The target of achieving high energy efficiency standard in order to comply with the EU Directives is leading to remarkable efforts to improve the performance of the building envelope. Excellent thermal insulation and ...The target of achieving high energy efficiency standard in order to comply with the EU Directives is leading to remarkable efforts to improve the performance of the building envelope. Excellent thermal insulation and airtight sealing of leakages are of the utmost importance to fulfil the expected targets. Unfortunately, airtightness produces the negative effect of increasing the indoor concentration of air pollutants like radon. Despite the seriousness of the problem is generally misconceived, long-term exposition to radon is acknowledged to be the second cause of lung cancer after smoke. The paper outlines the implications for the building sector and focuses on design and preventive criteria as well as on mitigation and remedial techniques.展开更多
As gradual improvement of living environment and indoor decoration form diversification, the indoor air pollution has become the "invisi- ble killer" harming human health, and has been listed as one of ten big threa...As gradual improvement of living environment and indoor decoration form diversification, the indoor air pollution has become the "invisi- ble killer" harming human health, and has been listed as one of ten big threats to human health by the World Health Organization, which also be- came one of hot issues concerned by countries all over the world. In this paper, through the determination of formaldehyde in some houses of Binzhou, the release of formaldehyde with the increase of time was explored; change of formaldehyde in the same residence in different functional areas was analyzed; the influence of the temperature, humidity and plant to formaldehyde content was also analyzed.展开更多
Objective The study was designed to compare the combustion products of coal gas, liquefied petroleum gas and natural gas in relation to indoor air pollution. Methods Regular pollutants including B(a)P were monitored a...Objective The study was designed to compare the combustion products of coal gas, liquefied petroleum gas and natural gas in relation to indoor air pollution. Methods Regular pollutants including B(a)P were monitored and 1-hydroxy pyrene were tested in urine of the enrolled subjects. Radon concentrations and their changes in four seasons were also monitored in the city natural gas from its source plant and transfer stations to final users. To analyze organic components of coal gas, liquefied petroleum gas and natural gas, a high-flow sampling device specially designed was used to collect their combustion products, and semi-volatile organic compounds contained in the particles were detected by gas chromatograph-mass spectrograph (GC/MS). Results Findings in the study showed that the regular indoor air pollutants particles and CO were all above the standard in winter when heating facilities were operated in the city, but they were lowest in kitchens using natural gas; furthermore, although NO2 and CO2 were slightly higher in natural gas, B(a)P concentration was lower in this group and 1-hydroxy pyrene was lowest in urine of the subjects exposed to natural gas. Organic compounds were more complicated in coal gas and liquefied petroleum gas than in natural gas. The concentration of radon in natural gas accounted for less than 1‰ of its effective dose contributing to indoor air pollution in Beijing households. Conclusion Compared to traditional fuels, gases are deemed as clean ones, and natural gas is shown to be cleaner than the other two gases.展开更多
To establish the model of indoor air pollution forecast for decoration. Methods The model was based on the balance model for diffusing mass. Results The data between testing concentration and estimating concentration ...To establish the model of indoor air pollution forecast for decoration. Methods The model was based on the balance model for diffusing mass. Results The data between testing concentration and estimating concentration were compared. The maximal error was less than 30% and average error was 14.6%. Conclusion The model can easily predict whether the pollution for decoration exceeds the standard and how long the room is decorated.展开更多
Three representative types of houses in Beijing were selected and, in each type, smoking and nonsmoking households were compared. IP, RP. and CO concentrations in the living room and kitchen were monitored during each...Three representative types of houses in Beijing were selected and, in each type, smoking and nonsmoking households were compared. IP, RP. and CO concentrations in the living room and kitchen were monitored during each season. and the level of COHb in the heads of the households were measured. The study showed that indoor air pollution was rather severe, especially during winter. when paniculate concentrations markedly exceeded the standard and CO concentration was as high as 47 ppm. Indoor air pollution was closely related to the type of house, particularly to the mode of heating. In houses. of the same type, pollution improved greatly after central heating facilities were installed. Analysis of 30 elements revealed that pollution was typically caused by coal burning. aggravated by dusty wind, but high indoor Pb levels were probably due to the use of LPG for cooking. In our study the effect of cigarette smoking was sometimes masked by the severe indoor pollution. (C)1990 Academic Press, Inc.展开更多
Individuals spend 90% of their time indoors, primarily at home or at work. Indoor environmental factors have a significant impact on human well-being. It was a longitudinal study that assessed the major factors that r...Individuals spend 90% of their time indoors, primarily at home or at work. Indoor environmental factors have a significant impact on human well-being. It was a longitudinal study that assessed the major factors that reduce indoor air quality, namely particulate matter, and bio-aerosols, using low-cost sensors and the settle plate method, respectively also to determine the effect of atmospheric parameters and land use patterns in households of commercial, industrial, residential, slum, and rural areas of the city. PM2.5 concentration levels were similar in most parts of the day across all sites. PM10.0 concentration levels increased indoors in a commercial area. PM2.5 concentration showed a negative correlation with temperature and a positive correlation with relative humidity in some areas. Very high values of PM2.5 concentration and PM10.0 concentration have been observed in this study, inside households of selected rural and urban areas. Pathogenic gram-positive cocci, gram-positive rods, Aspergillus, and Mucor species were the most common bacterial and fungal species respectively found inside households. This study examined particulate matter concentration along with bio-aerosols, as very less studies have been conducted in Jaipur the capital of Rajasthan, a state in the western part of India which assessed both of these factors together to determine the indoor air quality. Rural households surrounding the periphery of the city were found to have similar pollution levels as urban households. So, this study may form the basis for reducing pollution inside households and also for taking suitable measures for the reduction of pollution in the indoor environment.展开更多
