Aerosol indirect effects (AIEs) on global climate were quantitatively investigated by introducing aerosol–cloud interaction parameterizations for water stratus clouds into an AGCM (BCC AGCM2.0.1), which was devel...Aerosol indirect effects (AIEs) on global climate were quantitatively investigated by introducing aerosol–cloud interaction parameterizations for water stratus clouds into an AGCM (BCC AGCM2.0.1), which was developed by the National Climate Center of the China Meteorological Administration. The study yielded a global annual mean of -1.14 W m^-2 for the first indirect radiative forcing (IRF), with an obvious seasonal change. In summer, large forcing mainly occurred in mid to high latitudes of the Northern Hemisphere, whereas in winter, large values were found at 60°S. The second indirect effect led to global annual mean changes in net shortwave flux of -1.03 W m^-2 at the top of the atmosphere (TOA), which was relatively significant in mid-latitude regions of both hemispheres. The total AIE reduced the global annual means of net shortwave flux at the TOA and of surface temperature by 1.93 W m^-2 and 0.12 K, respectively. Change in surface temperature induced by the total AIE was clearly larger in the Northern Hemisphere (-0.23 K) than in the Southern Hemisphere, where changes were negligible. The interhemispheric asymmetry in surface cooling resulted in significant differences in changes of the interhemispheric annual mean precipitation rate, which could lead to a tendency for the ITCZ to broaden. The total AIE decreased the global annual mean precipitation rate by 0.055 mm df^-1.展开更多
The deployment of the U.S. Atmospheric Radiation Measurement mobile facility in Shouxian from May to December 2008 amassed the most comprehensive set of measurements of atmospheric, surface, aerosol, and cloud variabl...The deployment of the U.S. Atmospheric Radiation Measurement mobile facility in Shouxian from May to December 2008 amassed the most comprehensive set of measurements of atmospheric, surface, aerosol, and cloud variables in China. This deployment provided a unique opportunity to investigate the aerosol-cloud interactions, which are most challenging and, to date, have not been examined to any great degree in China. The relationship between cloud droplet effective radius (CER) and aerosol index (AI) is very weak in summer because the cloud droplet growth is least affected by the competition for water vapor. Mean cloud liquid water path (LWP) and cloud optical depth (COD) significantly increase with increasing AI in fall. The sensitivities of CER and LWP to aerosol loading increases are not significantly different under different air mass conditions. There is a significant correlation between the changes in hourly mean AI and the changes in hourly mean CER, LWP, and COD. The aerosol first indirect effect (FIE) is estimated in terms of relative changes in both CER (FIEcER) and COD (FIEcoD) with changes in AI for different seasons and air masses. FIEcoD and FIEcER are similar in magnitude and close to the typical FIE value of - 0.23, and do not change much between summer and fall or between the two different air mass conditions. Similar analyses were done using spaceborne Moderate Resolution Imaging Spectroradiometer data. The satellite-derived FIE is contrary to the FIE estimated from surface retrievals and may have large uncertainties due to some inherent limitations.展开更多
This study investigated the second indirect climatic effect of anthropogenic aerosols,including sulfate,organic carbon(OC) ,and black carbon(BC) ,over East Asia.The seasonal variation of the climatic response to the s...This study investigated the second indirect climatic effect of anthropogenic aerosols,including sulfate,organic carbon(OC) ,and black carbon(BC) ,over East Asia.The seasonal variation of the climatic response to the second indirect effect was also characterized.The simulation period for this study was 2006.Due to a decrease in autoconversion rate from cloud water to rain as a result of aerosols,the cloud liquid water path(LWP) ,and radiative flux(RF) at the top of the atmosphere(TOA) changed dramatically,increasing by 14.3 g m-2 and decreasing by-4.1 W m-2 in terms of domain and annual average.Both LWP and RF changed most in autumn. There were strong decreases in ground temperature in Southwest China,the middle reaches of the Yangtze River in spring and autumn,while maximum cooling of up to-1.5 K occurred in the Chongqing district.The regional and annual mean change in ground temperature reached-0.2 K over eastern China.In all seasons except summer,precipitation generally decreased in most areas north of the Yangtze River,whereas precipitation changed little in South China.Precipitation changed most in summer,with alternating bands of increasing(~40 mm) and decreasing(~40 mm) precipitation appearing in eastern China.Precipitation decreased by 1.5-40 mm over large areas of Northeast China and the Huabei Plain.The domain and annual mean change in precipitation was approximately-0.3 mm over eastern China.The maximum reduction in precipitation occurred in summer,with mean absolute and relative changes of-1.2 mm and-3.8%over eastern China.This study revealed considerable climate responses to the second indirect effect of aerosols over specific regions of China.展开更多
