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Self-Mixing Interference Effects in LD Pumped Multi-Mode Solid-State Laser 被引量:2
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作者 张勇 姚建铨 +2 位作者 王鹏 禹延光 陈进 《Transactions of Tianjin University》 EI CAS 2003年第4期261-263,共3页
Based on the effective structure of the self-mixing interference effects,a general model for the self-mixing interference effects in the LD pumped solid-state laser has been established for the first time.The numerica... Based on the effective structure of the self-mixing interference effects,a general model for the self-mixing interference effects in the LD pumped solid-state laser has been established for the first time.The numerical simulation of the self-mixing interference signal has been done,the results show that when the external cavity length is integral times of 1/2,1/3,2/3,1/4,3/4 of the effective cavity length,the intensity of the self-mixing interference signals reach maximum in value.While that of single mode laser is integral times of half of the effective cavity length,the measuring precision of displacement of single mode laser is λ/2.A conclusion can be drawn from the above results that the measuring precision of displacement of multi-mode laser is higher than that of single mode laser. 展开更多
关键词 general model self-mixing interference effects LD pumped multi-mode solid-state laser numerical simulations
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Analytical modelling of end thermal coupling in a solid-state laser longitudinally bonded by a vertical-cavity top-emitting laser diode
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作者 吴坚 H.D.Summers 《Chinese Physics B》 SCIE EI CAS CSCD 2009年第11期4912-4918,共7页
The intrinsic features involving a circularly symmetric beam profile with low divergence, planar geometry as well as the increasingly enhanced power of vertical-cavity surface-emitting lasers (VCSELs) have made the ... The intrinsic features involving a circularly symmetric beam profile with low divergence, planar geometry as well as the increasingly enhanced power of vertical-cavity surface-emitting lasers (VCSELs) have made the VCSEL a promising pump source in direct end bonding to a solid-state laser medium to form the minimized, on-wafer integrated laser system. This scheme will generate a surface contact pump configuration and thus additional end thermal coupling to the laser medium through the joint interface of both materials, apart from pump beam heating. This paper analytically models temperature distributions in both VCSEL and the laser medium from the end thermal coupling regarding surface contact pump configuration using a top-emitting VCSEL as the pump source for the first time. The analytical solutions are derived by introducing relative temperature and mean temperature expressions. The results show that the end contact heating by the VCSEL could lead to considerable temperature variations associated with thermal phase shift and thermal lensing in the laser medium. However, if the central temperature of the interface is increased by less than 20 K, the end contact heating does not have a significant thermal influence on the laser medium. In this case, the thermal effect should be dominated by pump beam heating. This work provides useful analytical results for further analysis of hybrid thermal effects on those lasers pumped by a direct VCSEL bond. 展开更多
关键词 solid-state laser end pump thermal coupling vertical-cavity surface-emitting laser
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High-Power Continuous-Wave Nd:GdVO4 Solid-State Laser Dual-End-Pumped at 880 nm
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作者 毛叶飞 张恒利 +5 位作者 桑思晗 张新 余西龙 邢冀川 辛建国 江毅 《Chinese Physics Letters》 SCIE CAS CSCD 2015年第9期43-45,共3页
A high-power cw all-solid-state Nd:GdVO4 laser operating at 88Onto is reported. The laser consists of a low doped level Nd:GdV04 crystal dual-end-pumped by two high-power diode lasers and a compact negative confocM ... A high-power cw all-solid-state Nd:GdVO4 laser operating at 88Onto is reported. The laser consists of a low doped level Nd:GdV04 crystal dual-end-pumped by two high-power diode lasers and a compact negative confocM unstable-stable hybrid resonator. At an incident pump power of 820 W, a maximum cw output of 240 W at 1064nm is obtained. The optical-to-optical efficiency and Mope efficiency are 40.7% and 53.2%, respectively. The M2 factors in the unstable direction and in the stable direction are 4.38 and 5.44, respectively. 展开更多
