Rapid development of deepfake technology led to the spread of forged audios and videos across network platforms,presenting risks for numerous countries,societies,and individuals,and posing a serious threat to cyberspa...Rapid development of deepfake technology led to the spread of forged audios and videos across network platforms,presenting risks for numerous countries,societies,and individuals,and posing a serious threat to cyberspace security.To address the problem of insufficient extraction of spatial features and the fact that temporal features are not considered in the deepfake video detection,we propose a detection method based on improved CapsNet and temporal–spatial features(iCapsNet–TSF).First,the dynamic routing algorithm of CapsNet is improved using weight initialization and updating.Then,the optical flow algorithm is used to extract interframe temporal features of the videos to form a dataset of temporal–spatial features.Finally,the iCapsNet model is employed to fully learn the temporal–spatial features of facial videos,and the results are fused.Experimental results show that the detection accuracy of iCapsNet–TSF reaches 94.07%,98.83%,and 98.50%on the Celeb-DF,FaceSwap,and Deepfakes datasets,respectively,displaying a better performance than most existing mainstream algorithms.The iCapsNet–TSF method combines the capsule network and the optical flow algorithm,providing a novel strategy for the deepfake detection,which is of great significance to the prevention of deepfake attacks and the preservation of cyberspace security.展开更多
Independent manipulation of transmitted and reflected light fields is a key technology for the realization of multifunctional optical applications,which can be implemented based on multilayered plasmonic or supercell ...Independent manipulation of transmitted and reflected light fields is a key technology for the realization of multifunctional optical applications,which can be implemented based on multilayered plasmonic or supercell subwavelength structures.However,the former is not suitable for the optical bands,while the latter is insufficient in generating large phase gradients.Here,an adjoint-optimization-based inverse design methodology is proposed,which utilizes the polarization-selective local interference between individual meta-atoms and enables monolayer dielectric metasurfaces to decouple the wavefront of transmitted and reflected optical fields.Moreover,this methodology serves to mitigate the aperiodic electromagnetic crosstalk inherent between adjacent meta-atoms,consequently leading to a significant enhancement in the performance of meta-devices.We analyzed the physical mechanism of adjoint optimization and proposed the concept of phase factors,highlighting their importance in the rapid inverse design of meta-devices—an aspect often overlooked in previous research.To demonstrate the feasibility and robustness of our method,we optimize monolayer metasurfaces with different initial structures.These devices efficiently focus and deflect x-linearly and y-linearly polarized incident light in transmission and reflection spaces,respectively.Overall,this methodology holds immense potential for designing multifunctional,high-performing metasurfaces that meet multiple constraints,opening up broad prospects for applications.展开更多
In order to study the mechanism of selective catalytic reduction of activated coke to remove NO in low-temperature flue gas and provide some theoretical basis for the development of related technologies.The pore sized...In order to study the mechanism of selective catalytic reduction of activated coke to remove NO in low-temperature flue gas and provide some theoretical basis for the development of related technologies.The pore sizedistribution and BET specific surface area of AC were obtain by data analyzing of N2 adsorption/desorption isotherm at -196 ℃ and carbon matrix and surface chemistry of virgin activated coke samples were characterized by acid-base titration and XPS.The process of selective catalytic reduction of activated coke (AC) samples with NH3 as reducing agent was studied in a fixed bed reactor at 150 ℃.The result shows that pore size distribution or BET specific surface of activated cokes have not correlation with denitrification activity for SCR.The NO reduction activities of the activated cokes are apparent to increase with their surface oxygen element content and total amount of acidic sites.Obviously there is good linear relationship between the NH3 adsorption capacity and activity for SCR with linear correlation coefficient 0.943.It has been presented that adsorption of NH3 on acidic functional groups in the edge of large polycyclic aromatic ring of activated coke is key rate controlling step in the SCR heterogeneous catalytic reaction.展开更多
Orbital angular momentum(OAM)is a fundamental physical characteristic to describe laser fields with a spiral phase structure.Vortex beams carrying OAMs have attracted more and more attention in recent years.However,th...Orbital angular momentum(OAM)is a fundamental physical characteristic to describe laser fields with a spiral phase structure.Vortex beams carrying OAMs have attracted more and more attention in recent years.However,the wavefront of OAM light would be destroyed when it passes through scattering media.Here,based on the feedback-based wavefront shaping method,we reconstitute OAM wavefronts behind strongly scattering media.The intensity of light with desired OAM states is enhanced to 150 times.This study provides a method to manipulate OAMs of scattered light and is of great significance for OAM optical communication and imaging to overcome complex environment interference.展开更多
