The rapid warming of the Arctic,accompanied by glacier and sea ice melt,has significant consequences for the Earth’s climate,ecosystems,and economy.Black carbon(BC)deposition on snow and ice can trigger a significant...The rapid warming of the Arctic,accompanied by glacier and sea ice melt,has significant consequences for the Earth’s climate,ecosystems,and economy.Black carbon(BC)deposition on snow and ice can trigger a significant reduction in snow albedo and accelerate melting of snow and ice in the Arctic.By reviewing the published literatures over the past decades,this work provides an overview of the progress in both the measurement and modeling of BC deposition and its impact on Arctic climate change.In summary,the maximum value of BC deposition appears in the western Russian Arctic(26 ng·g^(–1)),and the minimum value appears in Greenland(3 ng·g^(–1)).BC records in the Arctic ice core already peaked in 1920s and 1970s,and shows a regional difference between Greenland and Canadian Arctic.The different temporal variations of Arctic BC ice core records in different regions are closely related to the large variability of BC emissions and transportation processes across the Arctic region.Model simulations usually underestimate the concentration of BC in snow and ice by 2–3 times,and cannot accurately reflect the seasonal and regional changes in BC deposition.Wet deposition is the main removal mechanism of BC in the Arctic,and observations show different seasonal variations in BC wet deposition in Ny-Ålesund and Barrow.This discrepancy may result from varying contributions of anthropogenic and biomass burning(BB)emissions,given the strong influence by BC from BB emissions at Barrow.Arctic BC deposition significantly influences regional climate change in the Arctic,increasing fire activities in the Arctic have made BB source of Arctic BC more crucial.On average,BC in Arctic snow and ice causes an increase of+0.17 W·m^(–2)in radiative forcing and 8 Gt·a^(–1)in runoff in Greenland.As stressed in the latest Arctic Monitoring and Assessment Programme report,reliable source information and long-term and high-resolution observations on Arctic BC deposition will be crucial for a more comprehensive understanding and a better mitigation strategy of Arctic BC.In the future,it is necessary to collect more observations on BC deposition and the corresponding physical processes(e.g.,snow/ice melting,surface energy balance)in the Arctic to provide reliable data for understanding and clarifying the mechanism of the climatic impacts of BC deposition on Arctic snow and ice.展开更多
Air pollution caused by particulate matter has significantly improved in China in recent years since the implementation of a series of stringent clean-air regulations.However,surface ozone concentrations have increase...Air pollution caused by particulate matter has significantly improved in China in recent years since the implementation of a series of stringent clean-air regulations.However,surface ozone concentrations have increased,especially in developed city clusters,such as the Beijing–Tianjin–Hebei,Yangtze River Delta,Pearl River Delta,and Sichuan Basin regions.Due to the complexity and nonlinearity of the ozone formation,accurately locating major sources of ozone and its precursors is an important basis for the formulation of cost-effective pollution control strategies.In this paper,the authors systematically summarize the reported results and outcomes of the methods and main conclusions of ozone source apportionment(regions and categories)in China from the published literature,based on observation-based methods and emission-based methods,respectively.The authors aim to provide a comprehensive understanding of ozone pollution and reliable references for the formulation of air pollution prevention policies in China.展开更多
A regional chemical transport model,RAMS-CMAQ,was employed to assess the impacts of biosphere-atmosphere CO2 exchange on seasonal variations in atmospheric CO2 concentrations over East Asia.Simulated CO2 concentration...A regional chemical transport model,RAMS-CMAQ,was employed to assess the impacts of biosphere-atmosphere CO2 exchange on seasonal variations in atmospheric CO2 concentrations over East Asia.Simulated CO2 concentrations were compared with observations at 12 surface stations and the comparison showed they were generally in good agreement.Both observations and simulations suggested that surface CO2 over East Asia features a summertime trough due to biospheric absorption,while in some urban areas surface CO2 has a distinct summer peak,which could be attributed to the strong impact from anthropogenic emissions.Analysis of the model results indicated that biospheric fluxes and fossil-fuel emissions are comparably important in shaping spatial distributions of CO2 near the surface over East Asia.Biospheric flux plays an important role in the prevailing spatial pattern of CO2 enhancement and reduction on the synoptic scale due to the strong seasonality of biospheric CO2 flux.The elevation of CO2 levels by the biosphere during winter was found to be larger than 5 ppm in North China and Southeast China,and during summertime a significant depletion （≥ 7 ppm） occurred in most areas,except for the Indo-China Peninsula where positive bioflux values were found.展开更多
