Design of compact integrated diamond nitrogen-vacancy center quantum probe

An integrated quantum probe for magnetic field imaging is proposed,where the nitrogen–vacancy(NV)center fixed at the fiber tip is located on the periphery of flexible ring resonator.Using flexible polyimide(PI)as the substrate medium,we design a circular microstrip antenna,which can achieve a bandwidth of 140 MHz at Zeeman splitting frequency of 2.87 GHz,specifically suitable for NV center experiments.Subsequently,this antenna is seamlessly fixed at a three-dimensional-printed cylindrical support,allowing the optical fiber tip to extend out of a dedicated aperture.To mitigate errors originating from processing,precise tuning within a narrow range can be achieved by adjusting the conformal amplitude.Finally,we image the microwave magnetic field around the integrated probe with high resolution,and determine the suitable area for placing the fiber tip(SAP).

Current sensor based on diamond nitrogen-vacancy color center

High precision current measurement is very important for the calibration of various high-precision equipment and the measurement of other precision detection fields.A new current sensor based on diamond nitrogen-vacancy(NV)color center magnetic measurement method is proposed to realize the accurate measurement of current.This new current method can greatly improve the accuracy of current measurement.Experiments show that the linearity of the current sensor based on diamond NV color center can reach up to 33 ppm,which is superior to other current sensors and solves the problem of low linearity.When the range of input current is 5-40 A,the absolute error of the calculated current is less than 51μA,and the relative error is 2.42×10^(-6) at 40 A.Combined with the research content and results of the experiment,the application of the current sensor in the field of current precision measurement is prospected.

Non-destructive Testing Method for Crack Based on Diamond Nitrogen-vacancy Color Center

Magnetic field measurement plays an extremely important role in material science,electronic en-gineering,power system and even industrial fields.In particular,magnetic field measurement provides a safe and reliable tool for industrial non-destructive testing.The sensitivity of magnetic field measurement deter-mines the highest level of detection.The diamond nitrogen-vacancy(NV)color center is a new type of quan-tum sensor developed in recent years.The external magnetic field will cause Zeeman splitting of the ground state energy level of the diamond NV color center.Optical detection magnetic resonance(ODMR),using a mi-crowave source and a lock-in amplifier to detect the resonant frequency of the NV color center,and finally the change of the resonant frequency can accurately calculate the size of the external magnetic field and the sensi-tivity of the external magnetic field change.In the experiment,a diamond containing a high concentration of NV color centers is coupled with an optical fiber to realize the preparation of a magnetic field scanning probe.Then,the surface cracks of the magnetized iron plate weld are scanned,and the scanning results are drawn into a two-dimensional magnetic force distribution map,according to the magnetic field gradient change of the magnetic force distribution map,the position and size of the crack can be judged very accurately,which pro-vides a very effective diagnostic tool for industrial safety.

Electron Spin Decoherence of Nitrogen-Vacancy Center Coupled to Multiple Spin Baths

We present the experimental results of nitrogen-vacancy （NV） electron spin decoherence, which are linked to the coexistence of electron spin bath of nitrogen impurity （PI center） and 13C nuclear spin bath. In previous works, only one dominant decoherence source is studied： P1 electron spin bath for type-Ⅰb diamond; or 13C nuclear spin bath for type-Ⅱa diamond. In general, the thermal fluctuation from both spin baths can be eliminated by the Hahn echo sequence, resulting in a long coherence time （T2 ） of about 400#8. However, in a high-purity type-Ⅱa diamond where 1℃ nuclear spin bath is the dominant decoherence source, dramatic decreases of NV electron spin T2 time caused by P1 electron spin bath are observed under certain magnetic field. We further apply the engineered Hahn echo sequence to confirm the decoherenee mechanism of multiple spin baths and quantitatively estimate the contribution of P1 electron spin bath. Our results are helpful to understand the NV decoherence mechanisms, which will benefit quantum computing and quantum metrology.

