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Simulation of the Ecosystem Productivity Responses to Aerosol Diffuse Radiation Fertilization Effects over the Pan-Arctic during 2001–19 被引量:1
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作者 Zhiding ZHANG Xu YUE +3 位作者 Hao ZHOU Jun ZHU Yadong LEI Chenguang TIAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第1期84-96,共13页
The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).Whil... The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).While such DRFEs have been explored at low to middle latitudes,the aerosol impacts on pan-Arctic ecosystems and the contributions by anthropogenic and natural emission sources remain less quantified.Here,we perform regional simulations at 0.2o×0.2ousing a well-validated vegetation model(Yale Interactive terrestrial Biosphere,YIBs)in combination with multi-source of observations to quantify the impacts of aerosol DRFEs on the net primary productivity(NPP)in the pan-Arctic during 2001-19.Results show that aerosol DRFEs increase pan-Arctic NPP by 2.19 Pg C(12.8%)yr^(-1)under clear-sky conditions,in which natural and anthropogenic sources contribute to 8.9% and 3.9%,respectively.Under all-sky conditions,such DRFEs are largely dampened by cloud to only 0.26 Pg C(1.24%)yr^(-1),with contributions of 0.65% by natural and 0.59% by anthropogenic species.Natural aerosols cause a positive NPP trend of 0.022% yr^(-1)following the increased fire activities in the pan-Arctic.In contrast,anthropogenic aerosols induce a negative trend of-0.01% yr^(-1)due to reduced emissions from the middle latitudes.Such trends in aerosol DRFEs show a turning point in the year of 2007 with more positive NPP trends by natural aerosols but negative NPP trends by anthropogenic aerosols thereafter.Though affected by modeling uncertainties,this study suggests a likely increasing impact of aerosols on terrestrial ecosystems in the pan-Arctic under global warming. 展开更多
关键词 diffuse radiation fertilization effects anthropogenic aerosols natural aerosols pan-Arctic net primary productivity
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Experimental investigation on effective aerosol scavenging using different spray configurations with pre-injection of water mist for Fukushima Daiichi decommissioning
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作者 Rui-Cong Xu Avadhesh Kumar Sharma +2 位作者 Erdal Ozdemir Shuichiro Miwa Shunichi Suzuki 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第5期154-172,共19页
During the decommissioning of the Fukushima Daiichi nuclear power plant,it is important to consider the retrieval of resolidified debris both in air and underwater configurations.For the subsequent retrieval of debris... During the decommissioning of the Fukushima Daiichi nuclear power plant,it is important to consider the retrieval of resolidified debris both in air and underwater configurations.For the subsequent retrieval of debris from the reactor building,the resolidified debris must be cut into smaller pieces using various cutting methods.During the cutting process,aerosol particles are expected to be generated at the submicron scale.It has been noted that such aerosols sizing within the Greenfield gap(0.1-1μm)are difficult to remove effectively using traditional spraying methods.Therefore,to improve the aerosol removal efficiency of the spray system,a new aerosol agglomeration method was recently proposed,which involves injecting water mist to enlarge the sizes of the aerosol particles before removing them using water sprays.In this study,a series of experiments were performed to clarify the proper spray configurations for effective aerosol scavenging and to improve the performance of the water mist.The experimental results showed that the spray flow rate and droplet characteristics are important factors for the aerosol-scavenging efficiency and performance of the water mist.The results obtained from this study will be helpful for the optimization of the spray system design for effective aerosol scavenging during the decommissioning of the Fukushima Daiichi plant. 展开更多
关键词 Fukushima Daiichi decommissioning aerosol scavenging Multiphase flow Spray system aerosol-mist agglomeration
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Contrast in Secondary Organic Aerosols between the Present Day and the Preindustrial Period:The Importance of Nontraditional Sources and the Changed Atmospheric Oxidation Capability
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作者 Yingchuan YANG Wenyi YANG +13 位作者 Xueshun CHEN Jiawen ZHU Huansheng CHEN Yuanlin WANG Wending WANG Lianfang WEI Ying WEI Qian YE Huiyun DU Zichen WU Zhe WANG Jie LI Xiaodong ZENG Zifa WANG 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第10期1936-1952,I0002-I0010,共26页
