing the Community Atmosphere Model,version 4,the influence of Arctic sea-ice concentration(SIC)on the extended-range prediction of three simulated cold events(CEs)in East Asia is investigated.Numerical results show that the Arctic SIC is crucial for the extended-range prediction of CEs in East Asia.The conditional nonlinear optimal perturbation approach is adopted to identify the optimal Arctic SIC perturbations with the largest influence on CE prediction on the extended-range time scale.It shows that the optimal SIC perturbations are more inclined to weaken the CEs and cause large prediction errors in the fourth pentad,as compared with random SIC perturbations under the same constraint.Further diagnosis reveals that the optimal SIC perturbations first modulate the local temperature through the diabatic process,and then influence the remote temperature by horizontal advection and vertical convection terms.Consequently,the optimal SIC perturbations trigger a warming center in East Asia through the propagation of Rossby wave trains,leading to the largest prediction uncertainty of the CEs in the fourth pentad.These results may provide scientific support for targeted observation of Arctic SIC to improve the extended-range CE prediction skill.展开更多
China experienced significant flooding in the summer of 2020 and multiple extreme cold surges during the winter of 2020/21.Additionally,the 2020 typhoon season had below average activity with especially quiet activity...China experienced significant flooding in the summer of 2020 and multiple extreme cold surges during the winter of 2020/21.Additionally,the 2020 typhoon season had below average activity with especially quiet activity during the first half of the season in the western North Pacific(WNP).Sea surface temperature changes in the Pacific,Indian,and Atlantic Oceans all contributed to the heavy rainfall in China,but the Atlantic and Indian Oceans seem to have played dominant roles.Enhancement and movement of the Siberian High caused a wavier pattern in the jet stream that allowed cold polar air to reach southward,inducing cold surges in China.Large vertical wind shear and low humidity in the WNP were responsible for fewer typhoons in the first half of the typhoon season.Although it is known that global warming can increase the frequency of extreme weather and climate events,its influences on individual events still need to be quantified.Additionally,the extreme cold surge during 16–18 February 2021 in the United States shares similar mechanisms with the winter 2020/21 extreme cold surges in China.展开更多
The rainfall over the Yangtze River Valley(YRV)in June 2020 broke the record since 1979.Here we show that all three oceans of the Pacific,Indian and Atlantic Oceans contribute to the YRV rainfall in June 2020,but the ...The rainfall over the Yangtze River Valley(YRV)in June 2020 broke the record since 1979.Here we show that all three oceans of the Pacific,Indian and Atlantic Oceans contribute to the YRV rainfall in June 2020,but the Atlantic plays a dominant role.The sea surface temperature(SST)anomalies in three oceans are associated with the two vorticity anomalies:negative 200-hPa relative vorticity anomalies over North China(NC)and negative 850-hPa relative vorticity anomalies in the South China Sea(SCS).The rainfall anomalies in the YRV are mainly controlled by atmospheric process associated with the NC vorticity.The positive SST anomalies in May over the western North Atlantic induce positive geopotential height anomalies in June over the mid-latitude North Atlantic,which affect the rainfall anomalies in the YRV by changing the NC vorticity via Atlantic-induced atmospheric wave train across Europe.The Indian Ocean and tropical North Atlantic,as capacitors of Pacific El Niño events in the preceding winter,affect the SCS vorticity associated with the anomalous anticyclone over the SCS and also facilitate the YRV rainfall by providing favorable moisture conditions.This study suggests that the May SST over the western North Atlantic is a good predictor of June rainfall anomalies in the YRV and highlights the important impacts of three-ocean SSTs on extreme weather and climate events in China.展开更多
基金supported by the Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) (GML2019ZD0306)National Natural Science Foundation of China (Grant Nos. 41731173 and 42192564)+5 种基金National Key R&D Program of China (2019YFA0606701)Strategic Priority Research Program of Chinese Academy of Sciences (XDB42000000 and XDA20060502)Innovation Academy of South China Sea Ecology and Environmental Engineering, Chinese Academy of Sciences (ISEE2021ZD01)Independent Research Project Program of State Key Laboratory of Tropical Oceanography (Grand No. LTOZZ2004)Leading Talents of Guangdong Province Programsupported by the High Performance Computing Division in the South China Sea Institute of Oceanology
文摘An extraordinary and unprecedented heatwave swept across western North America(i.e.,the Pacific Northwest)in late June of 2021,resulting in hundreds of deaths,a massive die-off of sea creatures off the coast,and horrific wildfires.Here,we use observational data to find the atmospheric circulation variabilities of the North Pacific and Arctic-Pacific-Canada patterns that co-occurred with the development and mature phases of the heatwave,as well as the North America pattern,which coincided with the decaying and eastward movement of the heatwave.Climate models from the Coupled Model Intercomparison Project(Phase 6)are not designed to simulate a particular heatwave event like this one.Still,models show that greenhouse gases are the main reason for the long-term increase of average daily maximum temperature in western North America in the past and future.
基金the National Natural Science Foundation of China (NSFC,52070006)BeijingNova Program of Science and Technology (Z191100001119116).