Aerosol indirect effects on warm clouds are estimated in the Grid-point Atmospheric Model of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics,Institute of Atmosphe...Aerosol indirect effects on warm clouds are estimated in the Grid-point Atmospheric Model of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics,Institute of Atmospheric Physics(IAP LASG)(GAMIL) with a new two-moment cloud microphysics scheme using two different physically-based aerosol activation parameterizations:Abdul-Razzak and Ghan,and Nenes and Seinfeld.The annual global mean changes in shortwave cloud forcing from preindustrial times to present day(a measure of the aerosol indirect effects) estimated from these two parameterizations are remarkably similar:0.76 W m?2 with the Abdul-Razzak and Ghan parameterization,and 0.78 W m?2 with the Nenes and Seinfeld parameterization.Physically-based parameterizations can provide robust representations of aerosol effects on droplet nucleation,meaning that aerosol activation is no longer the most uncertain factor in modeling aerosol indirect effects.展开更多
Drastic reduction in biodiversity has been a severe threat to ecosystems,which is exacerbated when losing few species leads to disastrous and even irreparable consequences.Therefore,revealing the mechanism underlying ...Drastic reduction in biodiversity has been a severe threat to ecosystems,which is exacerbated when losing few species leads to disastrous and even irreparable consequences.Therefore,revealing the mechanism underlying biodiversity loss is of uttermost importance.In this study,we show that abundant indirect interactions among mutualistic ecosystems are critical in determining species’status.Combining topological and ecological characteristics,we propose an indicator derived from a dynamic model to identify keystone species and quantify their influence,which outperforms widely-used indicators like degree in realistic and simulated networks.Furthermore,we demonstrate that networks with high modularity,heterogeneity,biodiversity,and less intimate interactions tend to have larger indirect effects,which are more amenable in predicting decline of biodiversity with the proposed indicator.These findings shed some light onto the influence of apposite biodiversities,paving the way from complex network theory to ecosystem protection and restoration.展开更多
Drastic reduction in biodiversity has been a severe threat to ecosystems,which is exacerbated when losing few species leads to disastrous and even irreparable consequences.Therefore,revealing the mechanism underlying ...Drastic reduction in biodiversity has been a severe threat to ecosystems,which is exacerbated when losing few species leads to disastrous and even irreparable consequences.Therefore,revealing the mechanism underlying biodiversity loss is of uttermost importance.In this study,we show that abundant indirect interactions among mutualistic ecosystems are critical in determining species’status.Combining topological and ecological characteristics,we propose an indicator derived from a dynamic model to identify keystone species and quantify their influence,which outperforms widely-used indicators like degree in realistic and simulated networks.Furthermore,we demonstrate that networks with high modularity,heterogeneity,biodiversity,and less intimate interactions tend to have larger indirect effects,which are more amenable in predicting decline of biodiversity with the proposed indicator.These findings shed some light onto the influence of apposite biodiversities,paving the way from complex network theory to ecosystem protection and restoration.展开更多
