Gas-liquid (G-L) and liquid-solid (L-S) mass transfer coefficients were characterized in a gas-liquid-solid (G-L-S) three-phase magnetically stabilized bed (MSB) using amorphous alloy SRNA-4 as the solid phase. Effect...Gas-liquid (G-L) and liquid-solid (L-S) mass transfer coefficients were characterized in a gas-liquid-solid (G-L-S) three-phase magnetically stabilized bed (MSB) using amorphous alloy SRNA-4 as the solid phase. Effects such as superficial liquid velocity, superficial gas velocity, magnetic strength, liquid viscosity, and particle size were investigated. Experimental results indicated that the G-L volumetric mass transfer coefficients (KLa) increased along with the magnetic strength, superficial gas and liquid velocities. Proper increase of liquid viscosity promoted KLa only in the range of lower liquid viscosity. The external magnetic field made L-S mass transfer coefficients (Ks) in the G-L-S MSB lower than those of conventional fluidized beds. Ks in the MSB almost kept constant as the su- perficial liquid velocity and superficial gas velocity increased and decreased with the liquid viscosity and surface tension, while increased with the particle size Ks showed uniform axial and radial distributions except of small de- creases close to the wall. Dimensionless correlations were established to estimate KLa and Ks of the MSB with SRNA-4 catalysts , which showed the average error of 5.4% and 2.5% respectively.展开更多
Liquid-solid （L-S） mass transfer coefficients （Ks） were characterized in a gas-liquid-solid （G-L-S） three-phase countercurrent magnetically stabilized bed （MSB） using amorphous alloy SRNA-4 as the solid phase....Liquid-solid （L-S） mass transfer coefficients （Ks） were characterized in a gas-liquid-solid （G-L-S） three-phase countercurrent magnetically stabilized bed （MSB） using amorphous alloy SRNA-4 as the solid phase. Effects of superficial liquid velocity, superficial gas velocity, magnetic field strength, liquid viscosity and surface tension were investigated. Experimental results indicated that the external magnetic field increased Ks in three-phase MSB, as compared to those in conventional G-L-S fluidized beds; that Ks increased with magnetic field strength, superficial gas and liquid velocities and decreased with liquid viscosity and surface tension; and that Ks showed uniform axial and radial distributions except for small increases close to the wall. Dimensionless correlations were established to estimate Ks of the G-L-S countercurrent MSB using SRNA-4 catalyst, with an average error of 3.6%.展开更多
基金the National Natural Science Foundation of China (No.20206023, No.20676096)the Special Funds for MajorState Basic Research Program of China (973 Program, 2006CB202500)SINOPEC (X504029).
文摘Gas-liquid (G-L) and liquid-solid (L-S) mass transfer coefficients were characterized in a gas-liquid-solid (G-L-S) three-phase magnetically stabilized bed (MSB) using amorphous alloy SRNA-4 as the solid phase. Effects such as superficial liquid velocity, superficial gas velocity, magnetic strength, liquid viscosity, and particle size were investigated. Experimental results indicated that the G-L volumetric mass transfer coefficients (KLa) increased along with the magnetic strength, superficial gas and liquid velocities. Proper increase of liquid viscosity promoted KLa only in the range of lower liquid viscosity. The external magnetic field made L-S mass transfer coefficients (Ks) in the G-L-S MSB lower than those of conventional fluidized beds. Ks in the MSB almost kept constant as the su- perficial liquid velocity and superficial gas velocity increased and decreased with the liquid viscosity and surface tension, while increased with the particle size Ks showed uniform axial and radial distributions except of small de- creases close to the wall. Dimensionless correlations were established to estimate KLa and Ks of the MSB with SRNA-4 catalysts , which showed the average error of 5.4% and 2.5% respectively.
文摘Liquid-solid （L-S） mass transfer coefficients （Ks） were characterized in a gas-liquid-solid （G-L-S） three-phase countercurrent magnetically stabilized bed （MSB） using amorphous alloy SRNA-4 as the solid phase. Effects of superficial liquid velocity, superficial gas velocity, magnetic field strength, liquid viscosity and surface tension were investigated. Experimental results indicated that the external magnetic field increased Ks in three-phase MSB, as compared to those in conventional G-L-S fluidized beds; that Ks increased with magnetic field strength, superficial gas and liquid velocities and decreased with liquid viscosity and surface tension; and that Ks showed uniform axial and radial distributions except for small increases close to the wall. Dimensionless correlations were established to estimate Ks of the G-L-S countercurrent MSB using SRNA-4 catalyst, with an average error of 3.6%.
