The large-aperture pulse compression grating(PCG) is a critical component in generating an ultra-high-intensity, ultra-short-pulse laser;however, the size of the PCG manufactured by transmission holographic exposure i...The large-aperture pulse compression grating(PCG) is a critical component in generating an ultra-high-intensity, ultra-short-pulse laser;however, the size of the PCG manufactured by transmission holographic exposure is limited to large-scale high-quality materials. The reflective method is a potential way for solving the size limitation, but there is still no successful precedent due to the lack of scientific specifications and advanced processing technology of exposure mirrors. In this paper, an analytical model is developed to clarify the specifications of components, and advanced processing technology is adopted to control the spatial frequency errors. Hereafter, we have successfully fabricated a multilayer dielectric grating of 200 mm × 150 mm by using an off-axis reflective exposure system with Φ300 mm. This demonstration proves that PCGs can be manufactured by using the reflection holographic exposure method and shows the potential for manufacturing the meter-level gratings used in 100 petawatt class high-power lasers.展开更多
As the most promising alternative to traditional indium tin oxide (ITO), silver nanowire (AgNW) composite transparent electrodes with improved stabilities compared with that of the pristine AgNWs networks have bee...As the most promising alternative to traditional indium tin oxide (ITO), silver nanowire (AgNW) composite transparent electrodes with improved stabilities compared with that of the pristine AgNWs networks have been demonstrated in various devices. However, a stable AgNW/polymer composite as the bottom electrode for perovskite solar cells has not yet been reported. Here, a long-term stable, smooth AgNW composite with an antioxidant-modified chitosan polymer was developed. The modified polymer can effectively protect pristine AgNWs from side reactions with perovskite, whereas it does not block the carrier drift through the interface of the insulating polymer. The as-prepared AgNW/polymer composite electrode exhibited a root mean square roughness below 10 nm at a scan size of 50 μm × 50 μm, and its original sheet resistance did not change obviously after aging at 85 ℃ for 40 days in air. As a result, the perovskite solar cell employing the composite as the bottom electrode yielded a power conversion efficiency of 7.9%, which corresponds to nearly 75% of that of the reference device with an ITO electrode.展开更多
In this paper,a 2D angle amplifier based on peristrophic multiplexed volume Bragg gratings is designed and prepared,in which a calculation method is firstly proposed to optimize the number of channels to a minimum.The...In this paper,a 2D angle amplifier based on peristrophic multiplexed volume Bragg gratings is designed and prepared,in which a calculation method is firstly proposed to optimize the number of channels to a minimum.The induction of peristrophic multiplexing reduces the performance difference in one bulk of the grating,whereas there is no need to deliberately optimize the fabrication process.It is revealed that a discrete 2D angle deflection range of±30°is obtained and the relative diffraction efficiency of all the grating channels reaches more than 55%with a root-meansquare deviation of less than 3.4%in the same grating.The deviation of the Bragg incidence and exit angles from the expected values is less than 0.07°.It is believed that the proposed 2D angle amplifier has the potential to realize high-performance and large-angle beam steering in high-power laser beam scanning systems.展开更多
Zn_3V_3O_8 two-dimensional micro sheets are successfully synthesized by combination of solvothermal method and heat treatment. The X-ray diffraction(XRD) and field emission scanning electron microscopy(SEM) are used t...Zn_3V_3O_8 two-dimensional micro sheets are successfully synthesized by combination of solvothermal method and heat treatment. The X-ray diffraction(XRD) and field emission scanning electron microscopy(SEM) are used to characterize the structure and morphology of the samples, and the battery testing system is used to investigate its electrochemical performance. The results show that the Zn_3V_3O_8 is successfully obtained using mix solvent(water:ethylene glycol =1:1), and the sample takes on morphology of two-dimensional sheets. The initial discharge capacity for Zn_3V_3O_8 two-dimensional micro sheets is 752.0 mAh/g at 100 mA/g in the voltage range of 0.01-3 V. After heat treatment in a tube furnace at 550 ℃, the sample had the initial discharge capacity as 1152.0 mAh/g and maintained it at 901.4 mAh/g after 100 cycles. The good electrochemical performance for Zn_3V_3O_8 two-dimensional micro sheets make it possible to be used as novel anode for lithium ion battery application.展开更多