Quantifying differences in secondary organic aerosols(SOAs)between the preindustrial period and the present day is crucial to assess climate forcing and environmental effects resulting from anthropogenic activities.Th... Quantifying differences in secondary organic aerosols(SOAs)between the preindustrial period and the present day is crucial to assess climate forcing and environmental effects resulting from anthropogenic activities.The lack of vegetation information for the preindustrial period and the uncertainties in describing SOA formation are two leading factors preventing simulation of SOA.This study calculated the online emissions of biogenic volatile organic compounds(VOCs)in the Aerosol and Atmospheric Chemistry Model of the Institute of Atmospheric Physics(IAP-AACM)by coupling the Model of Emissions of Gases and Aerosols from Nature(MEGAN),where the input vegetation parameters were simulated by the IAP Dynamic Global Vegetation Model(IAP-DGVM).The volatility basis set(VBS)approach was adopted to simulate SOA formation from the nontraditional pathways,i.e.,the oxidation of intermediate VOCs and aging of primary organic aerosol.Although biogenic SOAs(BSOAs)were dominant in SOAs globally in the preindustrial period,the contribution of nontraditional anthropogenic SOAs(ASOAs)to the total SOAs was up to 35.7%.In the present day,the contribution of ASOAs was 2.8 times larger than that in the preindustrial period.The contribution of nontraditional sources of SOAs to SOA was as high as 53.1%.The influence of increased anthropogenic emissions in the present day on BSOA concentrations was greater than that of increased biogenic emission changes.The response of BSOA concentrations to anthropogenic emission changes in the present day was more sensitive than that in the preindustrial period.The nontraditional sources and the atmospheric oxidation capability greatly affect the global SOA change. 展开更多
关键词 IAP-AACM VBS MEGAN secondary organic aerosol anthropogenic and biogenic emissions
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Composition optimization and performance prediction for ultra-stable water-based aerosol based on thermodynamic entropy theory
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作者 Tingting Kang Canjun Yan +6 位作者 Xinying Zhao Jingru Zhao Zixin Liu Chenggong Ju Xinyue Zhang Yun Zhang Yan Wu 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2024年第3期437-446,共10页
Water-based aerosol is widely used as an effective strategy in electro-optical countermeasure on the battlefield used to the preponderance of high efficiency,low cost and eco-friendly.Unfortunately,the stability of th... Water-based aerosol is widely used as an effective strategy in electro-optical countermeasure on the battlefield used to the preponderance of high efficiency,low cost and eco-friendly.Unfortunately,the stability of the water-based aerosol is always unsatisfactory due to the rapid evaporation and sedimentation of the aerosol droplets.Great efforts have been devoted to improve the stability of water-based aerosol by using additives with different composition and proportion.However,the lack of the criterion and principle for screening the effective additives results in excessive experimental time consumption and cost.And the stabilization time of the aerosol is still only 30 min,which could not meet the requirements of the perdurable interference.Herein,to improve the stability of water-based aerosol and optimize the complex formulation efficiently,a theoretical calculation method based on thermodynamic entropy theory is proposed.All the factors that influence the shielding effect,including polyol,stabilizer,propellant,water and cosolvent,are considered within calculation.An ultra-stable water-based aerosol with long duration over 120 min is obtained with the optimal fogging agent composition,providing enough time for fighting the electro-optic weapon.Theoretical design guideline for choosing the additives with high phase transition temperature and low phase transition enthalpy is also proposed,which greatly improves the total entropy change and reduce the absolute entropy change of the aerosol cooling process,and gives rise to an enhanced stability of the water-based aerosol.The theoretical calculation methodology contributes to an abstemious time and space for sieving the water-based aerosol with desirable performance and stability,and provides the powerful guarantee to the homeland security. 展开更多
关键词 Ultra-stable Water-based aerosol Thermodynamic entropy Composition optimization Performance prediction
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Applying the Dark Target Aerosol Algorithm to MERSI-Ⅱ:Retrieval and Validation of Aerosol Optical Depth over the Ocean
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作者 Xin PEI Leiku YANG +4 位作者 Weiqian JI Shuang CHEN Xiaoqian CHENG Xiaofeng LU Hongtao WANG 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第12期2446-2463,共18页