Indoor air pollution in buildings puts people at risk of developing respiratory and cardiovascular diseases.Particulate matter(PM)exposure is known to cause these health issues.Preliminary efforts were made in this st...Indoor air pollution in buildings puts people at risk of developing respiratory and cardiovascular diseases.Particulate matter(PM)exposure is known to cause these health issues.Preliminary efforts were made in this study to assess the quantity and quality of PM1.0,PM_(2.5),and PM_(10)present in an abattoir and a residential building in northern Nigeria.Canree A1 low-cost sensor was used to monitor the locations,8 hourly for two weeks.The results showed that the average values(μg/m^(3))of PM1.0,PM_(2.5),and PM_(10)in an abattoir were 62.74,161.94,and 199.08,respectively,and in a residential building were 28.70,83.31,and 103.71.The average Air Quality Index(AQI)of the abattoir office was Very Unhealthy,while the living room of the residential building was unhealthy.The PM_(2.5),and PM_(10)levels were higher than the international(WHO)and national(FMEnv)standard limits,indicating a potential danger to building occupants.It is expected that the indoor environment of the locations will be improved by the use of good ventilators(adequate windows and doors)and the provision of good extractors.展开更多
Objective Evidence on potential cardiovascular benefits of personal-level intervention among the elderly exposed to high levels of particulate matter(PM)remains limited.We aimed to assess improvements in surrogate mar...Objective Evidence on potential cardiovascular benefits of personal-level intervention among the elderly exposed to high levels of particulate matter(PM)remains limited.We aimed to assess improvements in surrogate markers of cardiovascular injury in vulnerable populations at risks by using indoor air filtration units.Methods We conducted a randomized crossover trial for 2 separate 2-week air filtration interventions in 20 households of patients with stable chronic obstructive pulmonary disease and their partners in the winter of 2013,with concurrent measurements of indoor PM.The changes in biomarkers indicative of cardiac injury,atherosclerosis progression and systemic inflammation following intervention were evaluated using linear mixed-effect models.Results In the analysis,average levels of indoor PM with aerodynamic diameters<2.5µm(PM2.5)decreased significantly by 59.2%(from 59.6 to 24.3µg/m3,P<0.001)during the active air filtration.The reduction was accompanied by improvements in levels of high-sensitivity cardiac troponin I by−84.6%(95%confidence interval[CI]:−90.7 to−78.6),growth differentiation factor-15 by−48.1%(95%CI:−31.2 to−25.6),osteoprotegerin by−65.4%(95%CI:−56.5 to−18.7),interleukin-4 by−46.6%(95%CI:−62.3 to−31.0)and myeloperoxidase by−60.3%(95%CI:−83.7 to−3.0),respectively.Conclusion Indoor air filtration intervention may provide potential cardiovascular benefits in vulnerable populations at risks.展开更多
Exposure to CO (carbon monoxide) during cooking in households using LPG (liquefied petroleum gas), natural gas and charcoal as fuels has been conducted. The study aimed at assessing the indoor air quality in order...Exposure to CO (carbon monoxide) during cooking in households using LPG (liquefied petroleum gas), natural gas and charcoal as fuels has been conducted. The study aimed at assessing the indoor air quality in order to address potential hazards associated with CO. Carbon monoxide concentrations and flame temperature were measured at an interval of 1 min for 1 h using CO and thermometer data loggers respectively. While the CO concentration from LPG and natural gas were found below 26 ppm for 1 h, as recommended by WHO (World Health Organization) standards, the average CO concentration from charcoal exceeded the standard limit. In addition closing the kitchen door during cooking increased the CO concentration from 26-295 ppm to 92-597 ppm. According to WHO, the observed CO concentrations from charcoal stove highlights questionable life support atmosphere. It can therefore be suggested that switching to LPG or natural gas from charcoal will reduce CO exposure to persons during cooking.展开更多
Domestic burning emits large amounts of pollutants into the ambient air due to incomplete and inefficient combustion, with significant impacts on indoor air quality and human health. Northeast China is one of the majo...Domestic burning emits large amounts of pollutants into the ambient air due to incomplete and inefficient combustion, with significant impacts on indoor air quality and human health. Northeast China is one of the major contributors to domestic burning emissions in China;however, the high-resolution emissions inventories of domestic biomass and coal burning in Northeast China are lacked, which are needed to estimate the extent of its impact. In this study, we established a town-level emissions inventory of gaseous pollutants and particulate matter(PM) from domestic biomass and coal burning, based on per household consumption in each town in rural region of Northeast China. The results revealed that biomass burning was the major domestic burning source over the region in 2016. Domestic biomass burning is the major contributor to PM and volatile organic compounds(VOCs) emissions, while coal burning is the major contributor to SO2 emissions. High emissions intensities were concentrated around the cities of Harbin, Suihua, Changchun, Qiqihar, and Chifeng, each with emissions intensity for PM2.5 and VOCs of more than 2000 Mg per 27 km × 27 km grid cell. Additionally, there are three burning peaks(6-7 am, 12 pm and 4-7 pm) during both the heating(from October to April) and non-heating seasons(from May to September), due to cooking and heating. The burning peaks in the non-heating season were more notable than those in the heating season. These results suggest that the government should pay more attention to domestic biomass and coal burning in rural areas, in order to reduce pollutant emissions and control regional haze during the heating season.展开更多
Because incomplete confirmation is available concerning the influential role of atmosphere contamination on conjunctivitis,myopia,asthma,and allergic rhinitis in Brazil,the focus of the present work is to explore the ...Because incomplete confirmation is available concerning the influential role of atmosphere contamination on conjunctivitis,myopia,asthma,and allergic rhinitis in Brazil,the focus of the present work is to explore the possible relations among atmosphere contamination and eye problems.Rather that a case study on eye diseases,by way of questionnaires supplemented by the investigation of nanoparticles(NPs)on eyeglasses,the study examines the mechanisms in which NPs and ultra-fine particles are deposited on the glasses of children up to 10 years of age in urban and rural area.The important connection between atmosphere contaminants and individual protection equipment justifies improving indoor school properties in order could protect children’s eyes,particularly in high-pollution/high-particulate areas.展开更多
