Through our newly-developed ＂chemical vapor deposition integrated process （ISVD-IP）＇＂ using carbon OlOXlae （t..u2） as me raw matenal and only carbon source introduced, CO2 could be catalytically activated and c...Through our newly-developed ＂chemical vapor deposition integrated process （ISVD-IP）＇＂ using carbon OlOXlae （t..u2） as me raw matenal and only carbon source introduced, CO2 could be catalytically activated and converted to a new solid-form product, i.e., carbon nanotubes （CO2-derived） at a quite high yield （the single-pass carbon yield in the solid-form carbon-product produced from CO2 catalytic capture and conversion was more than 30% at a single-pass carbon-base）. For comparison, when only pure carbon dioxide was introduced using the conventional CVD method without integrated process, no solid-form carbon-material product could be formed. In the addition of saturated steam at room temperature in the feed for CVD, there were much more end-opening carbon nano-tubes produced, at a slightly higher carbon yield. These inspiring works opened a remarkable and alternative new approach for carbon dioxide catalytic capture to solid-form product, comparing with that of CO2 sequestration （CCS） or CO2 mineralization （solidification）, etc. As a result, there was much less body volume and almost no greenhouse effect for this solid-form carbon-material than those of primitive carbon dioxide.展开更多
The effect of deuteron breakup in d-nucleus reaction is treated with the continuum discretized coupled channels （CDCC） approach, and the effects on the total reaction cross sections and elastic scattering angular di...The effect of deuteron breakup in d-nucleus reaction is treated with the continuum discretized coupled channels （CDCC） approach, and the effects on the total reaction cross sections and elastic scattering angular distributions are studied by comparing the calculations of CDCC and spherical optical model with our global deuteron optical potential [Phys. Rev. C 73 （2006） 054605] below 200 MeV, for target nuclei ranging from ^12C to ^208Pb. The contributions from the closed channels to the total reaction and breakup cross sections, and angular distributions of elastic scattering are also seriously discussed.展开更多
Continuum Discretized Coupled-Channel（CDCC） model calculations of total, complete and incomplete fusion cross sections for reactions of the weakly bound 6Li with 144,154Sm targets at energies around the Coulomb barr...Continuum Discretized Coupled-Channel（CDCC） model calculations of total, complete and incomplete fusion cross sections for reactions of the weakly bound 6Li with 144,154Sm targets at energies around the Coulomb barrier are presented. In the cluster structure frame of 6Li→α＋d, short-range absorption potentials are considered for the interactions between the ground state of the projectile 6Li and α-d fragments with the target. In order to separately calculate complete and incomplete fusion and to reduce double-counting, the corresponding absorption potentials are chosen to be of different range. Couplings to low-lying excited states 2＋, 3-of 144Sm and 2＋, 4＋ of 154Sm are included. So, the effect on total fusion from the excited states of the target is investigated. Similarly, the effect on fusion due to couplings to resonance breakup states of 6Li, namely, l = 2,Jπ= 3＋, 2＋, 1＋ is also calculated.The latter effect is determined by using two approaches,（a） by considering only resonance state couplings and（b）by omitting these states from the full discretized energy space. Among other things, it is found that both resonance and non-resonance continuum breakup couplings produce fusion suppression at all the energies considered.展开更多
基金the National 973 Program of Ministry of Sciences and Technologies of China(2011CB201202)the National Natural Science Foundation of China(20776089)
文摘Through our newly-developed ＂chemical vapor deposition integrated process （ISVD-IP）＇＂ using carbon OlOXlae （t..u2） as me raw matenal and only carbon source introduced, CO2 could be catalytically activated and converted to a new solid-form product, i.e., carbon nanotubes （CO2-derived） at a quite high yield （the single-pass carbon yield in the solid-form carbon-product produced from CO2 catalytic capture and conversion was more than 30% at a single-pass carbon-base）. For comparison, when only pure carbon dioxide was introduced using the conventional CVD method without integrated process, no solid-form carbon-material product could be formed. In the addition of saturated steam at room temperature in the feed for CVD, there were much more end-opening carbon nano-tubes produced, at a slightly higher carbon yield. These inspiring works opened a remarkable and alternative new approach for carbon dioxide catalytic capture to solid-form product, comparing with that of CO2 sequestration （CCS） or CO2 mineralization （solidification）, etc. As a result, there was much less body volume and almost no greenhouse effect for this solid-form carbon-material than those of primitive carbon dioxide.
文摘The effect of deuteron breakup in d-nucleus reaction is treated with the continuum discretized coupled channels （CDCC） approach, and the effects on the total reaction cross sections and elastic scattering angular distributions are studied by comparing the calculations of CDCC and spherical optical model with our global deuteron optical potential [Phys. Rev. C 73 （2006） 054605] below 200 MeV, for target nuclei ranging from ^12C to ^208Pb. The contributions from the closed channels to the total reaction and breakup cross sections, and angular distributions of elastic scattering are also seriously discussed.
基金partly supported by the NSF of China(11120101005,11275248,11525524,11621131001,11647601,11711540016)973 Program of China(2013CB834400)the Key Research Program of Frontier Sciences of CAS.H.Q.Z.from NSF China(11375266)
文摘Continuum Discretized Coupled-Channel（CDCC） model calculations of total, complete and incomplete fusion cross sections for reactions of the weakly bound 6Li with 144,154Sm targets at energies around the Coulomb barrier are presented. In the cluster structure frame of 6Li→α＋d, short-range absorption potentials are considered for the interactions between the ground state of the projectile 6Li and α-d fragments with the target. In order to separately calculate complete and incomplete fusion and to reduce double-counting, the corresponding absorption potentials are chosen to be of different range. Couplings to low-lying excited states 2＋, 3-of 144Sm and 2＋, 4＋ of 154Sm are included. So, the effect on total fusion from the excited states of the target is investigated. Similarly, the effect on fusion due to couplings to resonance breakup states of 6Li, namely, l = 2,Jπ= 3＋, 2＋, 1＋ is also calculated.The latter effect is determined by using two approaches,（a） by considering only resonance state couplings and（b）by omitting these states from the full discretized energy space. Among other things, it is found that both resonance and non-resonance continuum breakup couplings produce fusion suppression at all the energies considered.