关键词 Nd High-Power Continuous-Wave Nd:GdVO4 solid-state laser Dual-End-Pumped at 880 nm
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Self-Starting Passively Mode-Locking All-Solid-State Laser with GaAs Absorber Grown at Low Temperature 被引量:2
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作者 贾玉磊 令维军 +2 位作者 魏志义 王勇刚 马骁宇 《Chinese Physics Letters》 SCIE CAS CSCD 2005年第10期2575-2577,共3页
We realize a stable self-starting passively mode-locking all-solid-state laser by using novel GaAs mirrors as the absorber and output coupler. The GaAs mirror is grown by the technology of metal organic chemical vapou... We realize a stable self-starting passively mode-locking all-solid-state laser by using novel GaAs mirrors as the absorber and output coupler. The GaAs mirror is grown by the technology of metal organic chemical vapour deposition at low temperature. With such an absorber as the output coupler in the laser resonator, laser pulses with duration of 42ps were generated at a repetition rate of 400MHz, corresponding to the average power of 590mW. 展开更多
关键词 SEMICONDUCTOR SATURABLE ABSORBERS ND-YLF laserS ND-GDVO4 laser YAG laser MIRROR ND-YVO4
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Novel Single-Frequency Diode Pumped Solid-State Lasers and Their Applications in Laser Ranging and Velocimetry 被引量:1
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作者 YANG Su-Hui WU Ke-Ying WEI Guang-Hui 《Chinese Physics Letters》 SCIE CAS CSCD 2001年第7期906-908,共3页
Two models of laser diode pumped unidirectional single-frequency ring laser with maximum single frequency output power of 1 W and 780 mW are investigated.The Statistic linewidth of the free-run laser is measured to be... Two models of laser diode pumped unidirectional single-frequency ring laser with maximum single frequency output power of 1 W and 780 mW are investigated.The Statistic linewidth of the free-run laser is measured to be 2.1 kHz within 5μs by using a single mode fiber link.We use the monolithic laser to measure the angular speed of a spinning motor and simulate a linearly frequency modulated continuous-wave ladar system in laboratory. 展开更多
关键词 PUMPED laser FIBER
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Periodic adjustment of the position of a laser beam spot on a semiconductor saturable absorber mirror in a passively mode-locked solid-state laser
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作者 夏帕克提 闫平 巩马理 《Chinese Physics B》 SCIE EI CAS CSCD 2011年第9期211-215,共5页
A laser diode end-pumped passively mode-locked Nd:YVO4 solid-state laser with a semiconductor saturable ab- sorber mirror (SESAM), in which the intracavity laser beam spot on the SESAM can be adjusted periodically,... A laser diode end-pumped passively mode-locked Nd:YVO4 solid-state laser with a semiconductor saturable ab- sorber mirror (SESAM), in which the intracavity laser beam spot on the SESAM can be adjusted periodically, is investigated. Inserting a rectangular prism (RP) into the laser cavity is a promising approach towards the goal of periodically moving the position of the focus spot of the intracavity pulse on the SESAM surface to avoid the long-time irradiation of the laser beam on the same position, thereby solving a series of problems caused by damage to the SESAM and greatly prolonging its usage life. The adjustment of the rectangular prism in the laser cavity does not break the stable continuous wave (CW) mode-locked condition. The laser generates a stable picosecond pulse sequence at 1064 nm with an output power of 3.6 W and a pulse width of 14 ps. The instabilities of the output power and the pulse width are 1.77% and 4.5%, respectively. 展开更多
关键词 mode-locked laser rectangular prism Nd:YV04 semiconductor saturable absorber mir-ror
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Research on All-solid-state Laser and Its Industrial Development in China
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作者 SHIZhao-hui ZHANGJing FANZhong-wei 《光机电信息》 2005年第4期1-8,共8页
Some typical applications of solid-state laser are described, and its industrial development in China are also introduced in detail.
