[Objectives]To determine the potential habitat range of Caragana acanthophylla in Xinjiang.[Methods]The known distribution points of C.acanthophylla were used as samples,and a MaxEnt model was developed based on their...[Objectives]To determine the potential habitat range of Caragana acanthophylla in Xinjiang.[Methods]The known distribution points of C.acanthophylla were used as samples,and a MaxEnt model was developed based on their climatic variables to identify key environmental factors affecting the potential habitats of C.acanthophylla through jackknife method and construction of a response relationship between representative variables and habitat suitability;the suitability of habitats for C.acanthophylla in Xinjiang was evaluated based on the output results of the model.[Results](i)The accuracy of the model verified by AUC curve was 0.971,indicating that the potential habitats of C.acanthophylla in Xinjiang predicted by MaxEnt model were highly credible.(ii)The optimum climatic characteristics for the distribution of C.acanthophylla in Xinjiang were:isothermality 18.8%-34%,minimum temperature of coldest month-30℃to-13℃,mean temperature of coldest quarter-18℃ to-4℃,annual precipitation 80-410 mm,precipitation of driest month 0-25 mm,precipitation of driest quarter 0-82 mm,and precipitation of coldest quarter 0-75 mm.(iii)The total potential distribution area of C.acanthophylla in Xinjiang was modeled to be 1.03×10^(5) km^(2),of which 8.54×10^(3)km^(2) was high suitability area,mainly in the front mountain belt of the north slope of Tianshan Mountain in Urumqi City,Changji Hui Autonomous Prefecture,Bortala Mongol Autonomous Prefecture,and Yili Kazak Autonomous Prefecture and the front mountain belt of Barluk Mountain in Tacheng Prefecture.[Conclusions]This study is of great significance for the future scientific management,regeneration,vegetation restoration and ecological protection of C.acanthophylla.展开更多
The combined impact of the Pacific Decadal Oscillation (PDO) and Atlantic Multidecadal Oscillation (AMO) on the summer rainfall in eastern China was investigated using CCSM4. The strongest signals occur with the c...The combined impact of the Pacific Decadal Oscillation (PDO) and Atlantic Multidecadal Oscillation (AMO) on the summer rainfall in eastern China was investigated using CCSM4. The strongest signals occur with the combination of a positive PDO and a negative AMO (+PDO- AMO), as well as a negative PDO and a positive AMO (-PDO + AMO). For the +PDO- AMO set, significant positive rainfall anomalies occur over the lower reaches of the Yangtze River valley (YR), when the East Asian summer monsoon becomes weaker, while the East Asian westerly jet stream becomes stronger, and ascending motion over the YR becomes enhanced due to the jet-related secondary circulation. Contrary anomalies occur over East Asia for the -PDO + AMO set. The influence of these two combinations of PDO and AMO on the summer rainfall in eastern China can also be observed in the two interdecadal rainfall changes in eastern China in the late 1970s and late 1990s.展开更多
Classical monsoon dynamics considers the winter/spring snow amount on the Tibetan Plateau(TP)as a major factor driving the East Asian summer monsoon(EASM)for its direct influence on the land-sea thermal contrast.Actua...Classical monsoon dynamics considers the winter/spring snow amount on the Tibetan Plateau(TP)as a major factor driving the East Asian summer monsoon(EASM)for its direct influence on the land-sea thermal contrast.Actually,the TP snow increased and decreased after the late 1970s and 1990s,respectively,accompanying the two major interdecadal changes in the EASM.Although studies have explored the possible mechanisms of the EASM interdecadal variations,and change in TP snow is considered as one of the major drivers,few studies have illustrated the underlying mechanisms of the interdecadal changes in the winter TP snow.This study reveals a tripole pattern of change,with decreased winter precipitation over the TP and an increase to its north and south after the late 1990s.Further analyses through numerical experiments demonstrate that the tropical Pacific SST changes in the late 1990s can robustly