The concentrations of phthalate esters(PAEs) in Chinese hospitals were investigated by simultaneously determining concentrations of gas- and particle-phase PAEs. PAEs were detected in two third-class first-grade hos...The concentrations of phthalate esters(PAEs) in Chinese hospitals were investigated by simultaneously determining concentrations of gas- and particle-phase PAEs. PAEs were detected in two third-class first-grade hospitals, two second-class first-grade hospitals, and a community health service center. Hospital drugstores had the highest concentration(24.19 μg/m3), which was 1.54 times that of newly decorated houses. The second highest concentration was found in the transfusion rooms, averaging 21.89 μg/m3; this was followed by the concentrations of PAEs in the nurse's workstations, the wards, and the doctor's offices, with mean concentrations of 20.66, 20.0, and 16.92 μg/m3, respectively. The lowest concentrations were found in the hallways(16.30 μg/m3). Of the six different kinds of PAEs found, major pollutants included diethyl phthalates, dibutyl phthalates, butylbenzyl phthalates and di(2-ethylhexyl) phthalates, comprising more than 80% of all PAEs present.Meanwhile, a comparison between different wards showed that PAE concentrations in the maternity wards were 1.63 times higher than in the main wards. Based on known health hazards, our results suggest that the PAEs seriously influence the health of the pregnant women and babies; therefore, it is of great importance to take the phthalate concentrations in hospitals into consideration. In addition, hospital indoor air was more seriously contaminated than the air of newly decorated houses.展开更多
Chinese cooking features several unique processes,e.g.,stir-frying and pan-frying,which represent important sources of household air pollution.However,factors affecting household air pollution and the vertical variati...Chinese cooking features several unique processes,e.g.,stir-frying and pan-frying,which represent important sources of household air pollution.However,factors affecting household air pollution and the vertical variations of indoor pollutants during Chinese cooking are less clear.Here,using low-cost sensors with high time resolutions,we measured concentrations of five gas species and particulate matter(PM)in three different sizes at multiple heights in a kitchen during eighteen different Chinese cooking events.We found indoor gas species were elevated by 21%-106%during cooking,compared to the background,and PMs were elevated by 44%-159%.Vertically,the pollutants concentrations were highly variable during cooking periods.Gas species generally showed a monotonic increase with height,while PMs changed more diversely depending on the cooking activity's intensity.Intense cooking,e.g.,stir-frying,pan-frying,or cooking on high heat,tended to shoot PMs to the upper layers,while moderate ones left PMs within the breathing zone.Individuals with different heights would be subject to different levels of household air pollution exposure during cooking.The high vertical variability challenges the current indoor standard that presumes a uniform pollution level within the breathing zone and thus has important implications for public health and policy making.展开更多
This paper reports some experimental detecting results of pollutants in the atmosphere by means of laser mass spectrometry. For toluene as calibration gas, the calibration procedure was also given. Benzene, toluene an...This paper reports some experimental detecting results of pollutants in the atmosphere by means of laser mass spectrometry. For toluene as calibration gas, the calibration procedure was also given. Benzene, toluene and xylene were discovered in testing indoor atmosphere resulting from dope in the course of fitment. Meanwhile, it is noticeable that the concentration of various harmful elements is obviously decreasing as timegoeson.展开更多
Heating,ventilation and air conditioning(HVAC)systems are the most energy-consuming building implements for the improvement of indoor environmental quality(IEQ).We have developed the optimal control strategies for HVA...Heating,ventilation and air conditioning(HVAC)systems are the most energy-consuming building implements for the improvement of indoor environmental quality(IEQ).We have developed the optimal control strategies for HVAC system to respectively achieve the optimal selections of ventilation rate and supplied air temperature with consideration of energy conservation,through the fast prediction methods by using low-dimensional linear ventilation model(LLVM)based artificial neural network(ANN)and low-dimensional linear temperature model(LLTM)based contribution ratio of indoor climate(CRI_((T))).To be continued for integrated control of multi-parameters,we further developed the fast prediction model for indoor humidity by using low-dimensional linear humidity model(LLHM)and contribution ratio of indoor humidity(CRI_((H))),and thermal sensation index(TS)for assessment.CFD was used to construct the prediction database for CO_(2),temperature and humidity.Low-dimensional linear models(LLM),including LLVM,LLTM and LLHM,were adopted to expand database for the sake of data storage reduction.Then,coupling with ANN,CRI_((T)) and CRI_((H)), the distributions of indoor CO_(2) concentration,temperature,and humidity were rapidly predicted on the basis of LLVM-based ANN,LLTM-based CRIm and LLHM-based CRM respectively.Finally,according to the self-defined indices(i.e.,E_(V),E_(T),E_(H)),the optimal balancing between IEQ(indicated by CO_(2) concentration,PMV and TS)and energy consumption(indicated by ventilation rate,supplied air temperature and humidity)were synthetically evaluated.The total HVAC energy consumption could be reduced by 35%on the strength of current control strategies.This work can further contribute to development of the intelligent online control for HVAC systems.展开更多
Indoor air pollutants impact human health,comfort and productivity.The method of photocatalysis has been applied mainly in flow reactors and little information is available on indoor air pollutant removal in airtight ...Indoor air pollutants impact human health,comfort and productivity.The method of photocatalysis has been applied mainly in flow reactors and little information is available on indoor air pollutant removal in airtight reactors.In the paper,experiments were carried out to remove formaldehyde(HCHO),ammonia(NH_3) and volatile organic compounds(VOCs)in the airtight and ventilated chambers.Results demonstrated that 90.4%of HCHO,92.3%of NH_3 and 57.9%of VOCs were removed in the amine adsorption process,while 67.5% (hereinbefore,these are the mass fraction)of HCHO,60.0%of NH_3,and 61.2%of VOCs were removed in the photocatalytic process.However,ozone-assisted photocatalytic process showed great potential to degrade indoor air pollutants in the ventilated chamber.Factors and mechanisms of the photocatalytic degradation of HCHO, NH_3 and VOCs were also discussed.展开更多