文摘Formaldehyde(HCHO)has been identified as one of the most common indoor pollutions nowadays.Manganese oxides(MnO_(x))are considered to be a promising catalytic material used in indoor HCHO oxidation removal due to their high catalytic activity,low-cost,and environmentally friendly.In this paper,the progress in developing MnO_(x)-based catalysts for HCHO removal is comprehensively reviewed for exploring the mechanisms of catalytic oxidation and catalytic deactivation.The catalytic oxidation mechanisms based on three typical theory models(Mars-van-Krevelen,Eley-Rideal and Langmuir-Hinshelwood)are discussed and summarized.Furthermore,the research status of catalytic deactivation,catalysts’regeneration and integrated application of MnO_(x)-based catalysts for indoor HCHO removal are detailed in the review.Finally,the technical challenges in developing MnO_(x)-based catalysts for indoor HCHO removal are analyzed and the possible research direction is also proposed for overcoming the challenges toward practical application of such catalysts.
基金the National Natural Science Foundation of China(Grant Nos.42288101,41790475,42175051,and 42005046)the State Key Laboratory of Tropical Oceanography(South China Sea Institute of Oceanology,Chinese Academy of Sciences+1 种基金Grant No.LTO2109)the Guangdong Basic and Applied Basic Research Foundation(Grant No.2021A1515011868).
文摘Utilizing the Community Atmosphere Model,version 4,the influence of Arctic sea-ice concentration(SIC)on the extended-range prediction of three simulated cold events(CEs)in East Asia is investigated.Numerical results show that the Arctic SIC is crucial for the extended-range prediction of CEs in East Asia.The conditional nonlinear optimal perturbation approach is adopted to identify the optimal Arctic SIC perturbations with the largest influence on CE prediction on the extended-range time scale.It shows that the optimal SIC perturbations are more inclined to weaken the CEs and cause large prediction errors in the fourth pentad,as compared with random SIC perturbations under the same constraint.Further diagnosis reveals that the optimal SIC perturbations first modulate the local temperature through the diabatic process,and then influence the remote temperature by horizontal advection and vertical convection terms.Consequently,the optimal SIC perturbations trigger a warming center in East Asia through the propagation of Rossby wave trains,leading to the largest prediction uncertainty of the CEs in the fourth pentad.These results may provide scientific support for targeted observation of Arctic SIC to improve the extended-range CE prediction skill.
基金the National Natural Science Foundation of China(Grant No.41731173)the National Key R&D Program of China(Grant No.2019YFA0606701)+2 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant Nos.XDB42000000 and XDA20060502)the Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou)(Grant No.GML2019ZD0306)the Innovation Academy of South China Sea Ecology and Environmental Engineering,the Chinese Academy of Sciences(Grant No.ISEE2018PY06)。
文摘China experienced significant flooding in the summer of 2020 and multiple extreme cold surges during the winter of 2020/21.Additionally,the 2020 typhoon season had below average activity with especially quiet activity during the first half of the season in the western North Pacific(WNP).Sea surface temperature changes in the Pacific,Indian,and Atlantic Oceans all contributed to the heavy rainfall in China,but the Atlantic and Indian Oceans seem to have played dominant roles.Enhancement and movement of the Siberian High caused a wavier pattern in the jet stream that allowed cold polar air to reach southward,inducing cold surges in China.Large vertical wind shear and low humidity in the WNP were responsible for fewer typhoons in the first half of the typhoon season.Although it is known that global warming can increase the frequency of extreme weather and climate events,its influences on individual events still need to be quantified.Additionally,the extreme cold surge during 16–18 February 2021 in the United States shares similar mechanisms with the winter 2020/21 extreme cold surges in China.
基金supported by the National Key R&D Program of China(Grand No.2019YFA0606701)the National Natural Science Foundation of China(Grand No.41731173)+4 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(Grand Nos.XDB42000000&XDA20060502)the Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou)(Grand No.GML2019ZD0306)the Innovation Academy of South China Sea Ecology and Environmental Engineering,the Chinese Academy of Sciences(Grand No.ISEE2018PY06)the Leading Talents of Guangdong Province Program,the National Program on Global Change and Air-Sea Interaction under grant GASI-IPOVAI-03the Independent Research Project Program of State Key Laboratory of Tropical Oceanography(Grand No.LTOZZ2004).
文摘The rainfall over the Yangtze River Valley(YRV)in June 2020 broke the record since 1979.Here we show that all three oceans of the Pacific,Indian and Atlantic Oceans contribute to the YRV rainfall in June 2020,but the Atlantic plays a dominant role.The sea surface temperature(SST)anomalies in three oceans are associated with the two vorticity anomalies:negative 200-hPa relative vorticity anomalies over North China(NC)and negative 850-hPa relative vorticity anomalies in the South China Sea(SCS).The rainfall anomalies in the YRV are mainly controlled by atmospheric process associated with the NC vorticity.The positive SST anomalies in May over the western North Atlantic induce positive geopotential height anomalies in June over the mid-latitude North Atlantic,which affect the rainfall anomalies in the YRV by changing the NC vorticity via Atlantic-induced atmospheric wave train across Europe.The Indian Ocean and tropical North Atlantic,as capacitors of Pacific El Niño events in the preceding winter,affect the SCS vorticity associated with the anomalous anticyclone over the SCS and also facilitate the YRV rainfall by providing favorable moisture conditions.This study suggests that the May SST over the western North Atlantic is a good predictor of June rainfall anomalies in the YRV and highlights the important impacts of three-ocean SSTs on extreme weather and climate events in China.