affect the winter TP precipitation through regulating the Walker and regional Hadley circulation.The cooling over the tropical central-eastern Pacific can enhance the Walker circulation cell over the Pacific and induce ascending motion anomalies over the Indo-Pacific region.These anomalies further drive descending motion anomalies over the TP and ascending motion anomalies to the north through regulating the regional Hadley circulation.Therefore,the positive-negative-positive winter precipitation anomalies around the TP are formed.This study improves the previously poor understanding of TP climate variation at interdecadal timescales.展开更多
Global warming accelerated after the late1970 s and slowed down after the late 1990 s, accompanying the significant interdecadal changes in the regional climate.We hypothesized that the interdecadal changes linearly c...Global warming accelerated after the late1970 s and slowed down after the late 1990 s, accompanying the significant interdecadal changes in the regional climate.We hypothesized that the interdecadal changes linearly consisted of two independent components, anthropogenic forcing and natural decadal variability, which can be represented simply by the radiative forcing effect of carbon dioxide (RFCO_2) and the Pacific Decadal Oscillation(PDO), respectively. The combined effect of the RFCO_2 and PDO could explain the majority of the surface temperature changes during the late 1970 s and 1990 s, but the magnitudes of the relative contribution of the RFCO_2 and the PDO are inconsistent in different regions. For both the surface temperature and geopotential height, the RFCO_2 could induce significantly positive anomalies over almost the entire globe for these two shifts, exhibiting a larger magnitude in the mid–high latitudes and in the late 1990 s shift.The PDO could induce opposite anomalies for the two interdecadal shifts due to its phase transitions(negativepositive–negative). Furthermore, for the shift in the late 1970s, both the RFCO2(53.7 %–66.7 %) and the PDO(33.3 %–46.3 %) were important in regulating the tropical geopotential height, whereas the RFCO_2 dominated the changes in the mid-latitudes. For the western Pacific subtropical high, the RFCO2(PDO) could explain 52.3 %–62.1 %(37.9 %–47.7 %) of the change. The negative effect of the PDO counteracted most of the RFCO_2 effects for the late 1990 s shift.展开更多
Most legume plants can associate with diazotrophic soil bacteria called rhizobia,resulting in new root organs called nodules that enable N2 fixation.Nodulation is an energy-consuming process,and nodule number is tight...Most legume plants can associate with diazotrophic soil bacteria called rhizobia,resulting in new root organs called nodules that enable N2 fixation.Nodulation is an energy-consuming process,and nodule number is tightly regulated by independent systemic signaling pathways controlled by CLE/SUNN and CEP/CRA2.Moreover,nitrate inhibits legume nodulation via local and systemic regulatory pathways.In Medicago truncatula,NLP1 plays important roles in nitrate-induced inhibition of nodulation,but the relationship between systemic and local pathways in mediating nodulation inhibition by nitrate is poorly understood.In this study,we found that nitrate induces CLE35 expression in an NLP1-dependent manner and that NLP1 binds directly to the CLE35 promoter to activate its expression.Grafting experiments revealed that the systemic control of nodule number involves negative regulation by SUNN and positive regulation by CRA2 in the shoot,and that NLP1’s control of the inhibition of rhizobial infection,nodule development,and nitrogenase activity in response to nitrate is determined by the root.Unexpectedly,grafting experiments showed that loss of CRA2 in the root increases nodule number at inhibitory nitrate levels,probably because of CEP1/2 upregulation in the cra2 mutants,suggesting that CRA2 exerts active negative feedback regulation in the root.展开更多