Scalable Quantum Information Transfer between Individual Nitrogen-Vacancy Centers by a Hybrid Quantum Interface

We develop a design of a hybrid quantum interface for quantum information transfer （QIT）, adopting a nanome- chanical resonator as the intermedium, which is magnetically coupled with individual nitrogen-vacancy centers as the solid qubits, while eapacitively coupled with a coplanar waveguide resonator as the quantum data bus. We describe the Hamiltonian of the model, and analytically demonstrate the QIT for both the resonant interaction and large detuning cases. The hybrid quantum interface allows for QIT between arbitrarily selected individual nitrogen-vacancy centers, and has advantages of the sealability and controllability. Our methods open an alter- native perspective for implementing QIT, which is important during quantum storing or processing procedures in quantum computing.

Time-bin-encoding-based remote states generation of nitrogen-vacancy centers through noisy channels

We design proposals to generate a remote Greenberger-Horne-Zeilinger（GHZ） state and a W state of nitrogenvacancy（NV） centers coupled to microtoroidal resonators（MTRs） through noisy channels by utilizing time-bin encoding processes and fast-optical-switch-based polarization rotation operations.The polarization and phase noise induced by noisy channels generally affect the time of state generation but not its success probability and fidelity.Besides,the above proposals can be generalized to n-qubit between two or among n remote nodes with success probability unity under ideal conditions.Furthennore,the proposals are robust for regular noise-changeable channels for the n-node case.This method is also useful in other remote quantum information processing tasks through noisy channels.

Orientation determination of nitrogen-vacancy center in diamond using a static magnetic field

Nitrogen-vacancy(NV)centers in a bulk diamond are often employed to realize measurement of multiple physical quantities,which depends on orientation information of NV axis.We report a fast and effective method to determine the orientation of NV axis with the aid of a static magnetic field.By measuring the optically detected magnetic resonance spectra,we can precisely extract the polar angle information between the NV axis and the known magnetic field.Combining with the polar angle information of different kinds of NV centers,we employ the Nelder-Mead algorithm to get the optimal solution of the orientation of NV axis.This method is simple and efficient,and is easily applied in NV-based quantum sensing.

A Bright Single-Photon Source from Nitrogen-Vacancy Centers in Diamond Nanowires

Single-photon flux is one of the crucial properties of nitrogen vacancy （NV） centers in diamond for its application in quantum information techniques. Here we fabricate diamond conical nanowires to enhance the single-photon count rate. Through the interaction between tightly confined optical mode in nanowires and NV centers, the single-photon lifetime is much shortened and the collection efficiency is enhanced. As a result, the detected single-photon rate can be at 564 kcps, and the total detection coefficient can be 0.8%, which is much higher than that in bulk diamond. Such a nanowire single-photon device with high photon flux can be applied to improve the fidelity of quantum computation and the precision of quantum sensors.

A nanosecond level current pulse capture taper optical fiber probe based on micron level nitrogen-vacancy color center diamond

This work demonstrates a micron-sized nanosecond current pulse probe using a quantum diamond magnetometer.A micron-sized diamond crystal affixed to a fiber tip is integrated on the end of a conical waveguide.We demonstrate real-time visualization of a single 100 nanosecond pulse and discrimination of two pulse trains of different frequencies with a coplanar waveguide and a home-made PCB circuit.This technique finds promising applications in the display of electronic stream and can be used as a pulse discriminator to simultaneously receive and demodulate multiple pulse frequencies.This method of detecting pulse current is expected to provide further detailed analysis of the internal working state of the chip.

Transient features of graphitization and nitrogen-vacancy color centers in a diamond fabricated by localization femtosecond laser direct writing

Femtosecond laser direct writing provides an efficient approach to fabricating single nitrogen vacancy(NV) color centers with a relatively high yield. Different from previously reported NV color centers with a random distribution in a bulk diamond or nanocrystals, this gives an opportunity to study the photophysical properties of single NV color centers with precise numbers and positions. However, ultrafast studies on single NV color centers prepared by localization femtosecond laser direct writing are still rare, especially for the graphitization inside a diamond and its relationship with single NV color centers. Here, we report the broadband transient absorption(TA) spectroscopic features of the graphitization and NV color centers in a diamond fabricated by localization femtosecond laser direct writing at room temperature under 400 nm excitation. In comparison with the graphene oxide film, the bleaching features of the graphitization point array in a diamond are similar to reduced graphene oxide,accompanied by excited state absorption signals from local carbon atom vacancy defects in graphene-like structures induced by laser writing. On the other hand, transient features of laser processing array containing single NV color centers with a yield of~50% are different from those of the graphitization point array. Our findings suggest that for ultrashort pulse processing of diamonds, broadband TA spectral signals are sensitive to the surrounding atomic environment of processing sites, which could be applied to laser writing point defects in other materials used as solid-state single photon sources.