The global concern over indoor air pollution in public vehicles has grown significantly.With a focus on enhancing passengers’comfort and health,this study endeavors to investigate the distribution characteristics of ...The global concern over indoor air pollution in public vehicles has grown significantly.With a focus on enhancing passengers’comfort and health,this study endeavors to investigate the distribution characteristics of formaldehyde within a high-speed train cabin by employing a computational fluid dynamics(CFD)model which is experimentally validated in a real cabin scenario.The research focuses on analyzing the impact of air supply modes,temperature,relative humidity,and fresh air change rate on the distribution and concentration of formaldehyde.The results demonstrate that the difference in average formaldehyde concentration between the two air supply modes is below 1.3%,but the top air supply mode leads to a higher accumulation of formaldehyde near the sidewalls,while the bottom air supply mode promotes a more uniform distribution of formaldehyde.Furthermore,the temperature,relative humidity,and fresh air change rate are the primary factors affecting formaldehyde concentration levels,but they have modest effects on formaldehyde’s distribution pattern within the cabin.As the temperature and relative humidity increase,the changes in formaldehyde concentrations in response to variations in these factors become more evident.Importantly,the formaldehyde concentration may surpass the standard limit of 0.10 mg/m^(3)if the fresh air change rate falls below 212 m^(3)/h.This research provides a systematic approach and referenceable results for exploring formaldehyde pollution in high-speed train cabins.展开更多
Nitrogen dioxide(NO_(2))is a prevalent air pollutant in urban areas,originating from outdoor sources,household gas consumption,and secondhand smoke.The limited evaluation of the disease burden attributable to NO_(2),e...Nitrogen dioxide(NO_(2))is a prevalent air pollutant in urban areas,originating from outdoor sources,household gas consumption,and secondhand smoke.The limited evaluation of the disease burden attributable to NO_(2),encompassing different health effects and contributions from various sources,impedes our understanding from a public health perspective.Based on modeled NO2 exposure concentrations,their exposure–response relationships with lung cancer,chronic obstructive pulmonary disease,and diabetes mellitus,and baseline disability-adjusted life years(DALYs),we estimated that 1,675(655–2,624)thousand DALYs were attributable to NO2 in urban China in 2019[138(54–216)billion Chinese yuan(CNY)economic losses].The transition from gas to electricity for household cooking was estimated to reduce the attributable economic losses by 35%.This reduction falls within the range of reductions achieved when outdoor air meets the World Health Organization interim target 3 and air quality guidelines for annual NO_(2),highlighting the significance of raising awareness of gas as a polluting household energy for cooking.These findings align with global sustainable development initiatives,providing a sustainable solution to promote public health while potentially mitigating climate change.展开更多
Filtration efficiency of portable air cleaner(PAC)is affected by resident perceptions and adherences to when and how to operate the PAC.Incorporating PAC with smart control and sensor technology holds the promise to e...Filtration efficiency of portable air cleaner(PAC)is affected by resident perceptions and adherences to when and how to operate the PAC.Incorporating PAC with smart control and sensor technology holds the promise to effectively reduce indoor air pollutants.This study aims to evaluate the efficiency of a PAC at removing indoor fine particulate matters(PM_(2.5))exposure under two automated operation settings:(1)a time-based mode in which the operation time is determined based on perceived time periods of indoor pollution by residents;(2)a sensor-based mode in which an air sensor monitor is used to determine the PAC based on the actual PM_(2.5) level against the indoor air quality guideline.The study was conducted in a residential room for 55 days with a rolling setting on PAC(no filtration,sensor-based,time-based fil-trations)and a continuous measurement of PM_(2.5).We found that the PAC operated with sensor-based mode removed PM_(2.5) concentrations by 47%and prolonged clean air(<35 μg/m^(3))period by 23%compared to the purifications with time-based mode which reduced PM_(2.5) by 29%and increased clean air period by 13%.The sensor-based filtration identified indoor pollution episodes that are hardly detected by personal perceptions.Our study findings support an automated sensor-based approach to optimize the use of PAC for effectively reducing indoor PM_(2.5) exposure.展开更多
MnxCe1- xO2(x: 0.3–0.9) prepared by Pechini method was used as a catalyst for the thermal catalytic oxidation of formaldehyde(HCHO). At x = 0.3 and 0.5, most of the manganese was incorporated in the fluorite str...MnxCe1- xO2(x: 0.3–0.9) prepared by Pechini method was used as a catalyst for the thermal catalytic oxidation of formaldehyde(HCHO). At x = 0.3 and 0.5, most of the manganese was incorporated in the fluorite structure of Ce O2 to form a solid solution. The catalytic activity was best at x = 0.5, at which the temperature of 100% removal rate is the lowest(270°C). The temperature for 100% removal of HCHO oxidation is reduced by approximately 40°C by loading 5 wt.% Cu Oxinto Mn0.5Ce0.5O2. With ozone catalytic oxidation, HCHO(61 ppm) in gas stream was completely oxidized by adding 506 ppm O3 over Mn0.5Ce0.5O2 catalyst with a GHSV(gas hourly space velocity) of 10,000 hr-1at 25°C. The effect of the molar ratio of O3 to HCHO was also investigated. As O3/HCHO ratio was increased from 3 to 8, the removal efficiency of HCHO was increased from 83.3% to 100%. With O3/HCHO ratio of 8, the mineralization efficiency of HCHO to CO2 was 86.1%. At 25°C, the p-type oxide semiconductor(Mn0.5Ce0.5O2) exhibited an excellent ozone decomposition efficiency of 99.2%,which significantly exceeded that of n-type oxide semiconductors such as Ti O2, which had a low ozone decomposition efficiency(9.81%). At a GHSV of 10,000 hr-1, [O3]/[HCHO] = 3 and temperature of 25°C, a high HCHO removal efficiency(≥ 81.2%) was maintained throughout the durability test of 80 hr, indicating the long-term stability of the catalyst for HCHO removal.展开更多
文摘The target of achieving high energy efficiency standard in order to comply with the EU Directives is leading to remarkable efforts to improve the performance of the building envelope. Excellent thermal insulation and airtight sealing of leakages are of the utmost importance to fulfil the expected targets. Unfortunately, airtightness produces the negative effect of increasing the indoor concentration of air pollutants like radon. Despite the seriousness of the problem is generally misconceived, long-term exposition to radon is acknowledged to be the second cause of lung cancer after smoke. The paper outlines the implications for the building sector and focuses on design and preventive criteria as well as on mitigation and remedial techniques.