A metal-organic framework (MOF) formulated as [Cd2(μ3-L)2(DMF)4]·H2O (CdL) [H2L=9-(pyridin-4-yl)- 9H-carbazole-3,6-dicarboxylic acid, DMF=N,N-dimethylformamide] was synthesized under solvothermal condi...A metal-organic framework (MOF) formulated as [Cd2(μ3-L)2(DMF)4]·H2O (CdL) [H2L=9-(pyridin-4-yl)- 9H-carbazole-3,6-dicarboxylic acid, DMF=N,N-dimethylformamide] was synthesized under solvothermal condition. Crystal structural analysis reveals that CalL features the layered 2D framework with L2- ligands as 3-connected nodes. The compound CdL emits blue-violet light with the narrow emission peak and the emission maximum at 414 nm upon excitation at the maximum excitation wavelength of 340 nm. The compound CalL has a similar emission spectrum curve to the free H2L ligand that indicates the emission of compound CdL should be originated from the coordinated L2 ligands.展开更多
A three-dimensional (3D) metal-organic framework (MOF) ZnL'O.5H20"O.75DMF (H2L=9-(pyridin-4-yl)-9H-carbazole- 3,6-dicarboxylic acid, DMF=N,N-dimethylformamide) has been synthesized under solvotherrnal condit...A three-dimensional (3D) metal-organic framework (MOF) ZnL'O.5H20"O.75DMF (H2L=9-(pyridin-4-yl)-9H-carbazole- 3,6-dicarboxylic acid, DMF=N,N-dimethylformamide) has been synthesized under solvotherrnal condition. Crystal structure analysis shows that, in ZnL, each dinuclear Zn2(COO)2 unit is doubly-bridged to the other two by the carbazole moieties to form the 1D chains, which are further connected together by pyridine moieties to lead to the 3D framework. ZnL exhibits both high structural stability and good luminescent stability in water with the pH range of 4-10. ZnL displays the luminescent quenching response for Fe3+ in water with good linear correlation between the quenching efficiency and the concentration with Ksv of 10800 M 1 in the low concentration range of 0-0.1 mM. Interestingly, it is observed that the sensing performance for Fe3+ is stable in the pH range of 4-9, enabling ZnL to detect Fe3+ ions in weak acidic and weak basic solutions.展开更多
基金supported by the National Natural Science Foundation of China [grant number 41991281]the National Key R&D Program of China [grant number 2018YFA0606403]the National Natural Science Foundation of China [grant number 41790472]。
基金supported by the National Natural Science Foundation of China [grant numbers 41991281 and 41675083]Fundamental Research Funds of Institute of Atmospheric PhysicsChinese Academy of Sciences [grant number E3680218]。
基金Supported by Natural Science Foundation of Xinjiang Uygur Autonomous Region-Youth Science Fund Project(2022D01B175)Basic Research Business Special Projects of Public Welfare Research Institutes of Xinjiang Uygur Autonomous Region(KY2021037,KY2021038).
文摘[Objectives]To determine the potential habitat range of Caragana acanthophylla in Xinjiang.[Methods]The known distribution points of C.acanthophylla were used as samples,and a MaxEnt model was developed based on their climatic variables to identify key environmental factors affecting the potential habitats of C.acanthophylla through jackknife method and construction of a response relationship between representative variables and habitat suitability;the suitability of habitats for C.acanthophylla in Xinjiang was evaluated based on the output results of the model.[Results](i)The accuracy of the model verified by AUC curve was 0.971,indicating that the potential habitats of C.acanthophylla in Xinjiang predicted by MaxEnt model were highly credible.(ii)The optimum climatic characteristics for the distribution of C.acanthophylla in Xinjiang were:isothermality 18.8%-34%,minimum temperature of coldest month-30℃to-13℃,mean temperature of coldest quarter-18℃ to-4℃,annual precipitation 80-410 mm,precipitation of driest month 0-25 mm,precipitation of driest quarter 0-82 mm,and precipitation of coldest quarter 0-75 mm.(iii)The total potential distribution area of C.acanthophylla in Xinjiang was modeled to be 1.03×10^(5) km^(2),of which 8.54×10^(3)km^(2) was high suitability area,mainly in the front mountain belt of the north slope of Tianshan Mountain in Urumqi City,Changji Hui Autonomous Prefecture,Bortala Mongol Autonomous Prefecture,and Yili Kazak Autonomous Prefecture and the front mountain belt of Barluk Mountain in Tacheng Prefecture.[Conclusions]This study is of great significance for the future scientific management,regeneration,vegetation restoration and ecological protection of C.acanthophylla.