Hybrid opto-mechanical systems with nitrogen-vacancy centers

In this review, we briefly review recent works on hybrid （nano） and diamond nitrogen-vacancy （NV） centers. We also review opto-mechanical systems that contain both mechanical oscillators two different types of mechanical oscillators. The first one is a clamped mechanical oscillator, such as a cantilever, with a fixed frequency. The second one is an optically trapped nano-diamond with a built-in nitrogen-vacancy center. By coupling mechanical resonators with electron spins, we can use the spins to control the motion of mechanical oscillators. For the first setup, we discuss two different coupling mechanisms, which are magnetic coupling and strain induced coupling. We summarize their applications such as cooling the mechanical oscillator, generating entanglements between NV centers, squeezing spin ensembles etc. For the second setup, we discuss how to generate quantum superposition states with magnetic coupling, and realize matter wave interferometer. We will also review its applications as ultra-sensitive mass spectrometer. Finally, we discuss new coupling mechanisms and applications of the field.

Virtual-photon-induced entanglement with two nitrogen-vacancy centers coupled to a high-Q silica microsphere cavity

We propose a potentially practical scheme for efcient generation of entanglement with two nitrogen-vacancy centers(NVC)coupled to a whispering-gallery mode cavity.By virtue of the virtual-photon-excitation,the entanglement with two separate NVC can be produced in a deterministic way.The required operations are very close to the capabilities of current experimental techniques.The efects of decoherence induced by the cavity decay and the atomic spontaneous decay are also investigated.

Time-optimal control for hybrid systems based on the nitrogen-vacancy center

Fast and high fidelity quantum control is the key technology of quantum computing. The hybrid system composed of the nitrogen-vacancy center and nearby Carbon-13 nuclear spin is expected to solve this problem. The nitrogen-vacancy center electron spin enables fast operations for its strong coupling to the control field, whereas the nuclear spins preserve the coherence for their weak coupling to the environment. In this paper, we describe a strategy to achieve time-optimal control of the Carbon-13 nuclear spin qubit by alternating controlling the nitrogen-vacancy center electron spin as an actuator. We transform the qubit gate operation into a switched system. By using the maximum principle, we study the minimum time control of the switched system and obtain the time-optimal control of the qubit gate operation. We show that the X gate and Y gate operations are within 10μs while the fidelity reaches 0.995.

Preparation of Macroscopic Entangled Coherent States in Nitrogen-Vacancy Centers Ensembles Coupled to a Superconducting Flux Qubit

We propose a potentially practical scheme for creating macroscopic entangled coherent state between two separate nitrogen-vacancy center spin ensembles placed near a superconducting flux qubit. Through the collective magnetic coupling and the in situ tunability of the flux qubit, the arbitrary entangled coherent states of spin ensembles can be achieved with high success possibilities under the influence from decoherence of the flux qubit and spin ensembles.The experimental feasibility and challenge are justified using currently available technology.

Nonadiabatic holonomic quantum computation based on nitrogen-vacancy centers

Because of quantum superposition, quantum computation can solve many problems, such as factoring large integers [ 1 ] and searching unsorted databases [2,3], much faster than clas- sical computation. To realize practical quantum computation and then gain the desired advantages, a universal set of quantum gates with sufficiently high fidelities are needed. However, various inevitable errors reduce the gate fidelities and finally collapse the computation results, which makes the realizations of quantum computation very challenging.