Maximizing the energy-loading performance of gratings is a universal theme in high-energy pulse compression.However,sporadic grating designs strongly restrict the development of high-power laser engineering.This study...Maximizing the energy-loading performance of gratings is a universal theme in high-energy pulse compression.However,sporadic grating designs strongly restrict the development of high-power laser engineering.This study proposes an all-and mixed-dielectric grating design paradigm for Nd:glass-based pulse compressors.The solution regions are classified according to the line density.High diffraction efficiency solutions are described in more detail based on the dispersion amount and incident angle.Moreover,an energy scaling factor of 7.09 times larger than that of the National Ignition Facility’s Advanced Radiographic Capability(NIF-ARC)is obtained by taking advantage of the low electric field intensity at transverse magnetic polarization and a small incident angle.These results make a pioneering contribution to facilitate future 20–50-petawatt-class ultrafast laser systems.展开更多
Measuring the topological charge(TC) of optical vortex beams by the edge-diffraction pattern of a single plate is proposed and demonstrated. The diffraction fringes can keep well discernible in a wide three-dimensiona...Measuring the topological charge(TC) of optical vortex beams by the edge-diffraction pattern of a single plate is proposed and demonstrated. The diffraction fringes can keep well discernible in a wide three-dimensional range in this method. The redundant fringes of the diffracted fork-shaped pattern in the near-field can determine the TC value, and the orientation of the fork tells the handedness of the vortex. The plate can be opaque or translucent, and the requirement of the translucent plate for TC measurement is analyzed. Measurement of TCs up to ±40 is experimentally demonstrated by subtracting the upper and lower fringe numbers with respect to the center of the light. The plate is easy to get, and this feasible measurement can bring great convenience and efficiency for researchers.展开更多
基金supported by the National Key R&D Program of China(2020YFA0714500)the National Natural Science Youth Foundation of China(62205352)+5 种基金the Member of Youth Innovation Promotion Association of the Chinese Academy of Sciencesthe International Partnership Program of the Chinese Academy of Sciences(181231KYSB20200040)the Chinese Academy of Sciences President’s International Fellowship Initiative(2023VMB0008)the Shanghai Sailing Program(20YF1454800)the Natural Science Foundation of Shanghai(21ZR1472000)the Shanghai Strategic Emerging Industry Development Special Fund(31011442501217020191D3101001)。
文摘The large-aperture pulse compression grating(PCG) is a critical component in generating an ultra-high-intensity, ultra-short-pulse laser;however, the size of the PCG manufactured by transmission holographic exposure is limited to large-scale high-quality materials. The reflective method is a potential way for solving the size limitation, but there is still no successful precedent due to the lack of scientific specifications and advanced processing technology of exposure mirrors. In this paper, an analytical model is developed to clarify the specifications of components, and advanced processing technology is adopted to control the spatial frequency errors. Hereafter, we have successfully fabricated a multilayer dielectric grating of 200 mm × 150 mm by using an off-axis reflective exposure system with Φ300 mm. This demonstration proves that PCGs can be manufactured by using the reflection holographic exposure method and shows the potential for manufacturing the meter-level gratings used in 100 petawatt class high-power lasers.
基金This study was sponsored by 59th China Postdoctoral Science Foundation (No. 2016M590318), Special Financial Grant from China Postdoctoral Sdence Foundation (No. 2017T100270), National Natural Science Foundation of China (Nos. 51603043 and 51673042), and the Program for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Leaming (No. TP2015002).
文摘As the most promising alternative to traditional indium tin oxide (ITO), silver nanowire (AgNW) composite transparent electrodes with improved stabilities compared with that of the pristine AgNWs networks have been demonstrated in various devices. However, a stable AgNW/polymer composite as the bottom electrode for perovskite solar cells has not yet been reported. Here, a long-term stable, smooth AgNW composite with an antioxidant-modified chitosan polymer was developed. The modified polymer can effectively protect pristine AgNWs from side reactions with perovskite, whereas it does not block the carrier drift through the interface of the insulating polymer. The as-prepared AgNW/polymer composite electrode exhibited a root mean square roughness below 10 nm at a scan size of 50 μm × 50 μm, and its original sheet resistance did not change obviously after aging at 85 ℃ for 40 days in air. As a result, the perovskite solar cell employing the composite as the bottom electrode yielded a power conversion efficiency of 7.9%, which corresponds to nearly 75% of that of the reference device with an ITO electrode.