基金supported by the National Natural Science Foundation of China(Grant Nos.4120505441205051 and 41210007)the CASPKU Pioneer Cooperation Program
文摘The combined impact of the Pacific Decadal Oscillation (PDO) and Atlantic Multidecadal Oscillation (AMO) on the summer rainfall in eastern China was investigated using CCSM4. The strongest signals occur with the combination of a positive PDO and a negative AMO (+PDO- AMO), as well as a negative PDO and a positive AMO (-PDO + AMO). For the +PDO- AMO set, significant positive rainfall anomalies occur over the lower reaches of the Yangtze River valley (YR), when the East Asian summer monsoon becomes weaker, while the East Asian westerly jet stream becomes stronger, and ascending motion over the YR becomes enhanced due to the jet-related secondary circulation. Contrary anomalies occur over East Asia for the -PDO + AMO set. The influence of these two combinations of PDO and AMO on the summer rainfall in eastern China can also be observed in the two interdecadal rainfall changes in eastern China in the late 1970s and late 1990s.
基金This study was jointly supported by the Second Tibetan Plateau Scientific Expedition and Research(STEP)program[grant number 2019QZKK0102]the National Natural Science Foundation of China[grant numbers 41675083 and 41991281].
文摘Classical monsoon dynamics considers the winter/spring snow amount on the Tibetan Plateau(TP)as a major factor driving the East Asian summer monsoon(EASM)for its direct influence on the land-sea thermal contrast.Actually,the TP snow increased and decreased after the late 1970s and 1990s,respectively,accompanying the two major interdecadal changes in the EASM.Although studies have explored the possible mechanisms of the EASM interdecadal variations,and change in TP snow is considered as one of the major drivers,few studies have illustrated the underlying mechanisms of the interdecadal changes in the winter TP snow.This study reveals a tripole pattern of change,with decreased winter precipitation over the TP and an increase to its north and south after the late 1990s.Further analyses through numerical experiments demonstrate that the tropical Pacific SST changes in the late 1990s can robustly affect the winter TP precipitation through regulating the Walker and regional Hadley circulation.The cooling over the tropical central-eastern Pacific can enhance the Walker circulation cell over the Pacific and induce ascending motion anomalies over the Indo-Pacific region.These anomalies further drive descending motion anomalies over the TP and ascending motion anomalies to the north through regulating the regional Hadley circulation.Therefore,the positive-negative-positive winter precipitation anomalies around the TP are formed.This study improves the previously poor understanding of TP climate variation at interdecadal timescales.
基金supported by the National Natural Science Foundation of China(4120505441205051)+1 种基金the Strategic Technological Program of the Chinese Academy of Sciences(XDA05090405)he Special Fund for the Public Welfare Industry(201006022)
文摘Global warming accelerated after the late1970 s and slowed down after the late 1990 s, accompanying the significant interdecadal changes in the regional climate.We hypothesized that the interdecadal changes linearly consisted of two independent components, anthropogenic forcing and natural decadal variability, which can be represented simply by the radiative forcing effect of carbon dioxide (RFCO_2) and the Pacific Decadal Oscillation(PDO), respectively. The combined effect of the RFCO_2 and PDO could explain the majority of the surface temperature changes during the late 1970 s and 1990 s, but the magnitudes of the relative contribution of the RFCO_2 and the PDO are inconsistent in different regions. For both the surface temperature and geopotential height, the RFCO_2 could induce significantly positive anomalies over almost the entire globe for these two shifts, exhibiting a larger magnitude in the mid–high latitudes and in the late 1990 s shift.The PDO could induce opposite anomalies for the two interdecadal shifts due to its phase transitions(negativepositive–negative). Furthermore, for the shift in the late 1970s, both the RFCO2(53.7 %–66.7 %) and the PDO(33.3 %–46.3 %) were important in regulating the tropical geopotential height, whereas the RFCO_2 dominated the changes in the mid-latitudes. For the western Pacific subtropical high, the RFCO2(PDO) could explain 52.3 %–62.1 %(37.9 %–47.7 %) of the change. The negative effect of the PDO counteracted most of the RFCO_2 effects for the late 1990 s shift.
