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Sustained low diffusing capacity in hepatopulmonary syndrome after liver transplantation 被引量:6
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作者 Graciela Martínez-Pallí Federico P Gómez +5 位作者 Joan A Barberà Miquel Navasa Josep Roca Robert Rodríguez-Roisin Felip Burgos Conchi Gistau 《World Journal of Gastroenterology》 SCIE CAS CSCD 2006年第36期5878-5883,共6页
AIM: To study the presence of sustained low diffusing capacity (DLco) after liver transplantation (LT) in patients with hepatopulmonary syndrome (HPS). METHODS: Six patients with mild-to-severe HPS and 24 with... AIM: To study the presence of sustained low diffusing capacity (DLco) after liver transplantation (LT) in patients with hepatopulmonary syndrome (HPS). METHODS: Six patients with mild-to-severe HPS and 24 without HPS who underwent LT were prospectively followed before and after LT at mid-term (median, 15 mo). HPS patients were also assessed at Iong-tem (median, 86 mo). RESULTS: Before LT, HPS patients showed lower PaO2 (71 ± 8 mmHg), higher AaPO2 (43 ± 10 mmHg) and lower DLco (54% ± 9% predicted), due to a combination of moderate-to-severe ventilation-perfusion (VA/Q) imbalance, mild shunt and diffusion limitation, than non- HPS patients (94 ± 4 mmHg and 19 ± 3 mmHg, and 85% ± 3% predicted, respectively) (P 〈 0.05 each). Seven non-HPS patients had also reduced DLco (70% ± 4% predicted). At mid- and long-term after LT, compared to pre- LT, HPS patients normalized PaO2 (91 ± 3 mmHg and 87 ± 5 mmHg), AaPO2 (14 ± 3 mmHg and 23 ± 5 mmHg) and all VA/Q descriptors (P 〈 0.05 each) without changes in DLco (53% ± 8% and 56% ± 7% predicted, respectively). Post-LT DLco in non-HPS patients with pre- LT low DLco was unchanged (75% ± 6% predicted). CONCLUSION: While complete VA/Q resolution in HPS indicates a reversible functional disturbance, sustained low DLco after LT also present in some non-HPS patients, points to persistence of sub-clinical liver-induced pulmonary vascular changes. 展开更多
关键词 Carbon monoxide diffusing capacity Multiple inert gas elimination technique Pulmonary gas exchange Pulmonary vascular disorders Ventilation- perfusion relationships
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A New Approach for Evaluating Rejuvenator Diffusing into Aged Bitumen 被引量:3
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作者 况栋梁 余剑英 《Journal of Wuhan University of Technology(Materials Science)》 SCIE EI CAS 2011年第1期43-46,共4页
Rejuvenator diffusing into aged bitumen was evaluated by determining penetration and chemical components of aged bitumen with rejuvenator coat before and after diffusing experiment. Effects of temperature, time and vi... Rejuvenator diffusing into aged bitumen was evaluated by determining penetration and chemical components of aged bitumen with rejuvenator coat before and after diffusing experiment. Effects of temperature, time and viscosity of rejuvenator on the diffusing ability of rejuvenator into aged bitumen were investigated. Results indicated that the diffusing ability of rejuvenator into aged bitumen could be enhanced with the increasing of temperature and time, however, the diffusing of rejuvenator into aged bitumen would be restricted due to the volatilization of light component and aging of rejuvenator under high temperature (over 170 ℃). Rejuvenator with low viscosity diffused into aged bitumen more easily. 展开更多
关键词 BITUMEN AGING rejuvenator diffusing
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Temperature and Flow Rate Control of Diffusing Chamber
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作者 Yongbo Lai Guoping Lu Zhiwei Wang 《World Journal of Engineering and Technology》 2017年第1期58-76,共19页