The regional climate model (RegCM3) and a tropospheric atmosphere chemistry model (TACM) were coupled, thus a regional climate chemistry modeling system (RegCCMS) was constructed, which was applied to investigat...The regional climate model (RegCM3) and a tropospheric atmosphere chemistry model (TACM) were coupled, thus a regional climate chemistry modeling system (RegCCMS) was constructed, which was applied to investigate the spatial distribution of anthropogenic nitrate aerosols, indirect radiative forcing, as well as its climatic effect over China. TACM includes the thermodynamic equilibrium model ISORROPIA and a condensed gas-phase chemistry model. Investigations show that the concentration of nitrate aerosols is relatively high over North and East China with a maximum of 29μg m-3 in January and 8 μg m-3 in July. Due to the influence of air temperature on thermodynamic equilibrium, wet scavenging of precipitation and the monsoon climate, there are obvious seasonal differences in nitrate concentrations. The average indirect radiative forcing at the tropopause due to nitrate aerosols is -1.63 W m 2 in January and -2.65 W m 2 in July, respectively. In some areas, indirect radiative forcing reaches -10 W m-2. Sensitivity tests show that nitrate aerosols make the surface air temperature drop and the precipitation reduce on the national level. The mean changes in surface air temperature and precipitation are 0.13 K and -0.01 mm d-1 in January and -0.09 K and -0.11 mm d-1 in July, respectively, showing significant differences in different regions.展开更多
Atmospheric aerosols (acting as cloud condensation nuclei) can enhance the cloud droplet number concentration and reduce the cloud droplet size, and in turn affect the cloud optical depth, as well as the cloud albed...Atmospheric aerosols (acting as cloud condensation nuclei) can enhance the cloud droplet number concentration and reduce the cloud droplet size, and in turn affect the cloud optical depth, as well as the cloud albedo, and thereby exert a radiative influence on climate (the first indirect aerosol effect). In this paper, based on various relationships between cloud droplet spectral dispersion (c) and cloud droplet number concentration (Nc), we analytically derive the corresponding expressions of the cloud radiative forcing induced by changes in the cloud droplet number concentration. Further quantitative evaluation indicates that the cloud radiative forcing induced by aerosols for the different ^-Nc relationships varies from -29.1% to 25.2%, compared to the case without considering spectral dispersion (e = 0). Our results suggest that an accurate description of e - Nc relationships helps to reduce the uncertainty of the first indirect aerosol effect and advances our scientific understanding of aerosol-cloud-radiation interactions.展开更多
We propose an indirect-link-weakened mass diffusion method(IMD), by considering the indirect linkage and the source object heterogeneity effect in the mass diffusion(MD) recommendation method. Experimental results...We propose an indirect-link-weakened mass diffusion method(IMD), by considering the indirect linkage and the source object heterogeneity effect in the mass diffusion(MD) recommendation method. Experimental results on the MovieLens, Netflix, and RYM datasets show that, the IMD method greatly improves both the recommendation accuracy and diversity, compared with a heterogeneity-weakened MD method(HMD), which only considers the source object heterogeneity. Moreover, the recommendation accuracy of the cold objects is also better elevated in the IMD than the HMD method. It suggests that eliminating the redundancy induced by the indirect linkages could have a prominent effect on the recommendation efficiency in the MD method.展开更多
The influences of specific heat capacity CP, temperature step ?T, electric field step ?E, and initial electric field E1 on predicted electrocaloric(EC) temperature ?T of monodomain Ba TiO3 are examined by combini...The influences of specific heat capacity CP, temperature step ?T, electric field step ?E, and initial electric field E1 on predicted electrocaloric(EC) temperature ?T of monodomain Ba TiO3 are examined by combining the Maxwell equation and phenomenological theory. Since the procedure is similar to indirect measurement of the EC effect, the results can serve as a reference for experiments. The results suggest that(i) it is reasonable to use zero-field CP,(ii) optimized ?T should be 2 K,(iii) it is better to keep △E 〈 EC, and(iv) E1〈 EC. Here, EC is the coercive field of material.展开更多
基金financially supported by the National Basic Research Program of China(Grant No. 2006CB403707)the Public Meteorology Special Foundation of MOST (Grant Nos. GYHY200706036 and 2010CB955608), the National Key Technology R&D Program (Grant Nos. 2007BAC03A01 and 2008BAC40B02)