In the process of enriching CH4 from coal-bed methane,the separation of CH_(4)/N_(2)is very difficult to accomplish by an adsorption process due to the similar physico-chemical properties of the two molecules.A series...In the process of enriching CH4 from coal-bed methane,the separation of CH_(4)/N_(2)is very difficult to accomplish by an adsorption process due to the similar physico-chemical properties of the two molecules.A series of coconut-shell-based granular activated carbons(GACs)with different pore structures were prepared,which were characterized by different methods.The influence of the pore structure on the separation properties was investigated in detail.The results show that one of the carbons prepared(GAC-3)has high CH4 equilibrium adsorption capacity(3.28 mol·kg–1)at 298 K and equilibrium separation coefficient(3.95).The CH_(4)/N_(2)separation on the GACs is controlled by adsorption equilibrium as compared with the dynamic effect.Taking the specific surface area,for example,the common characterization index of the pore structure is not enough to judge the separation performance of the GACs.However,the microstructure of carbon materials plays a decisive role for CH_(4)/N_(2)separation.According to the pore-structure analysis,the effective pore size for the CH_(4)/N_(2)separation is from 0.4 to 0.9 nm,with the optimum effect occurring in the range of 0.6–0.7 nm,followed by the range of 0.7~0.9 nm.Also,a four-bed vacuum pressure swing adsorption process was adopted to evaluate the performance of GACs for the separation of CH4 from nitrogen.展开更多
基金supported by the Fundamental Research Funds for the Central Universities under Grant 2020JKF101the Research Funds of Sugon under Grant 2022KY001.
文摘Rapid development of deepfake technology led to the spread of forged audios and videos across network platforms,presenting risks for numerous countries,societies,and individuals,and posing a serious threat to cyberspace security.To address the problem of insufficient extraction of spatial features and the fact that temporal features are not considered in the deepfake video detection,we propose a detection method based on improved CapsNet and temporal–spatial features(iCapsNet–TSF).First,the dynamic routing algorithm of CapsNet is improved using weight initialization and updating.Then,the optical flow algorithm is used to extract interframe temporal features of the videos to form a dataset of temporal–spatial features.Finally,the iCapsNet model is employed to fully learn the temporal–spatial features of facial videos,and the results are fused.Experimental results show that the detection accuracy of iCapsNet–TSF reaches 94.07%,98.83%,and 98.50%on the Celeb-DF,FaceSwap,and Deepfakes datasets,respectively,displaying a better performance than most existing mainstream algorithms.The iCapsNet–TSF method combines the capsule network and the optical flow algorithm,providing a novel strategy for the deepfake detection,which is of great significance to the prevention of deepfake attacks and the preservation of cyberspace security.
基金supported by the National Key Research and Development Program of China(Grant No.2023YFB2805800)the National Natural Science Foundation of China(Grant Nos.62175242,and U20A20217)the Sichuan Science and Technology Program(Grant No.2021ZYCD002)。
文摘Independent manipulation of transmitted and reflected light fields is a key technology for the realization of multifunctional optical applications,which can be implemented based on multilayered plasmonic or supercell subwavelength structures.However,the former is not suitable for the optical bands,while the latter is insufficient in generating large phase gradients.Here,an adjoint-optimization-based inverse design methodology is proposed,which utilizes the polarization-selective local interference between individual meta-atoms and enables monolayer dielectric metasurfaces to decouple the wavefront of transmitted and reflected optical fields.Moreover,this methodology serves to mitigate the aperiodic electromagnetic crosstalk inherent between adjacent meta-atoms,consequently leading to a significant enhancement in the performance of meta-devices.We analyzed the physical mechanism of adjoint optimization and proposed the concept of phase factors,highlighting their importance in the rapid inverse design of meta-devices—an aspect often overlooked in previous research.To demonstrate the feasibility and robustness of our method,we optimize monolayer metasurfaces with different initial structures.These devices efficiently focus and deflect x-linearly and y-linearly polarized incident light in transmission and reflection spaces,respectively.Overall,this methodology holds immense potential for designing multifunctional,high-performing metasurfaces that meet multiple constraints,opening up broad prospects for applications.