The temperature and flow rate control of diffusing chamber is one of the key technologies in the production of poly-crystal silicon thin film. As there exist some modeling uncertainties and errors in the actual system... The temperature and flow rate control of diffusing chamber is one of the key technologies in the production of poly-crystal silicon thin film. As there exist some modeling uncertainties and errors in the actual system, it is difficult to guarantee the chamber variable temperature conditions and the flow rate of diffusion gas being controlled within its targeted range in the rapid thermal processing (RTP). In this paper, the control applies the programmable logic controller (PLC) to configure control hardware system, proposes expert proportional integral derivative (PID) control method to regulate the gas flow rate and H∞ control strategy to attenuate chamber modeling uncertainties and disturbances, respectively, to steer the chamber rapid variable temperature very close to the expected product temperatures. Furthermore, it designs human-machine integrated user control interface (HMI) and achieves rapid and accurately control performances for user operating production. The designed control system are simulated and tested in the application, which demonstrates that the control method has strong robustness when the modeling uncertainties, errors, parameters perturbation and disturbances, the temperature and flow rate meet the requirements of precisely trajectory following. 展开更多
关键词 diffusing CHAMBER PLC HARDWARE Configuring EXPERT PID CONTROL H∞ CONTROL HMI
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Dynamics of Nano-Chain Diffusing in Porous Media
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作者 陈江星 郑强 +2 位作者 黄春云 徐江荣 应和平 《Chinese Physics Letters》 SCIE CAS CSCD 2015年第6期199-203,共5页
A coarse-grained model is proposed to study the dynamics of a nano-chain diffusing in porous media. The simulation utilizes a hybrid method which combines stochastic rotation dynamics with molecular dynamics. Solvent ... A coarse-grained model is proposed to study the dynamics of a nano-chain diffusing in porous media. The simulation utilizes a hybrid method which combines stochastic rotation dynamics with molecular dynamics. Solvent molecules are explicitly taken into account to represent the hydrodynamic interactions and random fluctuations. The conformation, relaxation, and diffusion properties of a polymer chain are investigated by changing the density degree of the obstacle matrix. It is found that the average size of the chain is a non- monotonic function of the obstacle volume faction Ф. A dense environment may contribute to extending a linear chain, which can be characterized by larger exponents in the corresponding power law. The relaxation behavior of a stretched chain to a steady state shows dramatic crossover from exponent to power-law relaxation when the values of φ are increased. The dependence of the diffusion coefficient on the chain size is also studied. Various kinds of scaling properties are presented and discussed. The results can give additional insight into the density effect of porous media on polymer structure and dynamics. 展开更多
关键词 Dynamics of Nano-Chain diffusing in Porous Media
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Computational Studies on Detecting a Diffusing Target in a Square Region by a Stationary or Moving Searcher
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作者 Hongyun Wang Hong Zhou 《American Journal of Operations Research》 2015年第2期47-68,共22页