The Medium-Resolution Spectral Imager-Ⅱ(MERSI-Ⅱ)instrument aboard China’s Fengyun-3D satellite shares similarities with NASA’s Moderate Resolution Imaging Spectroradiometer(MODIS)sensor,enabling the retrieval of g... The Medium-Resolution Spectral Imager-Ⅱ(MERSI-Ⅱ)instrument aboard China’s Fengyun-3D satellite shares similarities with NASA’s Moderate Resolution Imaging Spectroradiometer(MODIS)sensor,enabling the retrieval of global aerosol optical depth(AOD).However,no officially released operational MERSI-Ⅱ aerosol products currently exist over the ocean.This study focuses on adapting the MODIS dark target(DT)ocean algorithm to the MERSI-Ⅱ sensor.A retrieval test is conducted on the 2019 MERSI-Ⅱ data over the global ocean,and the retrieved AODs are validated against ground-based measurements from the automatic Aerosol Robotic Network(AERONET)and the shipborne Maritime Aerosol Network(MAN).The operational MODIS DT aerosol products are also used for comparison purposes.The results show that MERSI-Ⅱ AOD granule retrievals are in good agreement with MODIS products,boasting high correlation coefficients(R)of up to 0.96 and consistent spatial distribution trends.Furthermore,the MERSI-Ⅱ retrievals perform well in comparison to AERONET and MAN measurements,with high R-values(>0.86).However,the low-value retrievals from MERSI-Ⅱ tend to be slightly overestimated compared to MODIS,despite both AODs displaying a positive bias.Notably,the monthly gridded AODs over the high latitudes of the northern and southern hemispheres suggest that MERSI-Ⅱ exhibits greater stability in space and time,effectively reducing unrealistically high-value noise in the MODIS products.These results illustrate that the MERSI-Ⅱ retrievals meet specific accuracy requirements by maintaining the algorithmic framework and most of the algorithmic assumptions,providing a crucial data supplement for aerosol studies and climate change. 展开更多
关键词 aerosol optical depth MERSI-Ⅱ MODIS dark target
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Electric field and force characteristic of dust aerosol particles on the surface of high-voltage transmission line
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作者 刘滢格 李兴财 +2 位作者 王娟 马鑫 孙文海 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第1期368-378,共11页
High-voltage transmission lines play a crucial role in facilitating the utilization of renewable energy in regions prone to desertification. The accumulation of atmospheric particles on the surface of these lines can ... High-voltage transmission lines play a crucial role in facilitating the utilization of renewable energy in regions prone to desertification. The accumulation of atmospheric particles on the surface of these lines can significantly impact corona discharge and wind-induced conductor displacement. Accurately quantifying the force exerted by particles adhering to conductor surfaces is essential for evaluating fouling conditions and making informed decisions. Therefore, this study investigates the changes in electric field intensity along branched conductors caused by various fouling layers and their resulting influence on the adhesion of dust particles. The findings indicate that as individual particle size increases, the field strength at the top of the particle gradually decreases and eventually stabilizes at approximately 49.22 k V/cm, which corresponds to a field strength approximately 1.96 times higher than that of an unpolluted transmission line. Furthermore,when particle spacing exceeds 15 times the particle size, the field strength around the transmission line gradually decreases and approaches the level observed on non-adhering surface. The electric field remains relatively stable. In a triangular arrangement of three particles, the maximum field strength at the tip of the fouling layer is approximately 1.44 times higher than that of double particles and 1.5 times higher compared to single particles. These results suggest that particles adhering to the transmission line have a greater affinity for adsorbing charged particles. Additionally, relevant numerical calculations demonstrate that in dry environments, the primary adhesion forces between particles and transmission lines follow an order of electrostatic force and van der Waals force. Specifically, at the minimum field strength, these forces are approximately74.73 times and 19.43 times stronger than the gravitational force acting on the particles. 展开更多
关键词 high-voltage current electric field aerosol particles force characteristic
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Optical Modeling of Sea Salt Aerosols Using in situ Measured Size Distributions and the Impact of Larger Size Particles
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作者 Wushao LIN Lei BI 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第10期1917-1935,共19页
Sea salt aerosols play a critical role in regulating the global climate through their interactions with solar radiation.The size distribution of these particles is crucial in determining their bulk optical properties.... Sea salt aerosols play a critical role in regulating the global climate through their interactions with solar radiation.The size distribution of these particles is crucial in determining their bulk optical properties.In this study,we analyzed in situ measured size distributions of sea salt aerosols from four field campaigns and used multi-mode lognormal size distributions to fit the data.We employed super-spheroids and coated super-spheroids to account for the particles’non-sphericity,inhomogeneity,and hysteresis effect during the deliquescence and crystallization processes.To compute the singlescattering properties of sea salt aerosols,we used the state-of-the-art invariant imbedding T-matrix method,which allows us to obtain accurate optical properties for sea salt aerosols with a maximum volume-equivalent diameter of 12μm at a wavelength of 532 