Metal halide perovskites are attractive for light-emitting diodes due to their superior optoelectronic properties such as tunable bandgaps,high photoluminescence quantum yields(PLQYs),high color purities and solution ...Metal halide perovskites are attractive for light-emitting diodes due to their superior optoelectronic properties such as tunable bandgaps,high photoluminescence quantum yields(PLQYs),high color purities and solution processability[1–6].In the past several years,impressive progress has been made in perovskite light-emitting diodes(PeLEDs)via microstructure engineering[7],charge balancing[8],surface defect passivation[9,10],metal ion doping[11,12]and dimensional engineering[13].As such,the green,red and near-infrared PeLEDs have achieved impressive external quantum efficiencies(EQEs)exceeding 20%[7,8,14,15].However,the performances of pure-blue PeLEDs,i.e.,brightness and EQEs,still lag largely behind those of the green and red counterparts,which severely impedes the PeLED application in full-color display and solid-state lighting.展开更多
基金We acknowledge the financial support from the National Natural Science Foundation of China(51571184,21501165,21875236,21573211,21633007)the National Key R&D Program on Nano Science and Technology(2016YFA0200602,2018YFA0208702)+3 种基金the Fundamental Research Funds for the Central Universities(WK2060190085)the Joint Funds from Hefei National Synchrotron Radiation Laboratory(KY2060000111)the Anhui Initiative in Quantum Information Technologies(AHY090200)We also thank the support from the USTC Center for Micro and Nanoscale Research and Fabrication.
文摘Metal halide perovskites are attractive for light-emitting diodes due to their superior optoelectronic properties such as tunable bandgaps,high photoluminescence quantum yields(PLQYs),high color purities and solution processability[1–6].In the past several years,impressive progress has been made in perovskite light-emitting diodes(PeLEDs)via microstructure engineering[7],charge balancing[8],surface defect passivation[9,10],metal ion doping[11,12]and dimensional engineering[13].As such,the green,red and near-infrared PeLEDs have achieved impressive external quantum efficiencies(EQEs)exceeding 20%[7,8,14,15].However,the performances of pure-blue PeLEDs,i.e.,brightness and EQEs,still lag largely behind those of the green and red counterparts,which severely impedes the PeLED application in full-color display and solid-state lighting.