In this paper, we compute the non-detection probability of a randomly moving target by a stationary or moving searcher in a square search region. We find that when the searcher is stationary, the decay rate of the non... In this paper, we compute the non-detection probability of a randomly moving target by a stationary or moving searcher in a square search region. We find that when the searcher is stationary, the decay rate of the non-detection probability achieves the maximum value when the searcher is fixed at the center of the square search region;when both the searcher and the target diffuse with significant diffusion coefficients, the decay rate of the non-detection probability only depends on the sum of the diffusion coefficients of the target and searcher. When the searcher moves along prescribed deterministic tracks, our study shows that the fastest decay of the non-detection probability is achieved when the searcher scans horizontally and vertically. 展开更多
关键词 diffusing TARGET Non-Detection PROBABILITY SEARCH Theory Optimal SEARCH Path
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A diffusion model for solute atoms diffusing and aggregating in nuclear structural materials
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作者 宋泉 孟繁新 +2 位作者 宁博元 庄军 宁西京 《Chinese Physics B》 SCIE EI CAS CSCD 2017年第12期432-438,共7页
In nuclear structural materials, the nuclear irradiations induce the precipitations of soluble elements or produce the insoluble elements such as He atoms that may form clusters, heavily shortening the service life-ti... In nuclear structural materials, the nuclear irradiations induce the precipitations of soluble elements or produce the insoluble elements such as He atoms that may form clusters, heavily shortening the service life-times of the materials. In the present work, a diffusion model is developed to predict where and how fast the solute atoms (either soluble or insoluble) aggregate, and this model is applied to the study of the formation and growth of He bubbles in metal tritides (PdT0.6, ErT2, NbT0.0225, VT0.5, TaT0.097, TiT1.5, ZrT1.6) within one thousand days. The results are in good agreement with the available experimental observations and suggest that searching for metals with a barrier of more than 1.1 eV for a single He atom diffusion and making more defects in metal tritides can significantly reduce the growth of He bubbles and extend the service time of the metals. 展开更多
关键词 atomistic modeling diffusion growth metal tritides nucleation and growth helium bubble
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Absorption Rate into a Small Sphere for a Diffusing Particle Confined in a Large Sphere
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作者 Hongyun Wang Hong Zhou 《Applied Mathematics》 2016年第7期709-720,共12页
We study the problem of a diffusing particle confined in a large sphere in the n-dimensional space being absorbed into a small sphere at the center. We first non-dimensionalize the problem using the radius of large co... We study the problem of a diffusing particle confined in a large sphere in the n-dimensional space being absorbed into a small sphere at the center. We first non-dimensionalize the problem using the radius of large confining sphere as the spatial scale and the square of the spatial scale divided by the diffusion coefficient as the time scale. The non-dimensional normalized absorption rate is the product of the physical absorption rate and the time scale. We derive asymptotic expansions for the normalized absorption rate using the inverse iteration method. The small parameter in the asymptotic expansions is the ratio of the small sphere radius to the large sphere radius. In particular, we observe that, to the leading order, the normalized absorption rate is proportional to the (n - 2)-th power of the small parameter for . 展开更多
关键词 Diffusion Equation Brownian Diffusion Asymptotic Solutions Absorption Rate
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Performance Analysis of Optical Wireless Communication System Employing Neuro-Fuzzy Based Spot-Diffusing Techniques
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作者 Shamim Al Mamun M. Shamim Kaiser +2 位作者 Muhammad R Ahmed Md. Shafiqul Islam Md. Imdadul Islam 《Communications and Network》 2013年第3期260-265,共6页