基金supported by grants from The National Key Research&Development Program of China(2016YFA0500500 and 2016YFD0100702)the NSFC(31670242)to F.X.
文摘Most legume plants can associate with diazotrophic soil bacteria called rhizobia,resulting in new root organs called nodules that enable N2 fixation.Nodulation is an energy-consuming process,and nodule number is tightly regulated by independent systemic signaling pathways controlled by CLE/SUNN and CEP/CRA2.Moreover,nitrate inhibits legume nodulation via local and systemic regulatory pathways.In Medicago truncatula,NLP1 plays important roles in nitrate-induced inhibition of nodulation,but the relationship between systemic and local pathways in mediating nodulation inhibition by nitrate is poorly understood.In this study,we found that nitrate induces CLE35 expression in an NLP1-dependent manner and that NLP1 binds directly to the CLE35 promoter to activate its expression.Grafting experiments revealed that the systemic control of nodule number involves negative regulation by SUNN and positive regulation by CRA2 in the shoot,and that NLP1’s control of the inhibition of rhizobial infection,nodule development,and nitrogenase activity in response to nitrate is determined by the root.Unexpectedly,grafting experiments showed that loss of CRA2 in the root increases nodule number at inhibitory nitrate levels,probably because of CEP1/2 upregulation in the cra2 mutants,suggesting that CRA2 exerts active negative feedback regulation in the root.
文摘A metal-organic framework (MOF) formulated as [Cd2(μ3-L)2(DMF)4]·H2O (CdL) [H2L=9-(pyridin-4-yl)- 9H-carbazole-3,6-dicarboxylic acid, DMF=N,N-dimethylformamide] was synthesized under solvothermal condition. Crystal structural analysis reveals that CalL features the layered 2D framework with L2- ligands as 3-connected nodes. The compound CdL emits blue-violet light with the narrow emission peak and the emission maximum at 414 nm upon excitation at the maximum excitation wavelength of 340 nm. The compound CalL has a similar emission spectrum curve to the free H2L ligand that indicates the emission of compound CdL should be originated from the coordinated L2 ligands.
基金supported by Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD) (YX03001)Jiangsu Province Double Innovation Talent Program (090300014001)Nanjing University of Posts & Telecommunications (NY212004)
文摘A three-dimensional (3D) metal-organic framework (MOF) ZnL'O.5H20"O.75DMF (H2L=9-(pyridin-4-yl)-9H-carbazole- 3,6-dicarboxylic acid, DMF=N,N-dimethylformamide) has been synthesized under solvotherrnal condition. Crystal structure analysis shows that, in ZnL, each dinuclear Zn2(COO)2 unit is doubly-bridged to the other two by the carbazole moieties to form the 1D chains, which are further connected together by pyridine moieties to lead to the 3D framework. ZnL exhibits both high structural stability and good luminescent stability in water with the pH range of 4-10. ZnL displays the luminescent quenching response for Fe3+ in water with good linear correlation between the quenching efficiency and the concentration with Ksv of 10800 M 1 in the low concentration range of 0-0.1 mM. Interestingly, it is observed that the sensing performance for Fe3+ is stable in the pH range of 4-9, enabling ZnL to detect Fe3+ ions in weak acidic and weak basic solutions.