关键词 全固体激光器 中国 产业 DPL 锁模激光器
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Single Pass Third-Harmonic Generation of 310mW of 355 nm with an All-Solid-State Laser
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作者 JIA Yu-Lei HE Jing-Liang +2 位作者 WANG Hui-Tian ZHU Shi-Ning ZHU Yong-Yuan 《Chinese Physics Letters》 SCIE CAS CSCD 2001年第12期1589-1591,共3页
A maximum of 310mW average output power at 355nm has been obtained by extracavity frequency tripling with a BBO crystal in a Q-switched Nd:YV04 laser with 11.2 W of laser diode pump power. The single pass frequency co... A maximum of 310mW average output power at 355nm has been obtained by extracavity frequency tripling with a BBO crystal in a Q-switched Nd:YV04 laser with 11.2 W of laser diode pump power. The single pass frequency conversion efficiency (infrared-to-ultraviolet) is 14.3%. The power stability of the ultraviolet laser is better than 1% in 30min. 展开更多
关键词 laser SWITCHED Nd:
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Numerical Study of Transient Temperature Distribution in Passively Q-Switched Yb:YAG Solid-State Laser
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作者 Jala M. El-Azab Hamed M. Kandel +1 位作者 Mohamed A. Khedr Hatem M. El-Ghandoor 《Optics and Photonics Journal》 2014年第3期46-53,共8页
In this work, the thermal characterization of continuously pumped passively Q-switched laser is quantitatively represented. The system under investigation is end-pumped Yb:YAG passively Q-switched by Cr4+:YAG as satur... In this work, the thermal characterization of continuously pumped passively Q-switched laser is quantitatively represented. The system under investigation is end-pumped Yb:YAG passively Q-switched by Cr4+:YAG as saturable absorber. The rate equations describing the dynamics of laser action are numerically solved simultaneously with the temperature conductivity heat equation to depict the transient temperature distribution. The study has been performed in the cylindrical coordinates to characterize the temperature distribution in the axial and radial directions. The thermal transient time in both directions as well as the thermal focal length are calculated. The temporal behavior of the temperature distribution has been illustrated in a 3-dimensional diagram. 展开更多
关键词 Q-SWITCHED laser Temperature DISTRIBUTION Thermal LENSING
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Pushing the boundaries of diode-pumped solid-state lasers for high-energy applications 被引量:4
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作者 Saumyabrata Banerjee Paul Mason +10 位作者 Jonathan Phillips Jodie Smith Thomas Butcher Jacob Spear Mariastefania De Vido Gary Quinn Danielle Clarke Klaus Ertel Cristina Hernez-Gomez Chris Edwards John Collier 《High Power Laser Science and Engineering》 SCIE CAS CSCD 2020年第2期77-79,共3页
We report on the successful demonstration of a 150 J nanosecond pulsed cryogenic gas cooled,diode-pumped multi-slab Yb:YAG laser operating at 1 Hz.To the best of our knowledge,this is the highest energy ever recorded ... We report on the successful demonstration of a 150 J nanosecond pulsed cryogenic gas cooled,diode-pumped multi-slab Yb:YAG laser operating at 1 Hz.To the best of our knowledge,this is the highest energy ever recorded for a diodepumped laser system. 展开更多
关键词 cryogenic gas cooling diode-pumped solid-state laser multi-slab amplifier YB:YAG
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Two-dimensional tellurium saturable absorber for ultrafast solid-state laser 被引量:2
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作者 Zixin Yang Lili Han +10 位作者 Qi Yang Xianghe Ren Syed Zaheer Ud Din Xiaoyan Zhang Jiancai Leng Jiabao Zhang Baitao Zhang Kejian Yang Jingliang He Chunlong Li Jun Wang 《Chinese Optics Letters》 SCIE EI CAS CSCD 2021年第3期64-68,共5页
Two-dimensional(2 D) Te nanosheets were successfully fabricated through the liquid-phase exfoliation(LPE) method. The nonlinear optical properties of 2 D Te nanosheets were studied by the open-aperture Z-scan techniqu... Two-dimensional(2 D) Te nanosheets were successfully fabricated through the liquid-phase exfoliation(LPE) method. The nonlinear optical properties of 2 D Te nanosheets were studied by the open-aperture Z-scan technique. Furthermore, the continuous wave mode-locked Nd:YVO4 laser was successfully realized by using 2 D Te as a saturable absorber(SA) for the first time, to the best of our knowledge. Ultrashort pulses as short as 5.8 ps were obtained at 1064.3 nm with an output power of 851 m W. This primary investigation indicates that the 2 D Te SA is a promising photonic device in the fields of ultrafast solid-state lasers. 展开更多
关键词 TELLURIUM Z-SCAN saturable absorber ultrafast solid-state laser
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Ce:GdYAG phosphor-in-glass:An innovative yellow-emitting color converter for solid-state laser lighting 被引量:2
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作者 Luhan Wang Jiangdan Zhang +5 位作者 Li Xu Shuyang Bao Yu Wang Jiawei Liu Xiaojuan Liang Weidong Xiang 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2023年第3期42-49,共8页