The spot-diffusing technique provides better performance compared to conventional diffuse system for indoor optical-wireless communication (OWC) system. In this paper, the performance of an OW spot-diffusing communica... The spot-diffusing technique provides better performance compared to conventional diffuse system for indoor optical-wireless communication (OWC) system. In this paper, the performance of an OW spot-diffusing communication system using Neuro-Fuzzy (NF) adaptive multi-beam transmitter configuration has been proposed. The multi-beam transmitter generates multiple spots pointed in different directions, hence, forming a matrix of diffusing spots based on position of the receiver and receiver mobility. Regardless of the position of the transmitter and receiver, NF controller target the spots adaptively at the best locations and allocates optimal power to the spots and beam angle are adapted in order to achieve better signal-to-noise plus interference ratio (SNIR). Maximum ratio combining (MRC) is used in the imaging receiver. The proposed OW spot-diffusing communication system is compared with other spot-beam diffusion methods proposed in literature. Performance evaluation revels that the proposed NF based OW spot-diffusing communication system outperforms other spot-beam diffusion methods. 展开更多
关键词 Optical-wireless Communication SPOT Diffusion Technique NEURO-FUZZY Imaging RECEIVER Adaptive Power ALLOCATION
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GAN与Diffusion在传统纹样设计中的实验研究
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作者 李莉 毛子晗 +2 位作者 吕思奇 袁晨旭 彭玉旭 《丝绸》 CAS CSCD 北大核心 2024年第8期9-22,共14页
传统纹样是中国优秀传统文化的重要组成部分,传统人工设计已经无法满足纹样的现代设计需求,生成式AI为传统纹样设计提供了新的设计路径和方法。文章将生成式AI应用于传统纹样设计中,通过适配实验优选基于GAN的Style GAN和基于Diffusion... 传统纹样是中国优秀传统文化的重要组成部分,传统人工设计已经无法满足纹样的现代设计需求,生成式AI为传统纹样设计提供了新的设计路径和方法。文章将生成式AI应用于传统纹样设计中,通过适配实验优选基于GAN的Style GAN和基于Diffusion的Stable Diffusion两种主流图像生成模型进行实验,采用技术分析与艺术分析相结合,对实验结果进行多角度、多维度对比分析,为设计师选择生成设计方法提供参照。实验结果表明,两个模型均能满足基本的艺术设计需求。Style GAN模型生成的纹样图像更接近真实图像的分布,具有更高的图像质量和多样性;Stable Diffusion模型能较好地传承传统纹样的基因,艺术性与创造性兼具,更加符合传统纹样的艺术设计需求。 展开更多
关键词 GAN DIFFUSION 传统纹样 评价指标 对比分析 实验研究
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ControlNet插件在AI生成图像中的控制应用分析 被引量:1
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作者 温逸娴 《影视制作》 2024年第2期57-62,共6页
运用AI绘图工具Stable Diffusion生成图像的过程中,虽然可以用提示词来描述画面,但生成图像的不确定性很大。为了生成满意的图像,可以使用Stable Diffusion的插件ControlNet对图像生成进行控制。本文分析了用ControlNet对图像生成过程... 运用AI绘图工具Stable Diffusion生成图像的过程中,虽然可以用提示词来描述画面,但生成图像的不确定性很大。为了生成满意的图像,可以使用Stable Diffusion的插件ControlNet对图像生成进行控制。本文分析了用ControlNet对图像生成过程的控制方法,并运用该方法在具体案例中实现了在生成图像过程中对画面构图的控制。 展开更多
关键词 AIGC AI绘画 Stable Diffusion CONTROLNET 人工智能
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基于AI图像生成技术的家具设计研究
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作者 邹志娟 陈思洁 《林产工业》 北大核心 2024年第11期62-67,共6页
简述了AI图像生成技术及其在家具设计中的应用优势,提出AI图像生成技术在家具设计中的一般流程。基于Stable Diffusion AI设计平台,依据“文本指令”进行家具设计尝试,以包豪斯风格家具设计实践来验证AI图像生成技术辅助生成家具设计效... 简述了AI图像生成技术及其在家具设计中的应用优势,提出AI图像生成技术在家具设计中的一般流程。基于Stable Diffusion AI设计平台,依据“文本指令”进行家具设计尝试,以包豪斯风格家具设计实践来验证AI图像生成技术辅助生成家具设计效果图的高效性。研究表明:AI图像生成技术能合理运用于家具设计创意阶段,对缩短家具设计周期、提升家具设计质量具有实际意义。 展开更多
关键词 AI图像生成技术 Stable diffusion 文本指令 家具设计 机器学习
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从特征辨识到图像生成:基于AIGC范式的苗族服饰设计 被引量:9
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作者 于鹏 张毅 《丝绸》 CAS CSCD 北大核心 2024年第3期1-10,共10页
苗族服饰是中国民族服饰体系中重要的组成部分,在商品化发展中开辟了广阔的市场,但产品同质化现象将阻碍民族文化的进一步发展,人工智能生成内容(AIGC)的发展为传统服饰设计提供了新的可能。文章基于苗族服饰现代化的需要,通过搭建多模... 苗族服饰是中国民族服饰体系中重要的组成部分,在商品化发展中开辟了广阔的市场,但产品同质化现象将阻碍民族文化的进一步发展,人工智能生成内容(AIGC)的发展为传统服饰设计提供了新的可能。文章基于苗族服饰现代化的需要,通过搭建多模型组合流程,为苗族服饰成衣化设计提供灵感样本。实验结果表明,以服饰辨识性为基础,采用Lora训练方式,仅需少量样本即可实现苗族服饰特征在Stable Diffusion生成内容中的迁移。将深度学习引入非遗服饰现代化的进程中,旨在助力非遗服饰朝着成衣化、多样化、大众化方向发展,以数字化方式推动民族服饰转型升级。 展开更多