文摘As gradual improvement of living environment and indoor decoration form diversification, the indoor air pollution has become the "invisi- ble killer" harming human health, and has been listed as one of ten big threats to human health by the World Health Organization, which also be- came one of hot issues concerned by countries all over the world. In this paper, through the determination of formaldehyde in some houses of Binzhou, the release of formaldehyde with the increase of time was explored; change of formaldehyde in the same residence in different functional areas was analyzed; the influence of the temperature, humidity and plant to formaldehyde content was also analyzed.
文摘Objective The study was designed to compare the combustion products of coal gas, liquefied petroleum gas and natural gas in relation to indoor air pollution. Methods Regular pollutants including B(a)P were monitored and 1-hydroxy pyrene were tested in urine of the enrolled subjects. Radon concentrations and their changes in four seasons were also monitored in the city natural gas from its source plant and transfer stations to final users. To analyze organic components of coal gas, liquefied petroleum gas and natural gas, a high-flow sampling device specially designed was used to collect their combustion products, and semi-volatile organic compounds contained in the particles were detected by gas chromatograph-mass spectrograph (GC/MS). Results Findings in the study showed that the regular indoor air pollutants particles and CO were all above the standard in winter when heating facilities were operated in the city, but they were lowest in kitchens using natural gas; furthermore, although NO2 and CO2 were slightly higher in natural gas, B(a)P concentration was lower in this group and 1-hydroxy pyrene was lowest in urine of the subjects exposed to natural gas. Organic compounds were more complicated in coal gas and liquefied petroleum gas than in natural gas. The concentration of radon in natural gas accounted for less than 1‰ of its effective dose contributing to indoor air pollution in Beijing households. Conclusion Compared to traditional fuels, gases are deemed as clean ones, and natural gas is shown to be cleaner than the other two gases.
基金This study was support by Tenth-five Program of China (2001BA70B02)
文摘To establish the model of indoor air pollution forecast for decoration. Methods The model was based on the balance model for diffusing mass. Results The data between testing concentration and estimating concentration were compared. The maximal error was less than 30% and average error was 14.6%. Conclusion The model can easily predict whether the pollution for decoration exceeds the standard and how long the room is decorated.
文摘Three representative types of houses in Beijing were selected and, in each type, smoking and nonsmoking households were compared. IP, RP. and CO concentrations in the living room and kitchen were monitored during each season. and the level of COHb in the heads of the households were measured. The study showed that indoor air pollution was rather severe, especially during winter. when paniculate concentrations markedly exceeded the standard and CO concentration was as high as 47 ppm. Indoor air pollution was closely related to the type of house, particularly to the mode of heating. In houses. of the same type, pollution improved greatly after central heating facilities were installed. Analysis of 30 elements revealed that pollution was typically caused by coal burning. aggravated by dusty wind, but high indoor Pb levels were probably due to the use of LPG for cooking. In our study the effect of cigarette smoking was sometimes masked by the severe indoor pollution. (C)1990 Academic Press, Inc.
文摘Individuals spend 90% of their time indoors, primarily at home or at work. Indoor environmental factors have a significant impact on human well-being. It was a longitudinal study that assessed the major factors that reduce indoor air quality, namely particulate matter, and bio-aerosols, using low-cost sensors and the settle plate method, respectively also to determine the effect of atmospheric parameters and land use patterns in households of commercial, industrial, residential, slum, and rural areas of the city. PM2.5 concentration levels were similar in most parts of the day across all sites. PM10.0 concentration levels increased indoors in a commercial area. PM2.5 concentration showed a negative correlation with temperature and a positive correlation with relative humidity in some areas. Very high values of PM2.5 concentration and PM10.0 concentration have been observed in this study, inside households of selected rural and urban areas. Pathogenic gram-positive cocci, gram-positive rods, Aspergillus, and Mucor species were the most common bacterial and fungal species respectively found inside households. This study examined particulate matter concentration along with bio-aerosols, as very less studies have been conducted in Jaipur the capital of Rajasthan, a state in the western part of India which assessed both of these factors together to determine the indoor air quality. Rural households surrounding the periphery of the city were found to have similar pollution levels as urban households. So, this study may form the basis for reducing pollution inside households and also for taking suitable measures for the reduction of pollution in the indoor environment.
