The aerosol optical properties and direct radiative forcing over the Mu Us desert of northern China, acquired through a CE318 sunphotometer of the ground-based Aerosol Robotic Network (AERONET), are analyzed. The se...The aerosol optical properties and direct radiative forcing over the Mu Us desert of northern China, acquired through a CE318 sunphotometer of the ground-based Aerosol Robotic Network (AERONET), are analyzed. The seasonal variations in the aerosol optical properties are examined. The effect of meteorological elements (pressure, temperature, water vapor pressure, relative humidity and wind speed) on the aerosol optical properties is also studied. Then, the sources and optical properties under two different cases, a dust event and a pollution event, are compared. The results show that the high aerosol optical depth (AOD) found in Yulin was mostly attributed to the occurrence of dust events in spring from the Mu Us desert and deserts of West China and Mongolia, as well as the impacts of anthropogenic pollutant particles from the middle part of China in the other seasons. The seasonal variation and the probability distribution of the radiative forcing and the radiative forcing efficiency at the surface and the top of the atmosphere are analyzed and regressed using the linear and Gaussian regression methods.展开更多
Mineral compositions of aerosol particles were investigated at four sites (Aksu, Dunhuang, Zhenbeitai, and Tongliao) in desert regions of northern China from March to May in 2001 and 2002 during the intensive field ...Mineral compositions of aerosol particles were investigated at four sites (Aksu, Dunhuang, Zhenbeitai, and Tongliao) in desert regions of northern China from March to May in 2001 and 2002 during the intensive field campaign period of ACE-Asia (Aerosol Characterization Experiments-Asia). The X-ray diffraction (XRD) results show the main minerals for Asian dust are illite, chlorite, kaolinite, quartz, feldspar, calcite, and dolomite. Gypsum, hornblende, and halite are also detected in several samples. Semi-quantitative mineralogical data of aerosol samples show that carbonate content decreases from western to eastern source areas; that is, soil dust collected at western source area sites of Dunhuang and Aksu are enriched with carbonate, while northeastern source area site of Tongliao is associated with low carbonate content. But the spatial distribution of feldspar exhibits a different pattern as compared to carbonate, increasing from the western to the eastern sources. The total clay content is significantly higher (73% in average) at the deposition site of Changwu than those at source areas. Air-mass back trajectory studies for the three dust storm events observed at Changwu, showed that soil dust transport pathways were as expected from carbonate content for the source identification, further demonstrating that carbonate was a useful tracer for eolian dust on regional scale in northern China.展开更多
基金supported by grants from the National Key Project of Basic Research (2006CB403702 and 2006CB403701)the CAMS Basis Research Project and National Natural Science Foundation of China under Grant No. 40405001
文摘The aerosol optical properties and direct radiative forcing over the Mu Us desert of northern China, acquired through a CE318 sunphotometer of the ground-based Aerosol Robotic Network (AERONET), are analyzed. The seasonal variations in the aerosol optical properties are examined. The effect of meteorological elements (pressure, temperature, water vapor pressure, relative humidity and wind speed) on the aerosol optical properties is also studied. Then, the sources and optical properties under two different cases, a dust event and a pollution event, are compared. The results show that the high aerosol optical depth (AOD) found in Yulin was mostly attributed to the occurrence of dust events in spring from the Mu Us desert and deserts of West China and Mongolia, as well as the impacts of anthropogenic pollutant particles from the middle part of China in the other seasons. The seasonal variation and the probability distribution of the radiative forcing and the radiative forcing efficiency at the surface and the top of the atmosphere are analyzed and regressed using the linear and Gaussian regression methods.
基金supported by the National Natural Science Foundation of China (Grants 40405023,40675081,and 40599422)a grant from SKLLQG,CASthe staff of Shaanxi Institute of Desert Research,and Aksu Water Balance Observatory of the Chinese Academy of Sciences for their support during sampling
文摘Mineral compositions of aerosol particles were investigated at four sites (Aksu, Dunhuang, Zhenbeitai, and Tongliao) in desert regions of northern China from March to May in 2001 and 2002 during the intensive field campaign period of ACE-Asia (Aerosol Characterization Experiments-Asia). The X-ray diffraction (XRD) results show the main minerals for Asian dust are illite, chlorite, kaolinite, quartz, feldspar, calcite, and dolomite. Gypsum, hornblende, and halite are also detected in several samples. Semi-quantitative mineralogical data of aerosol samples show that carbonate content decreases from western to eastern source areas; that is, soil dust collected at western source area sites of Dunhuang and Aksu are enriched with carbonate, while northeastern source area site of Tongliao is associated with low carbonate content. But the spatial distribution of feldspar exhibits a different pattern as compared to carbonate, increasing from the western to the eastern sources. The total clay content is significantly higher (73% in average) at the deposition site of Changwu than those at source areas. Air-mass back trajectory studies for the three dust storm events observed at Changwu, showed that soil dust transport pathways were as expected from carbonate content for the source identification, further demonstrating that carbonate was a useful tracer for eolian dust on regional scale in northern China.