nm.Our results demonstrated that the particle models developed in this study were successful in replicating both the measured depolarization and lidar ratios at various relative humidity(RH)levels.Importantly,we observed that large-size particles with diameters larger than 4μm had a substantial impact on the optical properties of sea salt aerosols,which has not been accounted for in previous studies.Specifically,excluding particles with diameters larger than 4μm led to underestimating the scattering and backscattering coefficients by 27%−38%and 43%−60%,respectively,for the ACE-Asia field campaign.Additionally,the depolarization ratios were underestimated by 0.15 within the 50%−70%RH range.These findings emphasize the necessity of considering large particle sizes for optical modeling of sea salt aerosols. 展开更多
关键词 sea salt aerosol particle size distribution LIDAR optical property
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A Deep-Learning and Transfer-Learning Hybrid Aerosol Retrieval Algorithm for FY4-AGRI:Development and Verification over Asia
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作者 Disong Fu Hongrong Shi +9 位作者 Christian AGueymard Dazhi Yang Yu Zheng Huizheng Che Xuehua Fan Xinlei Han Lin Gao Jianchun Bian Minzheng Duan Xiangao Xia 《Engineering》 SCIE EI CAS CSCD 2024年第7期164-174,共11页
The Advanced Geosynchronous Radiation Imager(AGRI)is a mission-critical instrument for the Fengyun series of satellites.AGRI acquires full-disk images every 15 min and views East Asia every 5 min through 14 spectral b... The Advanced Geosynchronous Radiation Imager(AGRI)is a mission-critical instrument for the Fengyun series of satellites.AGRI acquires full-disk images every 15 min and views East Asia every 5 min through 14 spectral bands,enabling the detection of highly variable aerosol optical depth(AOD).Quantitative retrieval of AOD has hitherto been challenging,especially over land.In this study,an AOD retrieval algorithm is proposed that combines deep learning and transfer learning.The algorithm uses core concepts from both the Dark Target(DT)and Deep Blue(DB)algorithms to select features for the machinelearning(ML)algorithm,allowing for AOD retrieval at 550 nm over both dark and bright surfaces.The algorithm consists of two steps:①A baseline deep neural network(DNN)with skip connections is developed using 10 min Advanced Himawari Imager(AHI)AODs as the target variable,and②sunphotometer AODs from 89 ground-based stations are used to fine-tune the DNN parameters.Out-of-station validation shows that the retrieved AOD attains high accuracy,characterized by a coefficient of determination(R2)of 0.70,a mean bias error(MBE)of 0.03,and a percentage of data within the expected error(EE)of 70.7%.A sensitivity study reveals that the top-of-atmosphere reflectance at 650 and 470 nm,as well as the surface reflectance at 650 nm,are the two largest sources of uncertainty impacting the retrieval.In a case study of monitoring an extreme aerosol event,the AGRI AOD is found to be able to capture the detailed temporal evolution of the event.This work demonstrates the superiority of the transfer-learning technique in satellite AOD retrievals and the applicability of the retrieved AGRI AOD in monitoring extreme pollution events. 展开更多
关键词 aerosol optical depth Retrieval algorithm Deep learning Transfer learning Advanced Geosynchronous Radiation IMAGER
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Aerosol deposition technology and its applications in batteries
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作者 Xinyu Wang Ramon Alberto Paredes Camacho +6 位作者 Xiaoyu Xu Yumei Wang Yi Qiang Hans Kungl Ruediger-AEichel Yunfeng Zhang Li Lu 《Nano Materials Science》 EI CAS CSCD 2024年第1期24-37,共14页
Aerosol deposition(AD)method is a kind of additive manufacturing technology for fabricating dense films such as metals and ceramics at room temperature.It resolves the challenge of integrating ceramic films onto tempe... Aerosol deposition(AD)method is a kind of additive manufacturing technology for fabricating dense films such as metals and ceramics at room temperature.It resolves the challenge of integrating ceramic films onto temperaturesensitive substrates,including metals,glasses,and polymers.It should be emphasized that the AD is a spray coating technology that uses powder without thermal assistance to generate films with high density.Compared to the traditional sputter-based approach,the AD shows several advantages in efficiency,convenience,better interfacial bonding and so on.Therefore,it opens some possibilities to the field of batteries,especially all-solidstate batteries(ASSBs)and draws much attention not only for research but also for large scale applications.The purpose of this work is to provide a critical review on the science and technology of AD as well as its applications in the field of batteries.The process,mechanism and effective parameters of AD,and recent developments in AD applications in the field of batteries will be systematically reviewed so that a trend for AD will be finally provided. 展开更多
关键词 aerosol deposition Room temperature impact consolidation Ceramic film All-solid-state battery Spray coating technology
