Nearly all real-world networks are complex networks and usually are in danger of collapse.Therefore,it is crucial to exploit and understand the mechanisms of network attacks and provide better protection for network f...Nearly all real-world networks are complex networks and usually are in danger of collapse.Therefore,it is crucial to exploit and understand the mechanisms of network attacks and provide better protection for network functionalities.Network dismantling aims to find the smallest set of nodes such that after their removal the network is broken into connected components of sub-extensive size.To overcome the limitations and drawbacks of existing network dismantling methods,this paper focuses on network dismantling problem and proposes a neighbor-loop structure based centrality metric,NL,which achieves a balance between computational efficiency and evaluation accuracy.In addition,we design a novel method combining NL-based nodes-removing,greedy tree-breaking and reinsertion.Moreover,we compare five baseline methods with our algorithm on ten widely used real-world networks and three types of model networks including Erd€os-Renyi random networks,Watts-Strogatz smallworld networks and Barabasi-Albert scale-free networks with different network generation parameters.Experimental results demonstrate that our proposed method outperforms most peer methods by obtaining a minimal set of targeted attack nodes.Furthermore,the insights gained from this study may be of assistance to future practical research into real-world networks.展开更多
Single-atomic site catalysts have drawn considerable attention because of their maximum atom-utilization efficiency and excellent catalytic activity.In this work,a highly active single-atomic Pt site photocatalyst was...Single-atomic site catalysts have drawn considerable attention because of their maximum atom-utilization efficiency and excellent catalytic activity.In this work,a highly active single-atomic Pt site photocatalyst was synthesized through employing defective Ti0_(2) nanosheets as solid support for photo-catalytic water splitting.It indicated that the surface oxygen vacancies on defective Ti0_(2) nanosheets could effectively stabilize the single-atomic Pt sites through constructing a three-center Ti-Pt-Ti structure.The Ti-Pt-Ti structure can hold the stability of isolated single-atomic Pt sites and facilitate the separation and transfer of photoinduced charge carriers,thereby greatly improving the photocatalytic H2 evolution.Notably,our synthesized photocatalyst exhibited a remarkably enhanced H2 evolution performance,and the H2 production rate is up to 13460.7μmol h^(-1)·g^(-1),which is up to around 29.0 and 4.7 times higher than those of Ti0_(2) nanosheets and Pt nanoparticles-Ti0_(2).In addition,a plausible enhanced reaction mechanism was also proposed combining with photo-electrochemical characterizations and density functional theoiy(DFT)calculation results.Ultimately,it is believed that this work highlights the benefits of a single-site catalyst and paves the way to rationally design the highly active and stable single-atomic site photocatalysts on metal oxide support.展开更多
This paper used 3 types of graphite with different physical structures as the porous matrix to prepare composite phase change materials(PCMs),and investigated their photo-thermal conversion performance and application...This paper used 3 types of graphite with different physical structures as the porous matrix to prepare composite phase change materials(PCMs),and investigated their photo-thermal conversion performance and application in battery thermal management.Multiple structure graphite minerals,including microcrystalline graphite(MG),scale graphite(SG),and expanded graphite(EG)were used as porous matrix,while stearic acid(SA)acts as the phase change material.The vacuum impregnation method was applied to prepare SA/MG,SA/SG,SA/EG,and SA/MG1,and SA/EG1was/were prepared by the ethyl alcohol method.Results show that the thermal conductivities of all composite phase change materials were 10.82 to 22.06 times higher than that of the pure SA.Thermogravimetric(TG)analysis showed that the loadages of SA were 43.61%,18.74%,and 92.66%for SA/MG,SA/SG,and SA/EG respectively.The load rates of SA were 18.98%and 18.88%for SA/MG1 and SA/EG1,respectively.For the 3 types of graphite materials of different dimensions,the BET(Brunauer,Emmett,and Teller)surface area determines the maximum load of SA.The Fourier-transform infrared(FTIR)and X-ray diffraction(XRD)results indicated that there was good compatibility between the SA and the supports.The SA/EG1 has better thermophysical properties in heat energy storage and release process.The thermal infrared images show that SA/EG1 has higher sensitivity to the temperature changes.SA/EG1 has better photo-heat conversion performance than SA/SG and SA/MG1 attributed to the multilayer structure of EG.SA/EG has better thermal management performance in the Li-ion batteries discharge process.展开更多
To improve the separation efficiency of air dense medium fluidized beds tor dry coal preparation, a gasvibro fluidized bed has been proposed in which magnetic powder is used as the heavy medium. Pressure fluctuations ...To improve the separation efficiency of air dense medium fluidized beds tor dry coal preparation, a gasvibro fluidized bed has been proposed in which magnetic powder is used as the heavy medium. Pressure fluctuations in the gas-vibro fluidized bed were investigated using time- and frequency-domain analysis methods. The relationship between pressure fluctuations, bubble behavior, and separation efficiency was established. The low amplitude of the standard deviation, the power spectral density (PSD), the incoherent-output PSD, and the high amplitude of the coherent-output PSD, which corresponds to the bubble behavior in the bed, were improved for coal preparation. The coal ash content was reduced from 42.5570 to 16.54% by using the gas-vibro fluidized bed.展开更多
基金the National Natural Science Foundation of China under Grants 61871209 and 61901210,in part by Artificial Intelligence and Intelligent Transportation Joint Technical Center of HUST and Hubei Chutian Intelligent Transportation Co.,LTD under project”Intelligent Transportation Operation Monitoring Network and System”.