关键词 AIGC 苗族 非遗服饰 少样本风格迁移 Stable Diffusion Lora 辅助设计
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AIGC视野下的浙北民居风格研究路径初探 被引量:1
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作者 陆激 沈东山 《建筑与文化》 2024年第2期2-9,共8页
文章以Stable Diffusion为工具,以通过机器学习特定建筑风格图像并输出结果的方式,尝试对浙北民居的建筑风格在AIGC视野下的研究路径进行探索。文章建立了浙北民居与现代住宅图像的数据集并进行训练,得到该语境下的浙北民居风格模型,接... 文章以Stable Diffusion为工具,以通过机器学习特定建筑风格图像并输出结果的方式,尝试对浙北民居的建筑风格在AIGC视野下的研究路径进行探索。文章建立了浙北民居与现代住宅图像的数据集并进行训练,得到该语境下的浙北民居风格模型,接着通过批量单独生成与混合生成,对生成的结果进行分类统计。最终发现了该模型在建筑风格模拟方面具有不同于人类直觉判断的抽象提取能力,进而概括了该类工具下生成结果的可能性与局限性。 展开更多
关键词 AIGC Stable Diffusion 机器学习 浙北民居 建筑风格
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基于美学梯度法的人工智能风格化绘画系统 被引量:1
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作者 钟梓锐 梁玲琳 《浙江理工大学学报(自然科学版)》 2024年第4期537-547,共11页
当前Stable diffusion等人工智能绘画模型在绘画时难以直接控制图像风格,同时风格模型训练仅针对单种风格。针对该问题,提出了一种基于美学梯度法的人工智能风格化绘画系统,以实现多种图像风格的控制和融合,并提供更加便捷的图像创作体... 当前Stable diffusion等人工智能绘画模型在绘画时难以直接控制图像风格,同时风格模型训练仅针对单种风格。针对该问题,提出了一种基于美学梯度法的人工智能风格化绘画系统,以实现多种图像风格的控制和融合,并提供更加便捷的图像创作体验。收集并分析网络用户数据,结合问卷得到用户对图像风格的感性需求;根据感性需求收集各风格图像数据得到对应的风格图像训练集。使用梯度下降算法计算风格化文本编码器的权重,实现生成图像风格化的效果。通过可用性测试对比用户对该系统与传统人工智能绘画系统产出图像的风格满意程度,结果表明:人工智能风格化绘画系统的平均满意度相较传统人工智能绘画系统提升23%,表明人工智能风格化绘画系统在图像风格生成上具有更好的效果,可满足用户对图像风格的需求。该人工智能风格化绘画系统可以更便捷地实现图像风格调整,允许用户直观选择不同风格的权重,便捷使用一种或多种风格,能够有效满足用户对图像风格设计的需求。 展开更多
关键词 人工智能绘画模型 Stable diffusion 美学梯度法 感性需求 风格化
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文生图扩散模型技术在病理学教学中的应用
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作者 陈张一 朱朝阳 +1 位作者 危晓莉 彭慧琴 《基础医学教育》 2024年第11期980-985,共6页
目前,病理教学中切片图像需要经过取材、固定、脱水透明、浸蜡、包埋、切片、染色和封片等步骤,操作复杂且容易质量不高,较为短缺。为解决这一问题,应用文生图技术制作数字病理切片图像。文生图技术是AIGC的一个重要分支,通过CLIP技术... 目前,病理教学中切片图像需要经过取材、固定、脱水透明、浸蜡、包埋、切片、染色和封片等步骤,操作复杂且容易质量不高,较为短缺。为解决这一问题,应用文生图技术制作数字病理切片图像。文生图技术是AIGC的一个重要分支,通过CLIP技术将提示词与病理图像进行关联,并运用Stable Diffusion模型自动随机生成病理切片图像,并有效提高生成图像速度,减少图像学习时间。通过算例分析,应用SD1.5预训练模型的微调技术可以有效提高病理切片图像质量和生成速度,生成的图库已能应用于学生的读片训练和随堂测试。 展开更多
关键词 病理学 病理切片 教学改革 文生图 图像学习 Stable Diffusion模型
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基于Stable Diffusion的虚拟人形象预设计的应用与研究 被引量:2
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作者 曾建勇 沈晓萍 《现代信息科技》 2024年第3期169-175,共7页
对当前AIGC在虚拟形象预设计方面的现状及影响进行了分析和探讨。以Stable Diffusion为例,详细介绍了工程构建和实现,对相关模块的作用、运行环境、使用方法及其指令等多个方面进行了综合叙述、分析和探讨,针对使用不同采样方法、不同... 对当前AIGC在虚拟形象预设计方面的现状及影响进行了分析和探讨。以Stable Diffusion为例,详细介绍了工程构建和实现,对相关模块的作用、运行环境、使用方法及其指令等多个方面进行了综合叙述、分析和探讨,针对使用不同采样方法、不同采样参数及不同训练模型生成图片效果的优劣进行了说明及展示。随后,通过项目实例,完整地展示了人物形象预设计的过程。最后,对AIGC等新技术可能带来的社会影响进行了预测和总结。 展开更多
关键词 AI生成内容 Stable Diffusion 生成对抗网络 提示词 虚拟人形象
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A rened analytical model for reconstruction problems in diuse reectance spectroscopy 被引量:1
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作者 Ekaterina Sergeeva Daria Kurakina Ilya Turchin and Mikhail Kirillin 《Journal of Innovative Optical Health Sciences》 SCIE EI CSCD 2024年第5期33-51,共19页
A rened analytical model of spatially resolved diffuse reectance with small source-detector separations(SDSs)for the in vivo skin studies is proposed.Compared to the conventional model developed by Farrell et al.,it a... A rened analytical model of spatially resolved diffuse reectance with small source-detector separations(SDSs)for the in vivo skin studies is proposed.Compared to the conventional model developed by Farrell et al.,it accounts for the limited acceptance angle of the detectorber.The rened model is validated in the wide range of optical parameters by Monte Carlo simulations of skin diffuse reectance at SDSs of units of mm.Cases of uniform dermis and two-layered epidermis-dermis structures are studied.Higher accuracy of the rened model compared to the conventional one is demonstrated in the separate,constraint-free reconstruction of absorption and reduced scattering spectra of uniform dermis from the Monte Carlo simulated data.In