文摘Aerosol indirect effects (AIEs) on global climate were quantitatively investigated by introducing aerosol–cloud interaction parameterizations for water stratus clouds into an AGCM (BCC AGCM2.0.1), which was developed by the National Climate Center of the China Meteorological Administration. The study yielded a global annual mean of -1.14 W m^-2 for the first indirect radiative forcing (IRF), with an obvious seasonal change. In summer, large forcing mainly occurred in mid to high latitudes of the Northern Hemisphere, whereas in winter, large values were found at 60°S. The second indirect effect led to global annual mean changes in net shortwave flux of -1.03 W m^-2 at the top of the atmosphere (TOA), which was relatively significant in mid-latitude regions of both hemispheres. The total AIE reduced the global annual means of net shortwave flux at the TOA and of surface temperature by 1.93 W m^-2 and 0.12 K, respectively. Change in surface temperature induced by the total AIE was clearly larger in the Northern Hemisphere (-0.23 K) than in the Southern Hemisphere, where changes were negligible. The interhemispheric asymmetry in surface cooling resulted in significant differences in changes of the interhemispheric annual mean precipitation rate, which could lead to a tendency for the ITCZ to broaden. The total AIE decreased the global annual mean precipitation rate by 0.055 mm df^-1.
基金supported by the National Basic Research "973" Program of China (Grant No. 2013CB955804)a Natural Science Foundation of China research project (Grant No. 91544217)the U.S. National Science Foundation (Grant No. AGS1534670)
文摘The deployment of the U.S. Atmospheric Radiation Measurement mobile facility in Shouxian from May to December 2008 amassed the most comprehensive set of measurements of atmospheric, surface, aerosol, and cloud variables in China. This deployment provided a unique opportunity to investigate the aerosol-cloud interactions, which are most challenging and, to date, have not been examined to any great degree in China. The relationship between cloud droplet effective radius (CER) and aerosol index (AI) is very weak in summer because the cloud droplet growth is least affected by the competition for water vapor. Mean cloud liquid water path (LWP) and cloud optical depth (COD) significantly increase with increasing AI in fall. The sensitivities of CER and LWP to aerosol loading increases are not significantly different under different air mass conditions. There is a significant correlation between the changes in hourly mean AI and the changes in hourly mean CER, LWP, and COD. The aerosol first indirect effect (FIE) is estimated in terms of relative changes in both CER (FIEcER) and COD (FIEcoD) with changes in AI for different seasons and air masses. FIEcoD and FIEcER are similar in magnitude and close to the typical FIE value of - 0.23, and do not change much between summer and fall or between the two different air mass conditions. Similar analyses were done using spaceborne Moderate Resolution Imaging Spectroradiometer data. The satellite-derived FIE is contrary to the FIE estimated from surface retrievals and may have large uncertainties due to some inherent limitations.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences(Grant No. KZCX2-YW-Q11-03)the"Strategic Priority Research Program"of the Chinese Academy of Sciences(Grant No.XDA05100502)+1 种基金the R&D Special Fund for Public Welfare Industry(Meteorology) (Grant No.GYHY200906020)100 Talents Program of the Chinese Academy of Sciences
文摘This study investigated the second indirect climatic effect of anthropogenic aerosols,including sulfate,organic carbon(OC) ,and black carbon(BC) ,over East Asia.The seasonal variation of the climatic response to the second indirect effect was also characterized.The simulation period for this study was 2006.Due to a decrease in autoconversion rate from cloud water to rain as a result of aerosols,the cloud liquid water path(LWP) ,and radiative flux(RF) at the top of the atmosphere(TOA) changed dramatically,increasing by 14.3 g m-2 and decreasing by-4.1 W m-2 in terms of domain and annual average.Both LWP and RF changed most in autumn. There were strong decreases in ground temperature in Southwest China,the middle reaches of the Yangtze River in spring and autumn,while maximum cooling of up to-1.5 K occurred in the Chongqing district.The regional and annual mean change in ground temperature reached-0.2 K over eastern China.In all seasons except summer,precipitation generally decreased in most areas north of the Yangtze River,whereas precipitation changed little in South China.Precipitation changed most in summer,with alternating bands of increasing(~40 mm) and decreasing(~40 mm) precipitation appearing in eastern China.Precipitation decreased by 1.5-40 mm over large areas of Northeast China and the Huabei Plain.The domain and annual mean change in precipitation was approximately-0.3 mm over eastern China.The maximum reduction in precipitation occurred in summer,with mean absolute and relative changes of-1.2 mm and-3.8%over eastern China.This study revealed considerable climate responses to the second indirect effect of aerosols over specific regions of China.