文摘Nearly all real-world networks are complex networks and usually are in danger of collapse.Therefore,it is crucial to exploit and understand the mechanisms of network attacks and provide better protection for network functionalities.Network dismantling aims to find the smallest set of nodes such that after their removal the network is broken into connected components of sub-extensive size.To overcome the limitations and drawbacks of existing network dismantling methods,this paper focuses on network dismantling problem and proposes a neighbor-loop structure based centrality metric,NL,which achieves a balance between computational efficiency and evaluation accuracy.In addition,we design a novel method combining NL-based nodes-removing,greedy tree-breaking and reinsertion.Moreover,we compare five baseline methods with our algorithm on ten widely used real-world networks and three types of model networks including Erd€os-Renyi random networks,Watts-Strogatz smallworld networks and Barabasi-Albert scale-free networks with different network generation parameters.Experimental results demonstrate that our proposed method outperforms most peer methods by obtaining a minimal set of targeted attack nodes.Furthermore,the insights gained from this study may be of assistance to future practical research into real-world networks.
基金This research was funded by the Canadian Centre for Clean Coal/Carbon and Mineral Processing Technologies(C5MPT),the National Key R&D Program of China(2017YFB0310803)and the China Scholarship Council(CSC).We thank the NanoFAB at the University of Alberta for the convenience of instruments use,and the kindly help of Nanqi Duan and Chao Qi on sample characterization.
文摘Single-atomic site catalysts have drawn considerable attention because of their maximum atom-utilization efficiency and excellent catalytic activity.In this work,a highly active single-atomic Pt site photocatalyst was synthesized through employing defective Ti0_(2) nanosheets as solid support for photo-catalytic water splitting.It indicated that the surface oxygen vacancies on defective Ti0_(2) nanosheets could effectively stabilize the single-atomic Pt sites through constructing a three-center Ti-Pt-Ti structure.The Ti-Pt-Ti structure can hold the stability of isolated single-atomic Pt sites and facilitate the separation and transfer of photoinduced charge carriers,thereby greatly improving the photocatalytic H2 evolution.Notably,our synthesized photocatalyst exhibited a remarkably enhanced H2 evolution performance,and the H2 production rate is up to 13460.7μmol h^(-1)·g^(-1),which is up to around 29.0 and 4.7 times higher than those of Ti0_(2) nanosheets and Pt nanoparticles-Ti0_(2).In addition,a plausible enhanced reaction mechanism was also proposed combining with photo-electrochemical characterizations and density functional theoiy(DFT)calculation results.Ultimately,it is believed that this work highlights the benefits of a single-site catalyst and paves the way to rationally design the highly active and stable single-atomic site photocatalysts on metal oxide support.
基金supported by the National Natural Science Foundation of China(Nos.52274252 and 51874047)the Special Fund for the Construction of Innovative Provinces in Hunan Province(Nos.2020RC3038 and 2022WK4004)+1 种基金the Changsha City Fund for Distinguished and Innovative Young Scholars(No.kq1802007)the Key Science and Technology Project of Changsha City(No.kq2102005).
文摘This paper used 3 types of graphite with different physical structures as the porous matrix to prepare composite phase change materials(PCMs),and investigated their photo-thermal conversion performance and application in battery thermal management.Multiple structure graphite minerals,including microcrystalline graphite(MG),scale graphite(SG),and expanded graphite(EG)were used as porous matrix,while stearic acid(SA)acts as the phase change material.The vacuum impregnation method was applied to prepare SA/MG,SA/SG,SA/EG,and SA/MG1,and SA/EG1was/were prepared by the ethyl alcohol method.Results show that the thermal conductivities of all composite phase change materials were 10.82 to 22.06 times higher than that of the pure SA.Thermogravimetric(TG)analysis showed that the loadages of SA were 43.61%,18.74%,and 92.66%for SA/MG,SA/SG,and SA/EG respectively.The load rates of SA were 18.98%and 18.88%for SA/MG1 and SA/EG1,respectively.For the 3 types of graphite materials of different dimensions,the BET(Brunauer,Emmett,and Teller)surface area determines the maximum load of SA.The Fourier-transform infrared(FTIR)and X-ray diffraction(XRD)results indicated that there was good compatibility between the SA and the supports.The SA/EG1 has better thermophysical properties in heat energy storage and release process.The thermal infrared images show that SA/EG1 has higher sensitivity to the temperature changes.SA/EG1 has better photo-heat conversion performance than SA/SG and SA/MG1 attributed to the multilayer structure of EG.SA/EG has better thermal management performance in the Li-ion batteries discharge process.
基金supported financially by the National Key Basic Research Program of China(973 Program,No.2012CB214904)the National Natural Science Foundation of China(Nos.51221462,51134022,51304196,and 91434133)+1 种基金the Specialized Research Fund for the Doctoral Program of Higher Education(No.20120095130001)a Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions
文摘To improve the separation efficiency of air dense medium fluidized beds tor dry coal preparation, a gasvibro fluidized bed has been proposed in which magnetic powder is used as the heavy medium. Pressure fluctuations in the gas-vibro fluidized bed were investigated using time- and frequency-domain analysis methods. The relationship between pressure fluctuations, bubble behavior, and separation efficiency was established. The low amplitude of the standard deviation, the power spectral density (PSD), the incoherent-output PSD, and the high amplitude of the coherent-output PSD, which corresponds to the bubble behavior in the bed, were improved for coal preparation. The coal ash content was reduced from 42.5570 to 16.54% by using the gas-vibro fluidized bed.