Stable,efficient and high color rendering index all-inorganic color converters are urgently demanded for white laser diodes.Phosphor-in-glass(PiG),possessing the advantages of phosphors excellent quantum efficiency as... Stable,efficient and high color rendering index all-inorganic color converters are urgently demanded for white laser diodes.Phosphor-in-glass(PiG),possessing the advantages of phosphors excellent quantum efficiency as well as favorable chemical and thermal stability of glass,has attracted widespread attention.There have been only very few reports of Y_(1.31)Ce_(0.09)Gd_(1.6)Al_(5)O_(12)(Ce:GdYAG)PiG for solid-state laser light-ing.Herein,a series of Ce:GdYAG PiG samples are fabricated by a simple solid-state sintering method.Impressively,the supreme internal quantum efficiency of as-prepared PiG is 91%,which is very close to original phosphors(95%).Furthermore,PiG exhibits a high thermal conductivity(1.844 W m^(−1)K^(−1))and a maximum transparency(62%).Remarkably,by changing the concentration of phosphors and the thickness of PiG samples,a luminous efficacy of 163.5 lm/W,high color rendering index of 74.8 and low correlated color temperature of 4806.8 K are achieved under blue laser irradiation.These results indicate that the Ce:GdYAG PiG samples have shown tremendous application foreground as all-inorganic color converter for solid-state laser lighting. 展开更多
关键词 Ce:GdYAG Phosphor-in-glass solid-state laser lighting Optical performance
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Passively Q-switched tri-wavelength Yb3+:GdAl3(BO3)4 solid-state laser with topological insulator Bi2Te3 as saturable absorber 被引量:2
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作者 Yi-Jian Sun Chao-Kuei Lee +6 位作者 Jin-Long Xu Zhao-Jie Zhu Ye-Qing Wang Shu-Fang Gao Hou-Ping Xia Zhen-Yu You Chao-Yang Tu 《Photonics Research》 SCIE EI 2015年第3期97-101,共5页
In this paper,we reported a multiwavelength passively Q-switched Yb3+:GdAl3(BO3)4 solid-state laser with topological insulator Bi2Te3 as a saturable absorber(SA) for the first time,to the best of our knowledge.Bi2... In this paper,we reported a multiwavelength passively Q-switched Yb3+:GdAl3(BO3)4 solid-state laser with topological insulator Bi2Te3 as a saturable absorber(SA) for the first time,to the best of our knowledge.Bi2Te3 nanosheets were prepared by the facile solvothermal method.The influence of three Bi2Te3 densities on the laser operation was compared.The maximum average output power was up to 57 mW with a pulse energy of 511.7 nJ.The shortest pulsewidth was measured to be 370 ns with 110 kHz pulse repetition rate and 40 mW average power.The laser operated at three wavelengths simultaneously at 1043.7,1045.3,and 1046.2 nm,of which the frequency differences were within the terahertz wave band.Our work suggests that solvothermal synthesized Bi2Te3 is a promising SA for simultaneously multiwavelength laser operation. 展开更多
关键词 Passively Q-switched tri-wavelength Yb BO3 Te GdAl3 solid-state laser with topological insulator Bi2Te3 as saturable absorber TISA Bi
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Watt-level broadly wavelength tunable mode-locked solid-state laser in the 2 μm water absorption region 被引量:5
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作者 WEI ZHOU XIAODONG XU +5 位作者 RUI XU XULIANG FAN YONGGUANG ZHAO LEI LI DINGYUAN TANG DEYUAN SHEN 《Photonics Research》 SCIE EI 2017年第6期102-106,共5页
We report on broadly wavelength-tunable passive mode-locking with high power operating at the 2 μm water absorption band in a Tm:CYA crystal laser. With a simple quartz plate, stable mode-locking wavelengths can be t... We report on broadly wavelength-tunable passive mode-locking with high power operating at the 2 μm water absorption band in a Tm:CYA crystal laser. With a simple quartz plate, stable mode-locking wavelengths can be tuned from 1874 to 1973 nm, with a tunable wavelength range up to ~100 nm and maximum output power up to 1.35 W. The bandwidth is narrow as ~6 GHz, corresponding to a high coherence. To our knowledge, this is the first demonstration of wavelength-tunable mode-locking with watt-level in the 2 μm water absorption band.The high temporal coherent laser can be further applied in spectroscopy, the efficient excitation of molecules, sensing, and quantum optics. 展开更多
关键词 Watt-level broadly wavelength tunable mode-locked solid-state laser in the 2
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Band-gap modulation of two-dimensional saturable absorbers for solid-state lasers 被引量:1
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作者 Shuxian Wang Haohai Yu Huaijin Zhang 《Photonics Research》 SCIE EI 2015年第2期10-20,共11页
