综述了近几年来亚波长陷光结构Hg Cd Te红外探测器研究进展.系统介绍了一种结合有限元方法与时域有限差分方法对红外探测器的"光""电"特性进行联合模拟和设计方法,以及基于这种新的数值模拟方法对亚波长人工微结构H...综述了近几年来亚波长陷光结构Hg Cd Te红外探测器研究进展.系统介绍了一种结合有限元方法与时域有限差分方法对红外探测器的"光""电"特性进行联合模拟和设计方法,以及基于这种新的数值模拟方法对亚波长人工微结构Hg Cd Te红外探测器的模拟和分析结果.理论分析和实验研制数据均显示这种新型亚波长人工微结构结构具有很好的陷光特性,在提高长波红外探测器性能方面具有潜在应用前景.展开更多
Surface-enhanced Raman scattering(SERS) has been widely used as an effective technique for lowconcentration molecules detections in the past decades. This work proposes a rapid and accessible process to fabricate SERS...Surface-enhanced Raman scattering(SERS) has been widely used as an effective technique for lowconcentration molecules detections in the past decades. This work proposes a rapid and accessible process to fabricate SERS-active substrates with high uniformity and controllability based on two-step laser ablation. Laser beams directly ablate the surface of Si, concurrently creating microstructures and ejecting molten materials caused by the thermal effect that nucleate in ambient air. The nuclei grow into nanoparticles and deposit over the surface. These nanoparticles,together with microstructures, improve the light collection efficiency of the SERS-active substrates. Especially after Au thin film deposition, these nanoparticles can provide nanogaps as hotspots for SERS. By orthogonal experiment design,laser processing parameters for better performances are determined. Compared with substrates fabricated by single 1064 nm master oscillator power amplifier(MOPA) laser ablation, substrates ablated by the primary 1064 nm MOPA laser and secondary UV pulsed laser show more uniform nanoparticles’ deposition over the surface. The optimized largearea substrate has a SERS detection limit of 10^(-8)mol/L for 4-aminothiophenol(4-ATP), indicating the potential realworld applications for trace detection.展开更多
The stability of perovskite solar cells is an important issue to be addressed for future applications.Perovskite solar cells are vulnerable to exposure to UV light due to promoted chemical reactions.However, preventin...The stability of perovskite solar cells is an important issue to be addressed for future applications.Perovskite solar cells are vulnerable to exposure to UV light due to promoted chemical reactions.However, preventing UV light from entering solar cells lowers the power conversion efficiency by reducing the photocurrent. The challenge is to improve UV stability without sacrificing efficiency. Here, we demonstrate the reduction of UV light-related negative effects from the perspective of spectral modification. By simultaneously introducing UV–visible downshifting and light trapping, perovskite solar cells can achieve a comparable efficiency of over 21% to that of an unmodified device. The optimized device obtains increased UV stability due to UV–visible downshifting. Different from other strategies, spectral modification externally alters the composition of incident light and improves UV stability without changing the internal device architecture, which is broadly applicable to perovskite solar cells with different structures. The present work may also find applications in other types of solar cells to boost the stability of devices exposed to UV light.展开更多
文摘综述了近几年来亚波长陷光结构Hg Cd Te红外探测器研究进展.系统介绍了一种结合有限元方法与时域有限差分方法对红外探测器的"光""电"特性进行联合模拟和设计方法,以及基于这种新的数值模拟方法对亚波长人工微结构Hg Cd Te红外探测器的模拟和分析结果.理论分析和实验研制数据均显示这种新型亚波长人工微结构结构具有很好的陷光特性,在提高长波红外探测器性能方面具有潜在应用前景.
基金Project(2020H0006) supported by the Fujian Provincial Science and Technology ProgrammeChina+2 种基金Project(62175203) supported by the National Natural Science Foundation of ChinaProject(RD2020050301) supported by the Innovation Laboratory for Science and Technology of Energy Materials of Fujian Province Applied Research ProjectChina。
文摘Surface-enhanced Raman scattering(SERS) has been widely used as an effective technique for lowconcentration molecules detections in the past decades. This work proposes a rapid and accessible process to fabricate SERS-active substrates with high uniformity and controllability based on two-step laser ablation. Laser beams directly ablate the surface of Si, concurrently creating microstructures and ejecting molten materials caused by the thermal effect that nucleate in ambient air. The nuclei grow into nanoparticles and deposit over the surface. These nanoparticles,together with microstructures, improve the light collection efficiency of the SERS-active substrates. Especially after Au thin film deposition, these nanoparticles can provide nanogaps as hotspots for SERS. By orthogonal experiment design,laser processing parameters for better performances are determined. Compared with substrates fabricated by single 1064 nm master oscillator power amplifier(MOPA) laser ablation, substrates ablated by the primary 1064 nm MOPA laser and secondary UV pulsed laser show more uniform nanoparticles’ deposition over the surface. The optimized largearea substrate has a SERS detection limit of 10^(-8)mol/L for 4-aminothiophenol(4-ATP), indicating the potential realworld applications for trace detection.
基金supported by the National Natural Science Foundation of China (52025028, 51972218)the 1000 Youth Talents Plan+2 种基金the 333 High-level Talents Cultivation Project of Jiangsu Provincethe Six Talents Peak Project of Jiangsu Provincethe Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions。
文摘The stability of perovskite solar cells is an important issue to be addressed for future applications.Perovskite solar cells are vulnerable to exposure to UV light due to promoted chemical reactions.However, preventing UV light from entering solar cells lowers the power conversion efficiency by reducing the photocurrent. The challenge is to improve UV stability without sacrificing efficiency. Here, we demonstrate the reduction of UV light-related negative effects from the perspective of spectral modification. By simultaneously introducing UV–visible downshifting and light trapping, perovskite solar cells can achieve a comparable efficiency of over 21% to that of an unmodified device. The optimized device obtains increased UV stability due to UV–visible downshifting. Different from other strategies, spectral modification externally alters the composition of incident light and improves UV stability without changing the internal device architecture, which is broadly applicable to perovskite solar cells with different structures. The present work may also find applications in other types of solar cells to boost the stability of devices exposed to UV light.