基金The authors are grateful to the National Key Research and Development Program of China(NO.2016YFC0204100).
文摘In order to study the mechanism of selective catalytic reduction of activated coke to remove NO in low-temperature flue gas and provide some theoretical basis for the development of related technologies.The pore sizedistribution and BET specific surface area of AC were obtain by data analyzing of N2 adsorption/desorption isotherm at -196 ℃ and carbon matrix and surface chemistry of virgin activated coke samples were characterized by acid-base titration and XPS.The process of selective catalytic reduction of activated coke (AC) samples with NH3 as reducing agent was studied in a fixed bed reactor at 150 ℃.The result shows that pore size distribution or BET specific surface of activated cokes have not correlation with denitrification activity for SCR.The NO reduction activities of the activated cokes are apparent to increase with their surface oxygen element content and total amount of acidic sites.Obviously there is good linear relationship between the NH3 adsorption capacity and activity for SCR with linear correlation coefficient 0.943.It has been presented that adsorption of NH3 on acidic functional groups in the edge of large polycyclic aromatic ring of activated coke is key rate controlling step in the SCR heterogeneous catalytic reaction.
基金supported in part by the National Natural Science Foundation of China(NSFC)(Nos.11734011,62022058,12074252,and 12004245)the National Key R&D Program of China(Nos.2017YFA0303701 and 2018YFA0306301)+2 种基金the Shanghai Municipal Science and Technology Major Project(No.2019SHZDZX01)the Shanghai Rising-Star Program(No.20QA1405400)the Shandong Quancheng Scholarship(No.00242019024)。
文摘Orbital angular momentum(OAM)is a fundamental physical characteristic to describe laser fields with a spiral phase structure.Vortex beams carrying OAMs have attracted more and more attention in recent years.However,the wavefront of OAM light would be destroyed when it passes through scattering media.Here,based on the feedback-based wavefront shaping method,we reconstitute OAM wavefronts behind strongly scattering media.The intensity of light with desired OAM states is enhanced to 150 times.This study provides a method to manipulate OAMs of scattered light and is of great significance for OAM optical communication and imaging to overcome complex environment interference.
文摘In the process of enriching CH4 from coal-bed methane,the separation of CH_(4)/N_(2)is very difficult to accomplish by an adsorption process due to the similar physico-chemical properties of the two molecules.A series of coconut-shell-based granular activated carbons(GACs)with different pore structures were prepared,which were characterized by different methods.The influence of the pore structure on the separation properties was investigated in detail.The results show that one of the carbons prepared(GAC-3)has high CH4 equilibrium adsorption capacity(3.28 mol·kg–1)at 298 K and equilibrium separation coefficient(3.95).The CH_(4)/N_(2)separation on the GACs is controlled by adsorption equilibrium as compared with the dynamic effect.Taking the specific surface area,for example,the common characterization index of the pore structure is not enough to judge the separation performance of the GACs.However,the microstructure of carbon materials plays a decisive role for CH_(4)/N_(2)separation.According to the pore-structure analysis,the effective pore size for the CH_(4)/N_(2)separation is from 0.4 to 0.9 nm,with the optimum effect occurring in the range of 0.6–0.7 nm,followed by the range of 0.7~0.9 nm.Also,a four-bed vacuum pressure swing adsorption process was adopted to evaluate the performance of GACs for the separation of CH4 from nitrogen.