Due to the manifestation of fascinating physical phenomena and materials science, two-dimensional(2D) materials have recently attracted enormous research interest with respect to the fields of electronics and optoel... Due to the manifestation of fascinating physical phenomena and materials science, two-dimensional(2D) materials have recently attracted enormous research interest with respect to the fields of electronics and optoelectronics.There have been in-depth investigations of the nonlinear properties with respect to saturable absorption, and many 2D materials show potential application in optical switches for passive pulsed lasers. However, the Eigen band-gap determines the responding wavelength band and constrains the applications. In this paper, based on band-gap engineering, some different types of 2D broadband saturable absorbers are reviewed in detail, including molybdenum disulfide(MoS2), vanadium dioxide(VO2), graphene, and the Bi2Se3 topological insulator. The results suggest that the band-gap modification should play important roles in 2D broadband saturable materials and can provide some inspiration for the exploration and design of 2D nanodevices. 展开更多
关键词 MO Band-gap modulation of two-dimensional saturable absorbers for solid-state lasers
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Photo-physical Characterisation of Novel Organic Dye-doped Solid-state Laser Materials
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作者 A.Penzkofer A.Tyagi +5 位作者 T.Susdorf D.del Agua O.García R.Sastre A.Costela I.García-Moreno 《复旦学报(自然科学版)》 CAS CSCD 北大核心 2007年第5期593-,共1页
1 Results The development of tuneable solid-state organic dye lasers is a subject of considerable interest and research activity.Compared to conventional liquid dye lasers they have the advantage of being free of solv... 1 Results The development of tuneable solid-state organic dye lasers is a subject of considerable interest and research activity.Compared to conventional liquid dye lasers they have the advantage of being free of solvent handling,having small size,and being easy to operate.For high-performance solid-state dye lasers highly photo-stable dyes with low quantum yield of triplet formation and low triplet-triplet absorption cross-section in the lasing wavelength region are required.For solid state dye lasers ... 展开更多
关键词 pyrromethene dye PM597 solid-state laser dye characterisation polymer matrices
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High-power passively Q-switched 2 μm all-solid-state laser based on a Bi_2Te_3 saturable absorber 被引量:6
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作者 X.LIU K.YANG +9 位作者 S.ZHAO T.LI W.QIAO H.ZHANG B.ZHANG J.HE J.BIAN L.ZHENG L.SU J.XU 《Photonics Research》 SCIE EI 2017年第5期461-466,共6页
By using the ultrasound-assisted liquid phase exfoliation method, Bi_2Te_3 nanosheets are synthesized and deposited onto a quartz plate to form a kind of saturable absorber(SA), in which nonlinear absorption propertie... By using the ultrasound-assisted liquid phase exfoliation method, Bi_2Te_3 nanosheets are synthesized and deposited onto a quartz plate to form a kind of saturable absorber(SA), in which nonlinear absorption properties around 2 μm are analyzed with a home-made mode-locked laser. With the as-prepared Bi_2Te_3 SA employed,a stable passively Q-switched all-solid-state 2 μm laser is successfully realized. Q-switched pulses with a maximum average output power of 2.03 W are generated under an output coupling of 5%, corresponding to the maximum single-pulse energy of 18.4 μJ and peak power of 23 W. The delivered shortest pulse duration and maximum repetition rate are 620 ns and 118 k Hz under an output coupling of 2%, respectively. It is the first presentation of such Bi_2Te_3 SA employed in a solid-state Q-switched crystalline laser at 2 μm, to the best of our knowledge. In comparison with other 2 D materials suitable for pulsed 2 μm lasers, the saturable absorption performance of Bi_2Te_3 SA is proved to be promising in generating high power and high-repetition-rate 2 μm laser pulses. 展开更多
关键词 Te SA m all-solid-state laser based on a Bi2Te3 saturable absorber High-power passively Q-switched 2 BI
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12.6μm-Thick Asymmetric Composite Electrolyte with Superior Interfacial Stability for Solid-State Lithium-Metal Batteries 被引量:3
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作者 Zheng Zhang Jingren Gou +4 位作者 Kaixuan Cui Xin Zhang Yujian Yao Suqing Wang Haihui Wang 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第9期397-409,共13页
Solid-state lithium metal batteries(SSLMBs)show great promise in terms of high-energy-density and high-safety performance.However,there is an urgent need to address the compatibility of electrolytes with high-voltage ... Solid-state lithium metal batteries(SSLMBs)show great promise in terms of high-energy-density and high-safety performance.However,there is an urgent need to address the compatibility of electrolytes with high-voltage cathodes/Li anodes,and to minimize the electrolyte thickness to achieve highenergy-density of SSLMBs.Herein,we develop an ultrathin(12.6μm)asymmetric composite solid-state electrolyte with ultralight areal density(1.69 mg cm^(−2))for SSLMBs.The electrolyte combining a garnet(LLZO)layer and a metal organic framework(MOF)layer,which are fabricated on both sides of the polyethylene(PE)separator separately by tape casting.The PE separator endows the electrolyte with flexibility and excellent mechanical properties.The LLZO layer on the cathode side ensures high chemical stability at high voltage.The MOF layer on the anode side achieves a stable electric field and uniform Li flux,thus promoting uniform Li^(+)deposition.Thanks to the well-designed structure,the Li symmetric battery exhibits an ultralong cycle life(5000 h),and high-voltage SSLMBs achieve stable cycle performance.The assembled pouch cells provided a gravimetric/volume energy density of 344.0 Wh kg^(−1)/773.1 Wh L^(−1).This simple operation allows for large-scale preparation,and the design concept of ultrathin asymmetric structure also reveals the future development direction of SSLMBs. 展开更多
