IPCC AR6 states that the neglect of recent rapid warming in the Arctic generally leads to an underestimate of global warming trends.In this study,by reconstructing the surface temperature(ST)datasets in the Arctic und...IPCC AR6 states that the neglect of recent rapid warming in the Arctic generally leads to an underestimate of global warming trends.In this study,by reconstructing the surface temperature(ST)datasets in the Arctic under different sea ice extent scenarios(Imax and Imin),we respectively evaluated the annual and seasonal warming trends and their uncertainties from 1900 to 2020.The results show that the reconstructed datasets have a good representation of the ST change trends in the Arctic.In 1900e2020,the annual warming trends in the Arctic(0.17±0.031 and 0.14±0.025℃ per decade under the Imax and Imin reconstruction,respectively)are roughly 1.6e1.8 times the global mean warming trends(0.10±0.008 and 0.09±0.008℃ per decade).While in 1979e2020,the Arctic warming trends(0.66±0.100 and 0.55±0.080℃ per decade)increase to 3.1e3.5 times of the global warming trend(0.19±0.023 and 0.18±0.023℃ per decade)for Imax and Imin,respectively,indicating that the Arctic amplification effect has been significantly enhancing in recent decades.Although the seasonal warming trends are closely related to cloud feedback mechanisms,atmospheric circulation,and ocean circulation,they are not sensitive to the different reconstruction scenarios.展开更多
Separators play a critical role in lithium-ion batteries.However,the restrictions of thermal stability and inferior electrical performance in commercial polyolefin separators significantly limit their applications und...Separators play a critical role in lithium-ion batteries.However,the restrictions of thermal stability and inferior electrical performance in commercial polyolefin separators significantly limit their applications under harsh conditions.Here,we report a cellulose-assisted self-assembly strategy to construct a cellulose-based separator massively and continuously.With an ultrahigh ionic conductivity in electrolytes of 3.7 mS·cm^(-1) and the ability to regulate ion transport,the obtained separator is a promising alternative for high-performance lithium-ion batteries.In addition,integrated with high thermal stability,the cellulose-based separator endows batteries with high safety at high temperatures,greatly expanding the application scenarios of energy storage devices in extreme environments.展开更多
基金This study was supported by the National Key R&D Programs of China(2017YFC1502301,2018YFC1507705)the Natural Science Foundation of China(41975105).
文摘IPCC AR6 states that the neglect of recent rapid warming in the Arctic generally leads to an underestimate of global warming trends.In this study,by reconstructing the surface temperature(ST)datasets in the Arctic under different sea ice extent scenarios(Imax and Imin),we respectively evaluated the annual and seasonal warming trends and their uncertainties from 1900 to 2020.The results show that the reconstructed datasets have a good representation of the ST change trends in the Arctic.In 1900e2020,the annual warming trends in the Arctic(0.17±0.031 and 0.14±0.025℃ per decade under the Imax and Imin reconstruction,respectively)are roughly 1.6e1.8 times the global mean warming trends(0.10±0.008 and 0.09±0.008℃ per decade).While in 1979e2020,the Arctic warming trends(0.66±0.100 and 0.55±0.080℃ per decade)increase to 3.1e3.5 times of the global warming trend(0.19±0.023 and 0.18±0.023℃ per decade)for Imax and Imin,respectively,indicating that the Arctic amplification effect has been significantly enhancing in recent decades.Although the seasonal warming trends are closely related to cloud feedback mechanisms,atmospheric circulation,and ocean circulation,they are not sensitive to the different reconstruction scenarios.
基金supported by the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB0450402)the National Key Research and Development Program of China(Nos.2018YFE0202201 and 2021YFA0715700)+3 种基金the National Natural Science Foundation of China(Nos.22293044,U1932213,51732011,22105194,and 92163130)the Major Basic Research Project of Anhui Province(No.2023z04020009)the New Cornerstone Investigator Programcarried out at the USTC Center for Micro and Nanoscale Research and Fabrication。
文摘Separators play a critical role in lithium-ion batteries.However,the restrictions of thermal stability and inferior electrical performance in commercial polyolefin separators significantly limit their applications under harsh conditions.Here,we report a cellulose-assisted self-assembly strategy to construct a cellulose-based separator massively and continuously.With an ultrahigh ionic conductivity in electrolytes of 3.7 mS·cm^(-1) and the ability to regulate ion transport,the obtained separator is a promising alternative for high-performance lithium-ion batteries.In addition,integrated with high thermal stability,the cellulose-based separator endows batteries with high safety at high temperatures,greatly expanding the application scenarios of energy storage devices in extreme environments.