We propose a new method to estimate surface-level particulate matter(PM)concentrations by using satellite-retrieved Aerosol Optical Thickness(AOT).This method considers the distribution and variation of Planetary Boun...We propose a new method to estimate surface-level particulate matter(PM)concentrations by using satellite-retrieved Aerosol Optical Thickness(AOT).This method considers the distribution and variation of Planetary Boundary Layer(PBL)height and relative humidity(RH)at the regional scale.The method estimates surface-level particulate matter concentrations using the data simulated by an atmospheric boundary layer model RAMS and satellite-retrieved AOT.By incorporation MODIS AOT,PBL height and RH simulated by RAMS,this method is applied to estimate the surface-level PM 2.5 concentrations in North China region.The result is evaluated by using 16 ground-based observations deployed in the research region,and the result shows a good agreement between estimated PM 2.5 concentrations and observations,and the coefficient of determination R2 is 0.61 between the estimated PM 2.5 concentrations and the observations.In addition,surface-level PM 2.5 concentrations are also estimated by using MODIS AOT,ground-based LIDAR observations and RH measurements.A comparison between the two estimated PM 2.5 concentrations shows that the new method proposed in this paper is better than the traditional method.The coefficient of determination R2 is improved from 0.32 to 0.62.展开更多
Based on simulated major aerosol concentrations (e.g., sulfate, nitrate, ammonium, organic carbon, black carbon, and sea salt) over East Asia during the year 2005 by using the Multi-scale Air Quality modeling system (...Based on simulated major aerosol concentrations (e.g., sulfate, nitrate, ammonium, organic carbon, black carbon, and sea salt) over East Asia during the year 2005 by using the Multi-scale Air Quality modeling system (RAMS-CMAQ), the aerosol optical depth (AOD) was calculated by the reconstruction mass-extinction method and then analyzed to explore its characteristics in temporal-spatial distributions. For evaluating the model performances, simulated AOD values were compared against observations at stations of the Aerosol Robotic Network (AERONET) and the Chinese Sun Hazemeter Network (CSHNET). The comparison shows that the model can well reproduce observed temporal and spatial features of AOD, especially in natural en- vironment. However, the simulated AOD values are underestimated over urban and suburban regions with dense human activities. Analysis of simulation results indicates that AOD varies significantly in time and space, and generally, AOD values are lower in summer and higher in winter. Excluding the contribution from soil dust aerosols, high AOD values (over 0.8) are found over the Sichuan Basin, South China, and Central China in several months, while low values (less than 0.2) are over northern and western areas of East Asia and southern sea regions. Analysis also shows that aerosols such as sulfate, nitrate, and ammonium are main contributors to AOD in East Asia, and their contributions are over 80% in most high AOD areas, while black carbon aerosols play an important role in northern China where dense human activities exist, especially in the winter time.展开更多
Here we introduce generalized momentum and coordinate to transform seismic wave displacement equations into Hamiltonian system.We define the Lie operators associated with kinetic and potential energy,and construct a n...Here we introduce generalized momentum and coordinate to transform seismic wave displacement equations into Hamiltonian system.We define the Lie operators associated with kinetic and potential energy,and construct a new kind of second order symplectic scheme,which is extremely suitable for high efficient and long-term seismic wave simulations.Three sets of optimal coefficients are obtained based on the principle of minimum truncation error.We investigate the stability conditions for elastic wave simulation in homogeneous media.These newly developed symplectic schemes are compared with common symplectic schemes to verify the high precision and efficiency in theory and numerical experiments.One of the schemes presented here is compared with the classical Newmark algorithm and third order symplectic scheme to test the long-term computational ability.The scheme gets the same synthetic surface seismic records and single channel record as third order symplectic scheme in the seismic modeling in the heterogeneous model.展开更多
基金supported by the National Key Research and Development Program(Grant nos.2022YFC2807203,2022YFB2302701).
