设计了一种由1μm涡旋光泵浦的闲频光单谐振KTiOAsO_(4)涡旋光参量振荡器,并基于该光参量振荡器在近/中红外波段实现了高光束质量、高能量、窄光谱带宽的涡旋光输出。选取不同曲率半径的输入镜和平面输出镜分别建立平平腔和平凹腔两种...设计了一种由1μm涡旋光泵浦的闲频光单谐振KTiOAsO_(4)涡旋光参量振荡器,并基于该光参量振荡器在近/中红外波段实现了高光束质量、高能量、窄光谱带宽的涡旋光输出。选取不同曲率半径的输入镜和平面输出镜分别建立平平腔和平凹腔两种腔结构,基于所建结构可以控制泵浦光的轨道角动量(OAM)选择性地传递给输出的信号光或闲频光。当泵浦光最大能量为20.6 m J时,在近红外波段产生了3.04 m J的信号涡旋光(1.535μm),同时在中红外波段产生了0.82 m J的闲频涡旋光(3.468μm),它们对应的转换效率分别为28.21%和7.62%。基于泵浦光与谐振闲频光在两种腔型中的空间重叠效率,从理论上解释了泵浦光OAM的传递原理。测量得到输出信号光和闲频光的光谱带宽(半峰全宽)分别为λs=0.85 nm和λi=1.08 nm,其中闲频光在两个正交方向上的光束质量因子分别为Mx2≈2.1和My2≈2.2。展开更多
A series of tunable phosphors NaAlSiO_4：Ce^（3＋）,Sm^（3＋） were synthesized using a conventional high-temperature, solid-state method. Crystal structure, photoluminescence excitation, and emission spectra with flu...A series of tunable phosphors NaAlSiO_4：Ce^（3＋）,Sm^（3＋） were synthesized using a conventional high-temperature, solid-state method. Crystal structure, photoluminescence excitation, and emission spectra with fluorescence decay curves were investigated. Under UV excitation（325 nm）, NaAlSiO_4：Ce^（3＋）,Sm^（3＋） showed strong blue emission located at 444 nm and orange-reddish emission centered at 563, 601, 648 and 712 nm, stemming from the characteristic emission for 4f-5d transition of Ce^（3＋） and ~4G_（5/2）→~6H_J（J=5/2, 7/2, 9/2, 11/2） transition of Sm^（3＋）, respectively. In addition, we studied the detailed energy transfer process between Ce^（3＋） and Sm^（3＋） and found that it belonged to dipole-dipole resonance energy transfer. Furthermore, we noted that the white light emitting from the Ce^（3＋）, Sm^（3＋） co-doped phosphors with the color coordinate（x=0.313, y=0.283） could be observed under 325 nm excitation, which was close to the ideal white light（x=0.33, y=0.33）. The results indicated that this phosphor has a potential application as a single-phased alumino-silicate phosphor for ultraviolet white light-emitting diodes（UV-WLEDs）.展开更多
文摘设计了一种由1μm涡旋光泵浦的闲频光单谐振KTiOAsO_(4)涡旋光参量振荡器,并基于该光参量振荡器在近/中红外波段实现了高光束质量、高能量、窄光谱带宽的涡旋光输出。选取不同曲率半径的输入镜和平面输出镜分别建立平平腔和平凹腔两种腔结构,基于所建结构可以控制泵浦光的轨道角动量(OAM)选择性地传递给输出的信号光或闲频光。当泵浦光最大能量为20.6 m J时,在近红外波段产生了3.04 m J的信号涡旋光(1.535μm),同时在中红外波段产生了0.82 m J的闲频涡旋光(3.468μm),它们对应的转换效率分别为28.21%和7.62%。基于泵浦光与谐振闲频光在两种腔型中的空间重叠效率,从理论上解释了泵浦光OAM的传递原理。测量得到输出信号光和闲频光的光谱带宽(半峰全宽)分别为λs=0.85 nm和λi=1.08 nm,其中闲频光在两个正交方向上的光束质量因子分别为Mx2≈2.1和My2≈2.2。
基金supported by the National Natural Science Foundation of China(11464045)Autonomous Region Postgraduate Research Innovation Fund Project(XJGRI2016093)+1 种基金the subject of Xinjiang Normal University Key Laboratory(KWFG1605)the Introduction Program of High-Level Talents of Xinjiang Province
文摘A series of tunable phosphors NaAlSiO_4：Ce^（3＋）,Sm^（3＋） were synthesized using a conventional high-temperature, solid-state method. Crystal structure, photoluminescence excitation, and emission spectra with fluorescence decay curves were investigated. Under UV excitation（325 nm）, NaAlSiO_4：Ce^（3＋）,Sm^（3＋） showed strong blue emission located at 444 nm and orange-reddish emission centered at 563, 601, 648 and 712 nm, stemming from the characteristic emission for 4f-5d transition of Ce^（3＋） and ~4G_（5/2）→~6H_J（J=5/2, 7/2, 9/2, 11/2） transition of Sm^（3＋）, respectively. In addition, we studied the detailed energy transfer process between Ce^（3＋） and Sm^（3＋） and found that it belonged to dipole-dipole resonance energy transfer. Furthermore, we noted that the white light emitting from the Ce^（3＋）, Sm^（3＋） co-doped phosphors with the color coordinate（x=0.313, y=0.283） could be observed under 325 nm excitation, which was close to the ideal white light（x=0.33, y=0.33）. The results indicated that this phosphor has a potential application as a single-phased alumino-silicate phosphor for ultraviolet white light-emitting diodes（UV-WLEDs）.