文摘Indoor air pollution in buildings puts people at risk of developing respiratory and cardiovascular diseases.Particulate matter(PM)exposure is known to cause these health issues.Preliminary efforts were made in this study to assess the quantity and quality of PM1.0,PM_(2.5),and PM_(10)present in an abattoir and a residential building in northern Nigeria.Canree A1 low-cost sensor was used to monitor the locations,8 hourly for two weeks.The results showed that the average values(μg/m^(3))of PM1.0,PM_(2.5),and PM_(10)in an abattoir were 62.74,161.94,and 199.08,respectively,and in a residential building were 28.70,83.31,and 103.71.The average Air Quality Index(AQI)of the abattoir office was Very Unhealthy,while the living room of the residential building was unhealthy.The PM_(2.5),and PM_(10)levels were higher than the international(WHO)and national(FMEnv)standard limits,indicating a potential danger to building occupants.It is expected that the indoor environment of the locations will be improved by the use of good ventilators(adequate windows and doors)and the provision of good extractors.
基金This work was supported by Beijing Natural Science Foundation(7222246)Royal Dutch Philips Electronics Ltd.(Grant NL18-2100478471).
文摘Objective Evidence on potential cardiovascular benefits of personal-level intervention among the elderly exposed to high levels of particulate matter(PM)remains limited.We aimed to assess improvements in surrogate markers of cardiovascular injury in vulnerable populations at risks by using indoor air filtration units.Methods We conducted a randomized crossover trial for 2 separate 2-week air filtration interventions in 20 households of patients with stable chronic obstructive pulmonary disease and their partners in the winter of 2013,with concurrent measurements of indoor PM.The changes in biomarkers indicative of cardiac injury,atherosclerosis progression and systemic inflammation following intervention were evaluated using linear mixed-effect models.Results In the analysis,average levels of indoor PM with aerodynamic diameters<2.5µm(PM2.5)decreased significantly by 59.2%(from 59.6 to 24.3µg/m3,P<0.001)during the active air filtration.The reduction was accompanied by improvements in levels of high-sensitivity cardiac troponin I by−84.6%(95%confidence interval[CI]:−90.7 to−78.6),growth differentiation factor-15 by−48.1%(95%CI:−31.2 to−25.6),osteoprotegerin by−65.4%(95%CI:−56.5 to−18.7),interleukin-4 by−46.6%(95%CI:−62.3 to−31.0)and myeloperoxidase by−60.3%(95%CI:−83.7 to−3.0),respectively.Conclusion Indoor air filtration intervention may provide potential cardiovascular benefits in vulnerable populations at risks.
文摘Exposure to CO (carbon monoxide) during cooking in households using LPG (liquefied petroleum gas), natural gas and charcoal as fuels has been conducted. The study aimed at assessing the indoor air quality in order to address potential hazards associated with CO. Carbon monoxide concentrations and flame temperature were measured at an interval of 1 min for 1 h using CO and thermometer data loggers respectively. While the CO concentration from LPG and natural gas were found below 26 ppm for 1 h, as recommended by WHO (World Health Organization) standards, the average CO concentration from charcoal exceeded the standard limit. In addition closing the kitchen door during cooking increased the CO concentration from 26-295 ppm to 92-597 ppm. According to WHO, the observed CO concentrations from charcoal stove highlights questionable life support atmosphere. It can therefore be suggested that switching to LPG or natural gas from charcoal will reduce CO exposure to persons during cooking.
基金the auspices of National Key Research and Development Program of China(No.2017YFC0212303,2017YFC0212304)National Natural Science Foundation of China(No.41771504)National Natural Science Foundation of Jilin Province(No.20200201214JC)。
文摘Domestic burning emits large amounts of pollutants into the ambient air due to incomplete and inefficient combustion, with significant impacts on indoor air quality and human health. Northeast China is one of the major contributors to domestic burning emissions in China;however, the high-resolution emissions inventories of domestic biomass and coal burning in Northeast China are lacked, which are needed to estimate the extent of its impact. In this study, we established a town-level emissions inventory of gaseous pollutants and particulate matter(PM) from domestic biomass and coal burning, based on per household consumption in each town in rural region of Northeast China. The results revealed that biomass burning was the major domestic burning source over the region in 2016. Domestic biomass burning is the major contributor to PM and volatile organic compounds(VOCs) emissions, while coal burning is the major contributor to SO2 emissions. High emissions intensities were concentrated around the cities of Harbin, Suihua, Changchun, Qiqihar, and Chifeng, each with emissions intensity for PM2.5 and VOCs of more than 2000 Mg per 27 km × 27 km grid cell. Additionally, there are three burning peaks(6-7 am, 12 pm and 4-7 pm) during both the heating(from October to April) and non-heating seasons(from May to September), due to cooking and heating. The burning peaks in the non-heating season were more notable than those in the heating season. These results suggest that the government should pay more attention to domestic biomass and coal burning in rural areas, in order to reduce pollutant emissions and control regional haze during the heating season.
基金the Conselho Nacional de Desenvolvimento Científico e Tecnológico(CNPq)for financial support。
文摘Because incomplete confirmation is available concerning the influential role of atmosphere contamination on conjunctivitis,myopia,asthma,and allergic rhinitis in Brazil,the focus of the present work is to explore the possible relations among atmosphere contamination and eye problems.Rather that a case study on eye diseases,by way of questionnaires supplemented by the investigation of nanoparticles(NPs)on eyeglasses,the study examines the mechanisms in which NPs and ultra-fine particles are deposited on the glasses of children up to 10 years of age in urban and rural area.The important connection between atmosphere contaminants and individual protection equipment justifies improving indoor school properties in order could protect children’s eyes,particularly in high-pollution/high-particulate areas.