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Characteristics of Antarctic aerosol composition during the Australian fires of 2019-2020
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作者 CHEN Afeng WANG Longquan +2 位作者 LIU Hongwei YUE Fange XIE Zhouqing 《Advances in Polar Science》 CSCD 2024年第4期421-437,共17页
During the 36th Chinese National Antarctic Research Expedition,aerosol samples were gathered from the Ross Sea in Antarctic to assess the climatic impact of the Australian fires that occurred in 2019-2020.The chemical... During the 36th Chinese National Antarctic Research Expedition,aerosol samples were gathered from the Ross Sea in Antarctic to assess the climatic impact of the Australian fires that occurred in 2019-2020.The chemical compositions,including levoglucosan(Lev)and its isomers,galactosan(Gan)and mannosan(Man),were analyzed.Principal component analysis helped identify the potential sources of these chemical components.By combining backward trajectories with the ratios of CLev/CMan and CMan/CGan,it was further inferred that Australia might be the potential source region for biomass burning.The radiative forcing resulting from biomass burning was evaluated using the Santa Barbara DISORT Atmospheric Radiative Transfer(SBDART)model,which revealed that black carbon emitted from biomass burning could slightly warm the atmosphere(+0.52 W·m^(-2))while causing slightly cooling at the surface(-0.73 W·m^(-2))and the top of the atmosphere(-0.22 W·m^(-2))over the Ross Sea. 展开更多
关键词 Australian fires biomass burning aerosol composition climate effect Ross Sea
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Contribution of Satellite Observations in the Optical and Microphysical Characterization of Aerosols in Burkina Faso, West Africa
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作者 Nébon Bado Serge Dimitri Bazyomo +4 位作者 Germain Wende Pouiré Ouedraogo Bruno Korgo Mamadou Simina Dramé Florent P. Kieno Sié Kam 《Atmospheric and Climate Sciences》 2024年第1期154-171,共18页
In this work, we proceed to an optical and microphysical analysis of the observations reversed by the MODIS, SeaWiFS, MISR and OMI sensors with the aim of proposing the best-adapted airborne sensor for better monitori... In this work, we proceed to an optical and microphysical analysis of the observations reversed by the MODIS, SeaWiFS, MISR and OMI sensors with the aim of proposing the best-adapted airborne sensor for better monitoring of aerosols in Burkina Faso. To this end, a comparison of AOD between satellite observations and in situ measurements at the Ouagadougou site reveals an underestimation of AERONET AOD except for OMI which overestimates them. Also, an inter-comparison done based on the linear regression line representation shows the correlation between the aerosol models incorporated in the airborne sensor inversion algorithms and the aerosol population probed. This can be seen through the correlation coefficients R which are 0.84, 0.64, 0.55 and 0.054 for MODIS, SeaWiFS, MISR and OMI respectively. Furthermore, an optical analysis of aerosols in Burkina Faso by the MODIS sensor from 2001 to 2016 indicates a large spatial and temporal variability of particles strongly dominated by desert dust. This is corroborated by the annual and seasonal cycles of the AOD at 550 nm and the Angström coefficient measured in the spectral range between 412 nm and 470 nm. A zoom on a few sites chosen according to the three climatic zones confirms the majority presence of mineral aerosols in Burkina Faso, whose maxima are observed in spring and summer. 展开更多
关键词 AERONET Airborne Sensors aerosol Optical and Microphysical Properties
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Some Features of Black Carbon Aerosols Connected with Regional Climate Over Pristine Environment
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作者 Saurabh Yadav Panuganti C.S.Devara +4 位作者 S.M.Sonbawne B.S.Murthy S.Tiwari S.Wadhwa A.Kumar 《Journal of Atmospheric Science Research》 2024年第1期1-18,共18页
The authors report the results of aethalometer black carbon(BC)aerosol measurements carried out over a rural(pristine)site,Panchgaon,Haryana State,India during the winter months of 2021-2022 and 2022-2023.They are com... The authors report the results of aethalometer black carbon(BC)aerosol measurements carried out over a rural(pristine)site,Panchgaon,Haryana State,India during the winter months of 2021-2022 and 2022-2023.They are compared with collocated and concurrent observations from the Air Quality Monitoring Station(AQMS),which provides synchronous air pollution and surface meteorological parameters.Secular variations in BC mass concentration are studied and explained with variations in local meteorological parameters.The biomass burning fire count retrievals from NASA-NOAA VIIRS satellite,and backward airmass trajectories from NOAA-ERL HYSPLIT Model analysis have also been utilized to explain the findings.They reveal that the north-west Indian region contributes maximum to the BC mass concentration over the study site during the study period.Moreover,the observed BC mass concentrations corroborate the synchronous fire count,primary and secondary pollutant concentrations.The results were found to aid the development of mitigation methods to achieve a sustainable climate system. 展开更多