关键词 solid-state lithium metal batteries Composite solid-state electrolyte Ultrathin asymmetric structure Pouch cells
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Advances in All-Solid-State Lithium-Sulfur Batteries for Commercialization 被引量:2
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作者 Birhanu Bayissa Gicha Lemma Teshome Tufa +2 位作者 Njemuwa Nwaji Xiaojun Hu Jaebeom Lee 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第9期209-246,共38页
Solid-state batteries are commonly acknowledged as the forthcoming evolution in energy storage technologies.Recent development progress for these rechargeable batteries has notably accelerated their trajectory toward ... Solid-state batteries are commonly acknowledged as the forthcoming evolution in energy storage technologies.Recent development progress for these rechargeable batteries has notably accelerated their trajectory toward achieving commercial feasibility.In particular,all-solid-state lithium-sulfur batteries(ASSLSBs)that rely on lithium-sulfur reversible redox processes exhibit immense potential as an energy storage system,surpassing conventional lithium-ion batteries.This can be attributed predominantly to their exceptional energy density,extended operational lifespan,and heightened safety attributes.Despite these advantages,the adoption of ASSLSBs in the commercial sector has been sluggish.To expedite research and development in this particular area,this article provides a thorough review of the current state of ASSLSBs.We delve into an in-depth analysis of the rationale behind transitioning to ASSLSBs,explore the fundamental scientific principles involved,and provide a comprehensive evaluation of the main challenges faced by ASSLSBs.We suggest that future research in this field should prioritize plummeting the presence of inactive substances,adopting electrodes with optimum performance,minimizing interfacial resistance,and designing a scalable fabrication approach to facilitate the commercialization of ASSLSBs. 展开更多
关键词 All-solid-state lithium-sulfur batteries COMMERCIALIZATION Enhancement strategies solid-state electrolytes Sulfurbased cathodes
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How Does Stacking Pressure Affect the Performance of Solid Electrolytes and All-Solid-State Lithium Metal Batteries? 被引量:2
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作者 Junwu Sang Bin Tang +3 位作者 Yong Qiu Yongzheng Fang Kecheng Pan Zhen Zhou 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2024年第4期93-98,共6页
All-solid-state lithium metal batteries(ASSLMBs)with solid electrolytes(SEs)have emerged as a promising alternative to liquid electrolyte-based Li-ion batteries due to their higher energy density and safety.However,si... All-solid-state lithium metal batteries(ASSLMBs)with solid electrolytes(SEs)have emerged as a promising alternative to liquid electrolyte-based Li-ion batteries due to their higher energy density and safety.However,since ASSLMBs lack the wetting properties of liquid electrolytes,they require stacking pressure to prevent contact loss between electrodes and SEs.Though previous studies showed that stacking pressure could impact certain performance aspects,a comprehensive investigation into the effects of stacking pressure has not been conducted.To address this gap,we utilized the Li_(6)PS_(5)Cl solid electrolyte as a reference and investigated the effects of stacking pressures on the performance of SEs and ASSLMBs.We also developed models to explain the underlying origin of these effects and predict battery performance,such as ionic conductivity and critical current density.Our results demonstrated that an appropriate stacking pressure is necessary to achieve optimal performance,and each step of applying pressure requires a specific pressure value.These findings can help explain discrepancies in the literature and provide guidance to establish standardized testing conditions and reporting benchmarks for ASSLMBs.Overall,this study contributes to the understanding of the impact of stacking pressure on the performance of ASSLMBs and highlights the importance of careful pressure optimization for optimal battery performance. 展开更多
关键词 critical current density solid electrolyte solid-state lithium metal batteries stacking pressure
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