基金supported by the National High Technology Research and Development Program of China (Grant No. 2010AA012304)the Knowledge Innovation Program of the Chinese Academy of Sciences (Grant No. KZCX2-YW-Q11-04)the China Meteorological Administration for the R&D Special Fund for Public Welfare Industry (meteorology) (Grant Nos. GYHY200806006 and GYHY200906020)
文摘Aerosol indirect effects on warm clouds are estimated in the Grid-point Atmospheric Model of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics,Institute of Atmospheric Physics(IAP LASG)(GAMIL) with a new two-moment cloud microphysics scheme using two different physically-based aerosol activation parameterizations:Abdul-Razzak and Ghan,and Nenes and Seinfeld.The annual global mean changes in shortwave cloud forcing from preindustrial times to present day(a measure of the aerosol indirect effects) estimated from these two parameterizations are remarkably similar:0.76 W m?2 with the Abdul-Razzak and Ghan parameterization,and 0.78 W m?2 with the Nenes and Seinfeld parameterization.Physically-based parameterizations can provide robust representations of aerosol effects on droplet nucleation,meaning that aerosol activation is no longer the most uncertain factor in modeling aerosol indirect effects.
基金supported in part by the National Natural Science Foundation of China(U2141235 and 61803166)National Natural Science Foundation of Hubei Province(2019CFA005).
文摘Drastic reduction in biodiversity has been a severe threat to ecosystems,which is exacerbated when losing few species leads to disastrous and even irreparable consequences.Therefore,revealing the mechanism underlying biodiversity loss is of uttermost importance.In this study,we show that abundant indirect interactions among mutualistic ecosystems are critical in determining species’status.Combining topological and ecological characteristics,we propose an indicator derived from a dynamic model to identify keystone species and quantify their influence,which outperforms widely-used indicators like degree in realistic and simulated networks.Furthermore,we demonstrate that networks with high modularity,heterogeneity,biodiversity,and less intimate interactions tend to have larger indirect effects,which are more amenable in predicting decline of biodiversity with the proposed indicator.These findings shed some light onto the influence of apposite biodiversities,paving the way from complex network theory to ecosystem protection and restoration.
基金supported in part by the National Natural Science Foundation of China(U2141235 and 61803166)National Natural Science Foundation of Hubei Province(2019CFA005)。
文摘Drastic reduction in biodiversity has been a severe threat to ecosystems,which is exacerbated when losing few species leads to disastrous and even irreparable consequences.Therefore,revealing the mechanism underlying biodiversity loss is of uttermost importance.In this study,we show that abundant indirect interactions among mutualistic ecosystems are critical in determining species’status.Combining topological and ecological characteristics,we propose an indicator derived from a dynamic model to identify keystone species and quantify their influence,which outperforms widely-used indicators like degree in realistic and simulated networks.Furthermore,we demonstrate that networks with high modularity,heterogeneity,biodiversity,and less intimate interactions tend to have larger indirect effects,which are more amenable in predicting decline of biodiversity with the proposed indicator.These findings shed some light onto the influence of apposite biodiversities,paving the way from complex network theory to ecosystem protection and restoration.