关键词 Carbonaceous aerosols Dual-spot technique Temporal variations Primary and secondary pollutants Stubble burning Long-range transport Satellite products
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Establishment of a Collection and Detection Technology of Mycoplasma hyopneumoniae in Aerosol 被引量:1
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作者 华利忠 高昆 +4 位作者 武昱孜 白方方 冯志新 刘茂军 邵国青 《Agricultural Science & Technology》 CAS 2013年第7期998-1001,1031,共5页
ObjectiveThis study was to establish a simple method for collecting and detecting Mycoplasma hyopneumoniae (Mhp) in aerosol. MethodBased on the mechanisms of liquid impinger and filtration sampler, a double concentr... ObjectiveThis study was to establish a simple method for collecting and detecting Mycoplasma hyopneumoniae (Mhp) in aerosol. MethodBased on the mechanisms of liquid impinger and filtration sampler, a double concentration aerosol sampler was designed for collecting Mhp aerosol. Firstly, the collection was performed in a closed environment full of artificial aerosol of Mhp. Secondly, collection efficiency was detected by real-time PCR. Thereafter, the clinical feasibility of the designed equipment was tested by collecting aerosol samples in different pig herds. In one assay, the samples were collected at different times from one pig house challenged with Mhp. In another assay, the samples was collected from the delivery room, nursery and fattenning house of a MPS outbreak farm as well as a Mhp infection positive pig farm without obvious clinical symptoms. All the aerosol samples were then detected by real-time PCR or nested PCR. ResultThe collection efficiency of the designed bioaerosol sampler was (37.04±6.43) %, Mhp could be detected 7 d after intratracheal challenge with pneumonic lung homogenate suspension. Aerosol samples of 11 pig houses from the two Mhp positive pig farms with or without clinical symptoms all showed a positive result of PCR, the positivity rate was 100%. ConclusionA high sensitive collecting and detecting technology of aerosol was successfully established, which can be applied to clinical detection of Mhp in aerosol. 展开更多
关键词 Mycoplasma hyopneumoniae aerosol Bioaerosol sampler DETECTION
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Identification of Aerosol Types and Their Optical Properties in the North China Plain Based on Long-Term AERONET Data 被引量:4
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作者 SUN Li XIA Xiang-Ao +3 位作者 WANG Pu-Cai CHEN Hong-Bin Philippe GOLOUB ZHANG Wen-Xing 《Atmospheric and Oceanic Science Letters》 CSCD 2013年第4期216-222,共7页
Characterization of aerosols is required to reduce uncertainties in satellite retrievals of global aerosols and for modeling the effects of these aerosols on climate.Aerosols in the North China Plain(NCP) are complex,... Characterization of aerosols is required to reduce uncertainties in satellite retrievals of global aerosols and for modeling the effects of these aerosols on climate.Aerosols in the North China Plain(NCP) are complex,which provides a good opportunity to study key aerosol optical properties for various aerosol types.A cluster analysis of key optical properties obtained from Aerosol Robotic Network(AERONET) data in Beijing and Xianghe during 2001-11 was performed to identify dominant aerosol types and their associated optical properties.Five dominant aerosol types were identified.The results show that the urban/industrial aerosol of moderate absorption was dominant in the region and that this type varied little with season.Urban/industrial aerosol of weak absorption was the next most common type and mainly occurs in summer,followed by that strong aerosols occurring mainly in winter.All were predominantly fine mode particles.Mineral dust(MD) and polluted dust(PD) occurred mainly in spring,followed by winter,and their absorption decreased with wavelength.In addition,aerosol dynamics and optical parameters such as refractive index and asymmetry factor were examined.Results show that the size of coarse mode particles decreased with AOD indicating the domination of external mixing between aerosols. 展开更多
关键词 aerosol classification aerosol types aerosol optical properties
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Comments on "Direct Radiative Forcing of Anthropogenic Aerosols over Oceans from Satellite Observation" 被引量:1
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作者 Hye-Ryun OH Chang-Hoi HO Yong-Sang CHOI 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2013年第1期10-14,共5页
Previous observational studies have estimated anthropogenic aerosol direct radiative forcing over oceans without due consideration of cloudy-sky aerosols. However, when interaction between clouds and aerosols located ... Previous observational studies have estimated anthropogenic aerosol direct radiative forcing over oceans without due consideration of cloudy-sky aerosols. However, when interaction between clouds and aerosols located below or above the cloud level is taken into account, the aerosol direct radiative forcing is larger by as much as 5 W m-2 in most mid-latitude regions in the Northern Hemisphere. 展开更多