Simultaneous detection of position and temperature of micromagnet using a quantum microscope

Micromagnets,as a promising technology for microscale manipulation and detection,have been the subject of extensive study.However,providing real-time,noninvasive feedback on the position and temperature of micromagnets in complex operational environments continues to pose a significant challenge.This paper presents a quantum imaging device utilizing diamond nitrogen-vacancy(NV)centers capable of providing simultaneous feedback on both the position and temperature of a micromagnet.The device achieves a temporal resolution of 2 s and a spatial resolution of 1.3μm.Through flux localization analysis,we have determined a positioning accuracy within 50μm and a temperature accuracy within 0.4 K.

Sabatier principle guiding the design of cathode catalysts for Li-CO_(2) batteries

The Sabatier principle has been widely used for designing electrocatalysts for energy conversion applications,but it is rarely mentioned in the research of cathode catalyst of Li-CO_(2) batteries.In our work,the"volcanic"relationship between the catalytic activity and the adsorption energy of the catalyst to the intermediates is first demonstrated based on the first-principles calculation,which meets the Sabatier principle and can be used to design the cathode catalysts.The increases in the number of nitrogenvacancy in WN shift the d-band center and increase the interaction with the reactants.The catalytic activity increases first and then decreases with the increase of adsorption energy,which was proved in the experiment.The optimal catalyst for moderate adsorption of intermediate makes the thin LiaCO_(3) distribute evenly.It exhibits a median voltage difference of 0.68 V and an energy efficiency of 84.33%at20μA cm^(-2)with a limited capacity of 200μA h cm^(-2).

High-resolution imaging of magnetic fields of banknote anti-counterfeiting strip using fiber diamond probe

Counterfeiting of modern banknotes poses a significant challenge,prompting the use of various preventive measures.One such measure is the magnetic anti-counterfeiting strip.However,due to its inherent weak magnetic properties,visualizing its magnetic distribution has been a longstanding challenge.In this work,we introduce an innovative method by using a fiber optic diamond probe,a highly sensitive quantum sensor designed specifically for detecting extremely weak magnetic fields.We employ this probe to achieve high-resolution imaging of the magnetic fields associated with the RMB 50denomination anti-counterfeiting strip.Additionally,we conduct computer simulations by using COMSOL Multiphysics software to deduce the potential geometric characteristics and material composition of the magnetic region within the anti-counterfeiting strip.The findings and method presented in this study hold broader significance,extending the RMB 50 denomination to various denominations of the Chinese currency and other items that employ magnetic anti-counterfeiting strips.These advances have the potential to significantly improve and promote security measures in order to prevent the banknotes from being counterfeited.

Design and simulation of an accelerometer based on NV center spin–strain coupling

The nitrogen-vacancy (NV) center quantum systems have emerged as versatile tools in the field of precision measurement because of their high sensitivity in spin state detection and miniaturization potential as solid-state platforms.In this paper,an acceleration sensing scheme based on NV spin–strain coupling is proposed,which can effectively eliminate the influence of the stray noise field introduced by traditional mechanical schemes.Through the finite element simulation,it is found that the measurement bandwidth of this ensemble NV spin system ranges from 3 kHz to hundreds of kHz with structure√optimization.The required power is at the sub-μW level,corresponding to a noise-limited sensitivity of 6.7×10^(-5) /√Hz.Compared with other types of accelerometers,this micro-sized diamond sensor proposed here has low power consumption,exquisite sensitivity,and integration potential.This research opens a fresh perspective to realize an accelerometer with appealing comprehensive performance applied in biomechanics and inertial measurement fields.

Magnetic field analysis in a diamond anvil cell for Meissner effect measurement by using the diamond NV^- center

Diamond negatively charged nitrogen-vacancy(NV-) centers provide an opportunity for the measurement of the Meissner effect on extremely small samples in a diamond anvil cell(DAC) due to their high sensitivity in detecting the tiny change of magnetic field. We report on the variation of magnetic field distribution in a DAC as a sample transforms from normal to superconducting state by using finite element analysis. The results show that the magnetic flux density has the largest change on the sidewall of the sample, where NV-centers can detect the strongest signal variation of the magnetic field. In addition, we study the effect of magnetic coil placement on the magnetic field variation. It is found that the optimal position for the coil to generate the greatest change in magnetic field strength is at the place as close to the sample as possible.