基金supported by a grant from the National Science Foundation of China (No. 20977075)the National High Technology Research and Development Program of China (863) (No. 2010AA064902)
文摘The concentrations of phthalate esters(PAEs) in Chinese hospitals were investigated by simultaneously determining concentrations of gas- and particle-phase PAEs. PAEs were detected in two third-class first-grade hospitals, two second-class first-grade hospitals, and a community health service center. Hospital drugstores had the highest concentration(24.19 μg/m3), which was 1.54 times that of newly decorated houses. The second highest concentration was found in the transfusion rooms, averaging 21.89 μg/m3; this was followed by the concentrations of PAEs in the nurse's workstations, the wards, and the doctor's offices, with mean concentrations of 20.66, 20.0, and 16.92 μg/m3, respectively. The lowest concentrations were found in the hallways(16.30 μg/m3). Of the six different kinds of PAEs found, major pollutants included diethyl phthalates, dibutyl phthalates, butylbenzyl phthalates and di(2-ethylhexyl) phthalates, comprising more than 80% of all PAEs present.Meanwhile, a comparison between different wards showed that PAE concentrations in the maternity wards were 1.63 times higher than in the main wards. Based on known health hazards, our results suggest that the PAEs seriously influence the health of the pregnant women and babies; therefore, it is of great importance to take the phthalate concentrations in hospitals into consideration. In addition, hospital indoor air was more seriously contaminated than the air of newly decorated houses.
基金supported by the National Natural Science Foundation of China(Grants 41991312,41821005,41922057,41830641,and 42192510)Shenzhen Environmental Monitoring Center(Grant 0722-216FE4812SZF-2)+1 种基金Department of Education of Guangdong Province(2021KCXTD004)Center for Computational Science and Engineering at Southern University of Science and Technology.
文摘Chinese cooking features several unique processes,e.g.,stir-frying and pan-frying,which represent important sources of household air pollution.However,factors affecting household air pollution and the vertical variations of indoor pollutants during Chinese cooking are less clear.Here,using low-cost sensors with high time resolutions,we measured concentrations of five gas species and particulate matter(PM)in three different sizes at multiple heights in a kitchen during eighteen different Chinese cooking events.We found indoor gas species were elevated by 21%-106%during cooking,compared to the background,and PMs were elevated by 44%-159%.Vertically,the pollutants concentrations were highly variable during cooking periods.Gas species generally showed a monotonic increase with height,while PMs changed more diversely depending on the cooking activity's intensity.Intense cooking,e.g.,stir-frying,pan-frying,or cooking on high heat,tended to shoot PMs to the upper layers,while moderate ones left PMs within the breathing zone.Individuals with different heights would be subject to different levels of household air pollution exposure during cooking.The high vertical variability challenges the current indoor standard that presumes a uniform pollution level within the breathing zone and thus has important implications for public health and policy making.
文摘This paper reports some experimental detecting results of pollutants in the atmosphere by means of laser mass spectrometry. For toluene as calibration gas, the calibration procedure was also given. Benzene, toluene and xylene were discovered in testing indoor atmosphere resulting from dope in the course of fitment. Meanwhile, it is noticeable that the concentration of various harmful elements is obviously decreasing as timegoeson.
基金the funding support from National Natural Science Foundation of China(No.51778385).
文摘Heating,ventilation and air conditioning(HVAC)systems are the most energy-consuming building implements for the improvement of indoor environmental quality(IEQ).We have developed the optimal control strategies for HVAC system to respectively achieve the optimal selections of ventilation rate and supplied air temperature with consideration of energy conservation,through the fast prediction methods by using low-dimensional linear ventilation model(LLVM)based artificial neural network(ANN)and low-dimensional linear temperature model(LLTM)based contribution ratio of indoor climate(CRI_((T))).To be continued for integrated control of multi-parameters,we further developed the fast prediction model for indoor humidity by using low-dimensional linear humidity model(LLHM)and contribution ratio of indoor humidity(CRI_((H))),and thermal sensation index(TS)for assessment.CFD was used to construct the prediction database for CO_(2),temperature and humidity.Low-dimensional linear models(LLM),including LLVM,LLTM and LLHM,were adopted to expand database for the sake of data storage reduction.Then,coupling with ANN,CRI_((T)) and CRI_((H)), the distributions of indoor CO_(2) concentration,temperature,and humidity were rapidly predicted on the basis of LLVM-based ANN,LLTM-based CRIm and LLHM-based CRM respectively.Finally,according to the self-defined indices(i.e.,E_(V),E_(T),E_(H)),the optimal balancing between IEQ(indicated by CO_(2) concentration,PMV and TS)and energy consumption(indicated by ventilation rate,supplied air temperature and humidity)were synthetically evaluated.The total HVAC energy consumption could be reduced by 35%on the strength of current control strategies.This work can further contribute to development of the intelligent online control for HVAC systems.
基金the National Natural Science Foundation of China(No.21177087)the Shanghai Environmental Protection Bureau(SEPB)Program(No.09-26)
文摘Indoor air pollutants impact human health,comfort and productivity.The method of photocatalysis has been applied mainly in flow reactors and little information is available on indoor air pollutant removal in airtight reactors.In the paper,experiments were carried out to remove formaldehyde(HCHO),ammonia(NH_3) and volatile organic compounds(VOCs)in the airtight and ventilated chambers.Results demonstrated that 90.4%of HCHO,92.3%of NH_3 and 57.9%of VOCs were removed in the amine adsorption process,while 67.5% (hereinbefore,these are the mass fraction)of HCHO,60.0%of NH_3,and 61.2%of VOCs were removed in the photocatalytic process.However,ozone-assisted photocatalytic process showed great potential to degrade indoor air pollutants in the ventilated chamber.Factors and mechanisms of the photocatalytic degradation of HCHO, NH_3 and VOCs were also discussed.