文摘The rapid warming of the Arctic,accompanied by glacier and sea ice melt,has significant consequences for the Earth’s climate,ecosystems,and economy.Black carbon(BC)deposition on snow and ice can trigger a significant reduction in snow albedo and accelerate melting of snow and ice in the Arctic.By reviewing the published literatures over the past decades,this work provides an overview of the progress in both the measurement and modeling of BC deposition and its impact on Arctic climate change.In summary,the maximum value of BC deposition appears in the western Russian Arctic(26 ng·g^(–1)),and the minimum value appears in Greenland(3 ng·g^(–1)).BC records in the Arctic ice core already peaked in 1920s and 1970s,and shows a regional difference between Greenland and Canadian Arctic.The different temporal variations of Arctic BC ice core records in different regions are closely related to the large variability of BC emissions and transportation processes across the Arctic region.Model simulations usually underestimate the concentration of BC in snow and ice by 2–3 times,and cannot accurately reflect the seasonal and regional changes in BC deposition.Wet deposition is the main removal mechanism of BC in the Arctic,and observations show different seasonal variations in BC wet deposition in Ny-Ålesund and Barrow.This discrepancy may result from varying contributions of anthropogenic and biomass burning(BB)emissions,given the strong influence by BC from BB emissions at Barrow.Arctic BC deposition significantly influences regional climate change in the Arctic,increasing fire activities in the Arctic have made BB source of Arctic BC more crucial.On average,BC in Arctic snow and ice causes an increase of+0.17 W·m^(–2)in radiative forcing and 8 Gt·a^(–1)in runoff in Greenland.As stressed in the latest Arctic Monitoring and Assessment Programme report,reliable source information and long-term and high-resolution observations on Arctic BC deposition will be crucial for a more comprehensive understanding and a better mitigation strategy of Arctic BC.In the future,it is necessary to collect more observations on BC deposition and the corresponding physical processes(e.g.,snow/ice melting,surface energy balance)in the Arctic to provide reliable data for understanding and clarifying the mechanism of the climatic impacts of BC deposition on Arctic snow and ice.
基金supported by the National Natural Science Foundation of China grant number 41830109the National Key R&D Programs of China grant number2017YFB0503901。
文摘Air pollution caused by particulate matter has significantly improved in China in recent years since the implementation of a series of stringent clean-air regulations.However,surface ozone concentrations have increased,especially in developed city clusters,such as the Beijing–Tianjin–Hebei,Yangtze River Delta,Pearl River Delta,and Sichuan Basin regions.Due to the complexity and nonlinearity of the ozone formation,accurately locating major sources of ozone and its precursors is an important basis for the formulation of cost-effective pollution control strategies.In this paper,the authors systematically summarize the reported results and outcomes of the methods and main conclusions of ozone source apportionment(regions and categories)in China from the published literature,based on observation-based methods and emission-based methods,respectively.The authors aim to provide a comprehensive understanding of ozone pollution and reliable references for the formulation of air pollution prevention policies in China.
基金supported by the Strategic Priority Research Program–Climate Change: Carbon Budget and Relevant Issues (Grant No. XDA05040404)the National High Technology Research and Development Program of China (Grant No. 2013AA122002)+1 种基金the National Natural Science Foundation of China (Grant No. 41130528)support staff of the stations for providing their CO2 observation records on the WDCGG website
文摘A regional chemical transport model,RAMS-CMAQ,was employed to assess the impacts of biosphere-atmosphere CO2 exchange on seasonal variations in atmospheric CO2 concentrations over East Asia.Simulated CO2 concentrations were compared with observations at 12 surface stations and the comparison showed they were generally in good agreement.Both observations and simulations suggested that surface CO2 over East Asia features a summertime trough due to biospheric absorption,while in some urban areas surface CO2 has a distinct summer peak,which could be attributed to the strong impact from anthropogenic emissions.Analysis of the model results indicated that biospheric fluxes and fossil-fuel emissions are comparably important in shaping spatial distributions of CO2 near the surface over East Asia.Biospheric flux plays an important role in the prevailing spatial pattern of CO2 enhancement and reduction on the synoptic scale due to the strong seasonality of biospheric CO2 flux.The elevation of CO2 levels by the biosphere during winter was found to be larger than 5 ppm in North China and Southeast China,and during summertime a significant depletion （≥ 7 ppm） occurred in most areas,except for the Indo-China Peninsula where positive bioflux values were found.