关键词 cloudy-sky aerosol forcing anthropogenic aerosol aerosol optical depth satellite observations
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Aerosol-Cloud-Precipitation Interactions in a Closed-cell and Non-homogenous MBL Stratocumulus Cloud 被引量:1
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作者 Xiaojian ZHENG Xiquan DONG +3 位作者 Dale MWARD Baike XI Peng WU Yuan WANG 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2022年第12期2107-2123,共17页
A closed-cell marine stratocumulus case during the Aerosol and Cloud Experiments in the Eastern North Atlantic(ACE-ENA)aircraft field campaign is selected to examine the heterogeneities of cloud and drizzle microphysi... A closed-cell marine stratocumulus case during the Aerosol and Cloud Experiments in the Eastern North Atlantic(ACE-ENA)aircraft field campaign is selected to examine the heterogeneities of cloud and drizzle microphysical properties and the aerosol-cloud-precipitation interactions.The spatial and vertical variabilities of cloud and drizzle microphysics are found in two different sets of flight legs:Leg-1 and Leg-2,which are parallel and perpendicular to the cloud propagation,respectively.The cloud along Leg-2 was close to adiabatic,where cloud-droplet effective radius and liquid water content linearly increase from cloud base to cloud top with less drizzle.The cloud along Leg-1 was sub-adiabatic with lower clouddroplet number concentration and larger cloud-droplet effective,but higher drizzle droplet number concentration,larger drizzle droplet median diameter and drizzle liquid water content.The heavier drizzle frequency and intensity on Leg-1 were enhanced by the collision-coalescence processes within cloud due to strong turbulence.The sub-cloud precipitation rate on Leg-1 was significantly higher than that along Leg-2.As a result,the sub-cloud accumulation mode aerosols and CCN on Leg-1 were depleted,but the coarse model aerosols increased.This further leads to a counter-intuitive phenomenon that the CCN is less than cloud-droplet number concentration for Leg-1.The average CCN loss rates are −3.89 cm^(-3)h^(-1)and −0.77 cm^(-3)h^(-1) on Leg-1 and Leg-2,respectively.The cloud and drizzle heterogeneities inside the same stratocumulus can significantly alter the sub-cloud aerosols and CCN budget.Hence it should be treated with caution in the aircraft assessment of aerosol-cloud-precipitation interactions. 展开更多
关键词 maritime aerosol cloud and drizzle properties coalescence-scavenging effect of the sub-cloud aerosol and CCN and aerosol-cloud-precipitation interactions
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Vertical Profile Comparison of Aerosol and Cloud Optical Properties in Dominated Dust and Smoke Regions over Africa Based on Space-Based Lidar
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作者 Didier Ntwali Getachew Dubache Faustin Katchele Ogou 《Atmospheric and Climate Sciences》 CAS 2022年第3期588-602,共15页
This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surf... This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surface to 10km and from 2008 to 2011 based on LIVAS (LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies). Aerosol extinction (AE), aerosol backscatter (AB), and aerosol depolarization (AD) generally increase from the surface to 1.2 km and decrease from 1.2 km to the upper layers in both WNA and CSA. AE and AB in CSA (maximum of 0.13 km<sup>-1</sup>, 0.14 km<sup>-1</sup>, 0.0021 km<sup>-1</sup>&#8231;sr<sup>-1</sup>, 0.0033 km<sup>-1</sup>&#8231;sr<sup>-1</sup>) are higher than in WNA (maximum of 0.07 km<sup>-1</sup>, 0.08 km<sup>-1</sup>, 0.0017 km<sup>-1</sup>&#8231;sr<sup>-1</sup>, 0.0015 km<sup>-1</sup>&#8231;sr<sup>-1</sup>) at 532 and 1064 nm respectively. AD in WNA (maximum of 0.25) is significantly higher than in CSA (maximum of 0.05). There is a smooth change with the height of cloud extinction and backscatter in WNA and CSA, while there is a remarkable increase of cloud depolarization with height, whereby it is high in CSA and low in WNA due to high and low fraction of cirrus respectively. Altocumulus has the highest extinction in NA (0.0139 km<sup>-1</sup>), CA (0.058 km<sup>-1</sup>), WA (0.013 km<sup>-1</sup>), while low overcast transparent (0.76 km<sup>-1</sup>) below 1 km in SA. The major findings of this study may contribute to the improvement of our understanding of aerosol-cloud interaction studies in dominated dust and smoke aerosol regions. 展开更多
关键词 Vertical Profile Dust aerosols Smoke aerosols Clouds AFRICA Lidar Climatology of Vertical aerosol Structure for Space-Based Lidar Simulation Studies (LIVAS)
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A Smog Chamber Facility for Qualitative and Quantitative Study on Atmospheric Chemistry and Secondary Organic Aerosol 被引量:5
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作者 胡长进 程跃 +9 位作者 潘刚 盖艳波 顾学军 赵卫雄 王振亚 张为俊 陈军 刘付轶 单晓斌 盛六四 《Chinese Journal of Chemical Physics》 SCIE CAS CSCD 2014年第6期631-639,I0003,共10页