基金supported by the National Basic Research Program of China (Grant Nos. 2006CB403706 and 2006CB403703)the National Science and Technology Support Program (Grant No.2007BAC03A01)the Jiangsu Natural Science Foundation (Grant No. BK2006515)
文摘The regional climate model (RegCM3) and a tropospheric atmosphere chemistry model (TACM) were coupled, thus a regional climate chemistry modeling system (RegCCMS) was constructed, which was applied to investigate the spatial distribution of anthropogenic nitrate aerosols, indirect radiative forcing, as well as its climatic effect over China. TACM includes the thermodynamic equilibrium model ISORROPIA and a condensed gas-phase chemistry model. Investigations show that the concentration of nitrate aerosols is relatively high over North and East China with a maximum of 29μg m-3 in January and 8 μg m-3 in July. Due to the influence of air temperature on thermodynamic equilibrium, wet scavenging of precipitation and the monsoon climate, there are obvious seasonal differences in nitrate concentrations. The average indirect radiative forcing at the tropopause due to nitrate aerosols is -1.63 W m 2 in January and -2.65 W m 2 in July, respectively. In some areas, indirect radiative forcing reaches -10 W m-2. Sensitivity tests show that nitrate aerosols make the surface air temperature drop and the precipitation reduce on the national level. The mean changes in surface air temperature and precipitation are 0.13 K and -0.01 mm d-1 in January and -0.09 K and -0.11 mm d-1 in July, respectively, showing significant differences in different regions.
基金jointly supported by the National Natural Science Foundation of China (Grant No. 41105071)the CAS Strategic Priority Research Program (Grant No. XDA05110101)the National Basic Research Program of China (Grant No. 2011CB403406)
文摘Atmospheric aerosols (acting as cloud condensation nuclei) can enhance the cloud droplet number concentration and reduce the cloud droplet size, and in turn affect the cloud optical depth, as well as the cloud albedo, and thereby exert a radiative influence on climate (the first indirect aerosol effect). In this paper, based on various relationships between cloud droplet spectral dispersion (c) and cloud droplet number concentration (Nc), we analytically derive the corresponding expressions of the cloud radiative forcing induced by changes in the cloud droplet number concentration. Further quantitative evaluation indicates that the cloud radiative forcing induced by aerosols for the different ^-Nc relationships varies from -29.1% to 25.2%, compared to the case without considering spectral dispersion (e = 0). Our results suggest that an accurate description of e - Nc relationships helps to reduce the uncertainty of the first indirect aerosol effect and advances our scientific understanding of aerosol-cloud-radiation interactions.
基金Project supported by the National Natural Science Foundation of China(Grant No.11175079)the Young Scientist Training Project of Jiangxi Province,China(Grant No.20133BCB23017)
文摘We propose an indirect-link-weakened mass diffusion method(IMD), by considering the indirect linkage and the source object heterogeneity effect in the mass diffusion(MD) recommendation method. Experimental results on the MovieLens, Netflix, and RYM datasets show that, the IMD method greatly improves both the recommendation accuracy and diversity, compared with a heterogeneity-weakened MD method(HMD), which only considers the source object heterogeneity. Moreover, the recommendation accuracy of the cold objects is also better elevated in the IMD than the HMD method. It suggests that eliminating the redundancy induced by the indirect linkages could have a prominent effect on the recommendation efficiency in the MD method.
基金Project supported by the Natural Science Foundation of Shanghai,China(Grant No.17ZR1447200)
文摘The influences of specific heat capacity CP, temperature step ?T, electric field step ?E, and initial electric field E1 on predicted electrocaloric(EC) temperature ?T of monodomain Ba TiO3 are examined by combining the Maxwell equation and phenomenological theory. Since the procedure is similar to indirect measurement of the EC effect, the results can serve as a reference for experiments. The results suggest that(i) it is reasonable to use zero-field CP,(ii) optimized ?T should be 2 K,(iii) it is better to keep △E 〈 EC, and(iv) E1〈 EC. Here, EC is the coercive field of material.