基金supported by National Department Public Benefit Research Foundation (Ministry of Environmental Protection of the People’s Republic of China) (Grant No. 201009001)National Natural Science Foundation of China (Grant No. 41101327)
文摘We propose a new method to estimate surface-level particulate matter(PM)concentrations by using satellite-retrieved Aerosol Optical Thickness(AOT).This method considers the distribution and variation of Planetary Boundary Layer(PBL)height and relative humidity(RH)at the regional scale.The method estimates surface-level particulate matter concentrations using the data simulated by an atmospheric boundary layer model RAMS and satellite-retrieved AOT.By incorporation MODIS AOT,PBL height and RH simulated by RAMS,this method is applied to estimate the surface-level PM 2.5 concentrations in North China region.The result is evaluated by using 16 ground-based observations deployed in the research region,and the result shows a good agreement between estimated PM 2.5 concentrations and observations,and the coefficient of determination R2 is 0.61 between the estimated PM 2.5 concentrations and the observations.In addition,surface-level PM 2.5 concentrations are also estimated by using MODIS AOT,ground-based LIDAR observations and RH measurements.A comparison between the two estimated PM 2.5 concentrations shows that the new method proposed in this paper is better than the traditional method.The coefficient of determination R2 is improved from 0.32 to 0.62.
基金supported by National Basic Research Program of China (Grant Nos. 2006CB403702 and 2007CB407303)the Program for Innovative Research Team in Beijing Branch of Chinese Academy of Sciences and Beijing Academy of Science and Technology
文摘Based on simulated major aerosol concentrations (e.g., sulfate, nitrate, ammonium, organic carbon, black carbon, and sea salt) over East Asia during the year 2005 by using the Multi-scale Air Quality modeling system (RAMS-CMAQ), the aerosol optical depth (AOD) was calculated by the reconstruction mass-extinction method and then analyzed to explore its characteristics in temporal-spatial distributions. For evaluating the model performances, simulated AOD values were compared against observations at stations of the Aerosol Robotic Network (AERONET) and the Chinese Sun Hazemeter Network (CSHNET). The comparison shows that the model can well reproduce observed temporal and spatial features of AOD, especially in natural en- vironment. However, the simulated AOD values are underestimated over urban and suburban regions with dense human activities. Analysis of simulation results indicates that AOD varies significantly in time and space, and generally, AOD values are lower in summer and higher in winter. Excluding the contribution from soil dust aerosols, high AOD values (over 0.8) are found over the Sichuan Basin, South China, and Central China in several months, while low values (less than 0.2) are over northern and western areas of East Asia and southern sea regions. Analysis also shows that aerosols such as sulfate, nitrate, and ammonium are main contributors to AOD in East Asia, and their contributions are over 80% in most high AOD areas, while black carbon aerosols play an important role in northern China where dense human activities exist, especially in the winter time.
基金financially supported by the National Natural Science Foundation of China(Grant Nos.41174047,40874024&41204041)
文摘Here we introduce generalized momentum and coordinate to transform seismic wave displacement equations into Hamiltonian system.We define the Lie operators associated with kinetic and potential energy,and construct a new kind of second order symplectic scheme,which is extremely suitable for high efficient and long-term seismic wave simulations.Three sets of optimal coefficients are obtained based on the principle of minimum truncation error.We investigate the stability conditions for elastic wave simulation in homogeneous media.These newly developed symplectic schemes are compared with common symplectic schemes to verify the high precision and efficiency in theory and numerical experiments.One of the schemes presented here is compared with the classical Newmark algorithm and third order symplectic scheme to test the long-term computational ability.The scheme gets the same synthetic surface seismic records and single channel record as third order symplectic scheme in the seismic modeling in the heterogeneous model.