the case of epidermis-dermis geometry,the recovered values of reduced scattering in dermis are overestimated and the recovered values of absorption are underestimated for both analytical models.Presumably,in the presence of a thin mismatched topical layer,only the effective attenuation coe±cient of the bottom layer can be accurately recovered using a diffusion theorybased analytical model while separate reconstruction of absorption and reduced scattering fails due to the inapplicability of the method of images.These-ndings require implementation of more sophisticated models of light transfer in inhomogeneous media in the recovery algorithms. 展开更多
关键词 Diffuse reffectance spectroscopy in vivo skin studies optical properties reconstruction diffuse approximation Monte Carlo simulations method of images
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Diffusion and reaction mechanism of limestone and quartz in fluxed iron ore pellet roasting process 被引量:1
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作者 Yufeng Guo Jinlai Zhang +5 位作者 Shuai Wang Jianjun Fan Haokun Li Feng Chen Kuo Liu Lingzhi Yang 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS CSCD 2024年第3期485-497,共13页
The increase to the proportion of fluxed pellets in the blast furnace burden is a useful way to reduce the carbon emissions in the ironmaking process.In this study,the interaction between calcium carbonate and iron or... The increase to the proportion of fluxed pellets in the blast furnace burden is a useful way to reduce the carbon emissions in the ironmaking process.In this study,the interaction between calcium carbonate and iron ore powder and the mineralization mechanism of fluxed iron ore pellet in the roasting process were investigated through diffusion couple experiments.Scanning electron microscopy with energy dispersive spectroscopy was used to study the elements’diffusion and phase transformation during the roasting process.The results indicated that limestone decomposed into calcium oxide,and magnetite was oxidized to hematite at the early stage of preheating.With the increase in roasting temperature,the diffusion rate of Fe and Ca was obviously accelerated,while the diffusion rate of Si was relatively slow.The order of magnitude of interdiffusion coefficient of Fe_(2)O_(3)-CaO diffusion couple was 10^(−10) m^(2)·s^(−1) at a roasting temperature of 1200℃for 9 h.Ca_(2)Fe_(2)O_(5) was the initial product in the Fe_(2)O_(3)-CaO-SiO_(2) diffusion interface,and then Ca_(2)Fe_(2)O_(5) continued to react with Fe_(2)O_(3) to form CaFe_(2)O_(4).With the expansion of the diffusion region,the sillico-ferrite of calcium liquid phase was produced due to the melting of SiO_(2) into CaFe_(2)O_(4),which can strengthen the consolidation of fluxed pellets.Furthermore,andradite would be formed around a small part of quartz particles,which is also conducive to the consolidation of fluxed pellets.In addition,the principle diagram of limestone and quartz diffusion reaction in the process of fluxed pellet roasting was discussed. 展开更多
关键词 fluxed iron ore pellet LIMESTONE HEMATITE QUARTZ diffusion reaction
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Simulation of the Ecosystem Productivity Responses to Aerosol Diffuse Radiation Fertilization Effects over the Pan-Arctic during 2001–19 被引量:1
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作者 Zhiding ZHANG Xu YUE +3 位作者 Hao ZHOU Jun ZHU Yadong LEI Chenguang TIAN 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2024年第1期84-96,共13页