基金supported by the National Key R&D Program of China(No.2020YFA0714500)the Shanghai Strategic Emerging Industry Development Special Fund(No.31011442501217020191D3101001)+1 种基金the National Natural Science Foundation of China(Nos.61875212 and U1831211)the International Partnership Program of Chinese Academy of Sciences(No.181231KYSB20200040)
文摘In this paper,a 2D angle amplifier based on peristrophic multiplexed volume Bragg gratings is designed and prepared,in which a calculation method is firstly proposed to optimize the number of channels to a minimum.The induction of peristrophic multiplexing reduces the performance difference in one bulk of the grating,whereas there is no need to deliberately optimize the fabrication process.It is revealed that a discrete 2D angle deflection range of±30°is obtained and the relative diffraction efficiency of all the grating channels reaches more than 55%with a root-meansquare deviation of less than 3.4%in the same grating.The deviation of the Bragg incidence and exit angles from the expected values is less than 0.07°.It is believed that the proposed 2D angle amplifier has the potential to realize high-performance and large-angle beam steering in high-power laser beam scanning systems.
基金Financial support by the National Natural Science Foundation of China (No. 21476063)
文摘Zn_3V_3O_8 two-dimensional micro sheets are successfully synthesized by combination of solvothermal method and heat treatment. The X-ray diffraction(XRD) and field emission scanning electron microscopy(SEM) are used to characterize the structure and morphology of the samples, and the battery testing system is used to investigate its electrochemical performance. The results show that the Zn_3V_3O_8 is successfully obtained using mix solvent(water:ethylene glycol =1:1), and the sample takes on morphology of two-dimensional sheets. The initial discharge capacity for Zn_3V_3O_8 two-dimensional micro sheets is 752.0 mAh/g at 100 mA/g in the voltage range of 0.01-3 V. After heat treatment in a tube furnace at 550 ℃, the sample had the initial discharge capacity as 1152.0 mAh/g and maintained it at 901.4 mAh/g after 100 cycles. The good electrochemical performance for Zn_3V_3O_8 two-dimensional micro sheets make it possible to be used as novel anode for lithium ion battery application.
基金This work was supported by the National Key R&D Program of China(No.2020YFA0714500)the National Natural Science Foundation of China(Nos.61875212 and U1831211)+2 种基金the Shanghai Strategic Emerging Industry Development Special Fund(No.31011442501217020191D3101001)the International Partnership Program of Chinese Academy of Sciences(No.181231KYSB20200040)the Strategic Priority Research Program of Chinese Academy of Sciences(No.XDA25020314).
文摘Maximizing the energy-loading performance of gratings is a universal theme in high-energy pulse compression.However,sporadic grating designs strongly restrict the development of high-power laser engineering.This study proposes an all-and mixed-dielectric grating design paradigm for Nd:glass-based pulse compressors.The solution regions are classified according to the line density.High diffraction efficiency solutions are described in more detail based on the dispersion amount and incident angle.Moreover,an energy scaling factor of 7.09 times larger than that of the National Ignition Facility’s Advanced Radiographic Capability(NIF-ARC)is obtained by taking advantage of the low electric field intensity at transverse magnetic polarization and a small incident angle.These results make a pioneering contribution to facilitate future 20–50-petawatt-class ultrafast laser systems.
基金supported by the National Key R&D Program of China (No. 2020YFA0714500)National Natural Science Foundation of China (Nos. 61875212 and U1831211)Shanghai Strategic Emerging Industry Development Special Fund (No. 31011442501217020191D3101001)。
文摘Measuring the topological charge(TC) of optical vortex beams by the edge-diffraction pattern of a single plate is proposed and demonstrated. The diffraction fringes can keep well discernible in a wide three-dimensional range in this method. The redundant fringes of the diffracted fork-shaped pattern in the near-field can determine the TC value, and the orientation of the fork tells the handedness of the vortex. The plate can be opaque or translucent, and the requirement of the translucent plate for TC measurement is analyzed. Measurement of TCs up to ±40 is experimentally demonstrated by subtracting the upper and lower fringe numbers with respect to the center of the light. The plate is easy to get, and this feasible measurement can bring great convenience and efficiency for researchers.