基金This work is supported by the National Natural Science Foundation of China(No.52072413)the graduate school of Central South University(No.1053320220012).The authors are grateful for resources from the High-Performance Computing Center of Central South University.
文摘The global concern over indoor air pollution in public vehicles has grown significantly.With a focus on enhancing passengers’comfort and health,this study endeavors to investigate the distribution characteristics of formaldehyde within a high-speed train cabin by employing a computational fluid dynamics(CFD)model which is experimentally validated in a real cabin scenario.The research focuses on analyzing the impact of air supply modes,temperature,relative humidity,and fresh air change rate on the distribution and concentration of formaldehyde.The results demonstrate that the difference in average formaldehyde concentration between the two air supply modes is below 1.3%,but the top air supply mode leads to a higher accumulation of formaldehyde near the sidewalls,while the bottom air supply mode promotes a more uniform distribution of formaldehyde.Furthermore,the temperature,relative humidity,and fresh air change rate are the primary factors affecting formaldehyde concentration levels,but they have modest effects on formaldehyde’s distribution pattern within the cabin.As the temperature and relative humidity increase,the changes in formaldehyde concentrations in response to variations in these factors become more evident.Importantly,the formaldehyde concentration may surpass the standard limit of 0.10 mg/m^(3)if the fresh air change rate falls below 212 m^(3)/h.This research provides a systematic approach and referenceable results for exploring formaldehyde pollution in high-speed train cabins.
基金was supported by the National Natural Science Foundation of China(grant number 51978366).
文摘Nitrogen dioxide(NO_(2))is a prevalent air pollutant in urban areas,originating from outdoor sources,household gas consumption,and secondhand smoke.The limited evaluation of the disease burden attributable to NO_(2),encompassing different health effects and contributions from various sources,impedes our understanding from a public health perspective.Based on modeled NO2 exposure concentrations,their exposure–response relationships with lung cancer,chronic obstructive pulmonary disease,and diabetes mellitus,and baseline disability-adjusted life years(DALYs),we estimated that 1,675(655–2,624)thousand DALYs were attributable to NO2 in urban China in 2019[138(54–216)billion Chinese yuan(CNY)economic losses].The transition from gas to electricity for household cooking was estimated to reduce the attributable economic losses by 35%.This reduction falls within the range of reductions achieved when outdoor air meets the World Health Organization interim target 3 and air quality guidelines for annual NO_(2),highlighting the significance of raising awareness of gas as a polluting household energy for cooking.These findings align with global sustainable development initiatives,providing a sustainable solution to promote public health while potentially mitigating climate change.
基金supported by the start-up funding of University at Buffalo.
文摘Filtration efficiency of portable air cleaner(PAC)is affected by resident perceptions and adherences to when and how to operate the PAC.Incorporating PAC with smart control and sensor technology holds the promise to effectively reduce indoor air pollutants.This study aims to evaluate the efficiency of a PAC at removing indoor fine particulate matters(PM_(2.5))exposure under two automated operation settings:(1)a time-based mode in which the operation time is determined based on perceived time periods of indoor pollution by residents;(2)a sensor-based mode in which an air sensor monitor is used to determine the PAC based on the actual PM_(2.5) level against the indoor air quality guideline.The study was conducted in a residential room for 55 days with a rolling setting on PAC(no filtration,sensor-based,time-based fil-trations)and a continuous measurement of PM_(2.5).We found that the PAC operated with sensor-based mode removed PM_(2.5) concentrations by 47%and prolonged clean air(<35 μg/m^(3))period by 23%compared to the purifications with time-based mode which reduced PM_(2.5) by 29%and increased clean air period by 13%.The sensor-based filtration identified indoor pollution episodes that are hardly detected by personal perceptions.Our study findings support an automated sensor-based approach to optimize the use of PAC for effectively reducing indoor PM_(2.5) exposure.
文摘MnxCe1- xO2(x: 0.3–0.9) prepared by Pechini method was used as a catalyst for the thermal catalytic oxidation of formaldehyde(HCHO). At x = 0.3 and 0.5, most of the manganese was incorporated in the fluorite structure of Ce O2 to form a solid solution. The catalytic activity was best at x = 0.5, at which the temperature of 100% removal rate is the lowest(270°C). The temperature for 100% removal of HCHO oxidation is reduced by approximately 40°C by loading 5 wt.% Cu Oxinto Mn0.5Ce0.5O2. With ozone catalytic oxidation, HCHO(61 ppm) in gas stream was completely oxidized by adding 506 ppm O3 over Mn0.5Ce0.5O2 catalyst with a GHSV(gas hourly space velocity) of 10,000 hr-1at 25°C. The effect of the molar ratio of O3 to HCHO was also investigated. As O3/HCHO ratio was increased from 3 to 8, the removal efficiency of HCHO was increased from 83.3% to 100%. With O3/HCHO ratio of 8, the mineralization efficiency of HCHO to CO2 was 86.1%. At 25°C, the p-type oxide semiconductor(Mn0.5Ce0.5O2) exhibited an excellent ozone decomposition efficiency of 99.2%,which significantly exceeded that of n-type oxide semiconductors such as Ti O2, which had a low ozone decomposition efficiency(9.81%). At a GHSV of 10,000 hr-1, [O3]/[HCHO] = 3 and temperature of 25°C, a high HCHO removal efficiency(≥ 81.2%) was maintained throughout the durability test of 80 hr, indicating the long-term stability of the catalyst for HCHO removal.