The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).Whil... The pan-Arctic is confronted with air pollution transported from lower latitudes.Observations have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).While such DRFEs have been explored at low to middle latitudes,the aerosol impacts on pan-Arctic ecosystems and the contributions by anthropogenic and natural emission sources remain less quantified.Here,we perform regional simulations at 0.2o×0.2ousing a well-validated vegetation model(Yale Interactive terrestrial Biosphere,YIBs)in combination with multi-source of observations to quantify the impacts of aerosol DRFEs on the net primary productivity(NPP)in the pan-Arctic during 2001-19.Results show that aerosol DRFEs increase pan-Arctic NPP by 2.19 Pg C(12.8%)yr^(-1)under clear-sky conditions,in which natural and anthropogenic sources contribute to 8.9% and 3.9%,respectively.Under all-sky conditions,such DRFEs are largely dampened by cloud to only 0.26 Pg C(1.24%)yr^(-1),with contributions of 0.65% by natural and 0.59% by anthropogenic species.Natural aerosols cause a positive NPP trend of 0.022% yr^(-1)following the increased fire activities in the pan-Arctic.In contrast,anthropogenic aerosols induce a negative trend of-0.01% yr^(-1)due to reduced emissions from the middle latitudes.Such trends in aerosol DRFEs show a turning point in the year of 2007 with more positive NPP trends by natural aerosols but negative NPP trends by anthropogenic aerosols thereafter.Though affected by modeling uncertainties,this study suggests a likely increasing impact of aerosols on terrestrial ecosystems in the pan-Arctic under global warming. 展开更多
关键词 diffuse radiation fertilization effects anthropogenic aerosols natural aerosols pan-Arctic net primary productivity
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Boron-doped high-entropy oxide toward high-rate and long-cycle layered cathodes for wide-temperature sodium-ion batteries 被引量:1
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作者 Yuzhen Dang Zhe Xu +8 位作者 Yurong Wu Runguo Zheng Zhiyuan Wang Xiaopin Lin Yanguo Liu Zheng-Yao Li Kai Sun Dongfeng Chen Dan Wang 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第8期577-587,I0012,共12页
03-type layered metal oxides hold great promise for sodium-ion batteries cathodes owing to their energy density advantage.However,the severe irreversible phase transition and sluggish Na^(+)diffusion kinetics pose sig... 03-type layered metal oxides hold great promise for sodium-ion batteries cathodes owing to their energy density advantage.However,the severe irreversible phase transition and sluggish Na^(+)diffusion kinetics pose significant challenges to achieve high-performance layered cathodes.Herein,a boron-doped03-type high entropy oxide Na(Fe_(0.2)Co_(0.15)Cu_(0.05)Ni_(0.2)Mn_(0.2)Ti_(0.2))B_(0.02)O_(2)(NFCCNMT-B_(0.02))is designed and the covalent B-O bonds with high entropy configuration ensure a robust layered structure.The obtained cathode NFCCNMT-B_(0.02)exhibits impressive cycling performance(capacity retention of 95%and 82%after100 cycles and 300 cycles at 1 and 10 C,respectively)and outstanding rate capability(capacity of 83 mAh g^(-1)at 10 C).Furthermore,the NFCCNMT-B_(0.02)demonstrates a superior wide-temperature performance,maintaining the same capacity level(113,4 mAh g^(-1)@-20℃,121 mAh g^(-1)@25℃,and 119 mAh g^(-1)@60℃)and superior cycle stability(90%capacity retention after 100 cycles at 1 C at-20℃).The high-entropy configuration design with boron doping strategy contributes to the excellent sodium-ion storage performance.The high-entropy configuration design effectively suppresses irreversible phase transitions accompanied by small volume changes(ΔV=0.65 A3).B ions doping expands the Na layer distance and enlarges the P3 phase region,thereby enhancing Na^(+)diffusion kinetics.This work offers valuable insights into design of high-performance layered cathodes for sodium-ion batteries operating across a wide temperature. 展开更多
关键词 High entropy oxide Born substitution Phase transition Na~+diffusion kinetics Sodium-ion batteries
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