In order to investigate the atmospheric oxidation processes and the formation of secondary organic aerosol (SOA), an indoor environmental reaction smog chamber are constructed and characterized. The system consists ... In order to investigate the atmospheric oxidation processes and the formation of secondary organic aerosol (SOA), an indoor environmental reaction smog chamber are constructed and characterized. The system consists of the collapsible ~830 L FEP Teflon film main reactor, in which the atmospheric chemical reactions take place and the formation of SOA occurs under the simulated atmospheric conditions, and the diverse on-line gas- and particle-phase instrumentation, such as the proton transfer reaction mass spectrometer, the synchrotron radiation photoionization mass spectrometer, the aerosol laser time-of-flight mass spectrometer, and other traditional commercial instruments. The initial characterization experiments are described, concerning the temperature and ultraviolet light intensity, the reactivity of the pure air, the wall loss rates of gaseous compounds and particulate matter. And the initial evaluation experiments for SOA yields from the ozonolysis of α-pinene and for mass spectra of the products resulting from the photooxidation of OH initiated isoprene are also presented, which indicate the applicability of this facility on the studies of gas-phase chemical mechanisms as well as the formation of SOA expected in the atmosphere. 展开更多
关键词 Smog chamber Atmospheric chemical reactions Secondary organic aerosol Mass spectrum
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Using MAN and Coastal AERONET Measurements to Assess the Suitability of MODIS C6.1 Aerosol Optical Depth for Monitoring Changes from Increased Arctic Shipping
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作者 Nicole Mölders Mariel Friberg 《Open Journal of Air Pollution》 2020年第4期77-104,共28页
Collocated data of the moderate resolution imaging spectroradiometer (MO<span style="font-family:Verdana;">-</span><span style="font-family:Verdana;">DIS) Collection 6.1 aerosol o... Collocated data of the moderate resolution imaging spectroradiometer (MO<span style="font-family:Verdana;">-</span><span style="font-family:Verdana;">DIS) Collection 6.1 aerosol optical depths (AOD) at 3 km × 3 km north of 59.9</span><span style="font-family:Verdana;">°</span><span style="font-family:Verdana;">N over ocean were assessed at 550 nm by aerosol robotic network (AERONET) data from coastal sites and marine aerosol network (MAN) data from vessels during June to October 2006 to 2018. Typically, MODIS AOD w</span><span style="font-family:Verdana;">as</span><span style="font-family:Verdana;"> higher at low and lower at high values than the AERONET AOD. Discrepancies were largest for sites where the Earth’s surface around the site is very heterogeneous (Canadian Archipelago, coast of Greenland). Due to the higher likelihood for sea-ice, MAN and MODIS AOD differed stronger west of Greenland and over the Beaufort Sea than at location in the Greenland and Norwegian Seas and Atlantic. MODIS AOD well captured the inter-seasonal variability found in the AERONET AOD data (R = 0.933). At all sites, MO</span><span style="font-family:Verdana;">-</span><span style="font-family:Verdana;">DIS and AERONET AOD agreement improved as time progressed in the shipping season, hinting at errors in sea-ice vs. open water classification. Overall 75.3% of the MODIS AOD data fell within the limits of the error envelops of the AERONET/MAN AOD data with MAN ranging between 87.5% and 100%. Changes in both MODIS and AERONET mean AOD between two periods of same length (2006-2011, 2013-2018) were explainable by changes in emissions for all sites</span><span style="font-family:Verdana;">.</span> 展开更多
关键词 aerosol Optical Depth over the Arctic Ocean MODIS Evaluation by AERONET and MAN Data Changes in Arctic aerosol Optical Depth over the Ocean North of 59.9°N Arctic Shipping Season aerosol Optical Depths
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Analysis on the Distribution Characteristics of Atmospheric Aerosol Particles in Hebei Area in the Cloudy Day Condition 被引量:3
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作者 孙玉稳 孙霞 +1 位作者 姜岩 李云川 《Meteorological and Environmental Research》 CAS 2010年第7期9-11,共3页
By using the probe data of two sorties airplane in the middle and southern parts of Hebei Province in 2007 spring,the characteristics of atmospheric aerosol particles concentration and size distribution in the area in... By using the probe data of two sorties airplane in the middle and southern parts of Hebei Province in 2007 spring,the characteristics of atmospheric aerosol particles concentration and size distribution in the area in the cloudy day situation were analyzed.The results showed that the overall trend of aerosol particles concentration in the weather systems which included the south branch trough and North China low vortex was the decrease as the height increased.However,if the cirrostratus was in the high altitude,it increased as the height increased.In the bottom of inversion layer,there existed the obvious accumulation of aerosol and cloud droplet.Affected by the complex weather systems,the aerosol particle size distribution presented the multi-peak type for the disturbance of updraft or turbulence. 展开更多
关键词 Hebei Atmospheric aerosol Particle size distribution OBSERVATION China
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