二维数字图像相关(two-dimensional digital image correlation,2D-DIC)在测量过程中不可避免地会出现相机光轴与测量表面非垂直,由此产生的离面位移而将导致较大的测量误差,同时在视场受限的环境中难以通过单台相机完成大范围的变形测...二维数字图像相关(two-dimensional digital image correlation,2D-DIC)在测量过程中不可避免地会出现相机光轴与测量表面非垂直,由此产生的离面位移而将导致较大的测量误差,同时在视场受限的环境中难以通过单台相机完成大范围的变形测量。有鉴于此,该文开发了基于双反射镜的2D-DIC变形测量系统,使用双反射镜成像缓解离面运动对2D-DIC的影响,通过可移动相机实现小视场下的图像采集,提出基于频域移位的高精度图像拼接方法,并改进了融合函数,最终获得试样的高分辨率图像。单轴拉伸实验结果表明,轴向应变的平均相对误差相比传统2D-DIC方法降低12.82%,测量分辨率提高约34.92%,验证了测量系统的可行性和有效性。展开更多
Negatively thermo-responsive 2D membranes,which mimic the stomatal opening/closing of plants,have drawn substantial interest for tunable molecular separation processes.However,these membranes are still restricted sign...Negatively thermo-responsive 2D membranes,which mimic the stomatal opening/closing of plants,have drawn substantial interest for tunable molecular separation processes.However,these membranes are still restricted significantly on account of low water permeability and poor dynamic tunability of 2D nanochannels under temperature stimulation.Here,we present a biomimetic negatively thermo-responsive MXene membrane by covalently grafting poly(N-isopropylacrylamide)(PNIPAm)onto MXene nanosheets.The uniformly grafted PNIPAm polymer chains can enlarge the interlayer spacings for increasing water permeability while also allowing more tunability of 2D nanochannels for enhancing the capability of gradually separating multiple molecules of different sizes.As expected,the constructed membrane exhibits ultrahigh water permeance of 95.6 L m^(-2) h^(-1) bar^(-1) at 25℃,which is eight-fold higher than the state-of-the-art negatively thermoresponsive 2D membranes.Moreover,the highly temperature-tunable 2D nanochannels enable the constructed membrane to perform excellent graded molecular sieving for dye-and antibiotic-based ternary mixtures.This strategy provides new perspectives in engineering smart 2D membrane and expands the scope of temperature-responsive membranes,showing promising applications in micro/nanofluidics and molecular separation.展开更多
文摘二维数字图像相关(two-dimensional digital image correlation,2D-DIC)在测量过程中不可避免地会出现相机光轴与测量表面非垂直,由此产生的离面位移而将导致较大的测量误差,同时在视场受限的环境中难以通过单台相机完成大范围的变形测量。有鉴于此,该文开发了基于双反射镜的2D-DIC变形测量系统,使用双反射镜成像缓解离面运动对2D-DIC的影响,通过可移动相机实现小视场下的图像采集,提出基于频域移位的高精度图像拼接方法,并改进了融合函数,最终获得试样的高分辨率图像。单轴拉伸实验结果表明,轴向应变的平均相对误差相比传统2D-DIC方法降低12.82%,测量分辨率提高约34.92%,验证了测量系统的可行性和有效性。
基金supported by the National Nature Science Foundation of China(No.22278179,U23A20688)the National Key Research and Development Program of China(2021YFB3802600)+3 种基金the Fundamental Research Funds for the Central Universities(JUSRP622035)National First-Class Discipline Program of Light Industry Technology and Engineering(LIFE2018-19)MOE&SAFEA for the 111 Project(B13025)Natural Science Foundation of Xinjiang Uygur Autonomous Region(2022D01D030).
文摘Negatively thermo-responsive 2D membranes,which mimic the stomatal opening/closing of plants,have drawn substantial interest for tunable molecular separation processes.However,these membranes are still restricted significantly on account of low water permeability and poor dynamic tunability of 2D nanochannels under temperature stimulation.Here,we present a biomimetic negatively thermo-responsive MXene membrane by covalently grafting poly(N-isopropylacrylamide)(PNIPAm)onto MXene nanosheets.The uniformly grafted PNIPAm polymer chains can enlarge the interlayer spacings for increasing water permeability while also allowing more tunability of 2D nanochannels for enhancing the capability of gradually separating multiple molecules of different sizes.As expected,the constructed membrane exhibits ultrahigh water permeance of 95.6 L m^(-2) h^(-1) bar^(-1) at 25℃,which is eight-fold higher than the state-of-the-art negatively thermoresponsive 2D membranes.Moreover,the highly temperature-tunable 2D nanochannels enable the constructed membrane to perform excellent graded molecular sieving for dye-and antibiotic-based ternary mixtures.This strategy provides new perspectives in engineering smart 2D membrane and expands the scope of temperature-responsive membranes,showing promising applications in micro/nanofluidics and molecular separation.
