研究了活性炭固定床对水中苯酚的动态吸附特性及影响因素。结果表明,活性炭对苯酚废水的动态吸附随进水苯酚含量和流量的增大穿透时间缩短,但最大设计体积流量不能超过6.47 m L/min;随固定床高度增加,穿透时间推迟,但最小设计高度不能小...研究了活性炭固定床对水中苯酚的动态吸附特性及影响因素。结果表明,活性炭对苯酚废水的动态吸附随进水苯酚含量和流量的增大穿透时间缩短,但最大设计体积流量不能超过6.47 m L/min;随固定床高度增加,穿透时间推迟,但最小设计高度不能小于8 cm。无效层厚度随进水流量和固定床高度的增加而增大,随进水苯酚含量增大而减少。经拟合发现实验结果更符合Yoon-Nelson模型,且相关系数都在0.9以上。展开更多
The oxidation of elemental mercury （Hg~） by dielectric barrier discharge reactors was studied at room temperature, where concentric cylinder discharge reactor （CCDR） and surface discharge plasma reactor （SDPR） w...The oxidation of elemental mercury （Hg~） by dielectric barrier discharge reactors was studied at room temperature, where concentric cylinder discharge reactor （CCDR） and surface discharge plasma reactor （SDPR） were employed. The parameters （e.g. Hg^0 oxidation efficiency, energy constant, energy yield, energy consumption, and O3 concentration） were discussed. From comparison of the two reactors, higher Hg^0 oxidation efficiency and energy constant in the SDPR system were obtained by using lower specific energy density. At the same applied voltage, energy yield in the SDPR system was larger than that in the CCDR system, and energy consumption in the SDPR system was much less. Additionally, more 03 was generated in the SDPR system. The experimental results showed that 98% of Hg^0 oxidation efficiency, 0.6 J·L^-1 of energy constant, 13.7 μg·J^-1 of energy yield, 15.1 eV·molecule^-1 of energy consumption, and 12.7 μg·J^-1 of O3 concentration were achieved in the SDPR system. The study reveals an alternative and economical technology for Hg^0 oxidation in the coal-fired flue gas.展开更多
文摘研究了活性炭固定床对水中苯酚的动态吸附特性及影响因素。结果表明,活性炭对苯酚废水的动态吸附随进水苯酚含量和流量的增大穿透时间缩短,但最大设计体积流量不能超过6.47 m L/min;随固定床高度增加,穿透时间推迟,但最小设计高度不能小于8 cm。无效层厚度随进水流量和固定床高度的增加而增大,随进水苯酚含量增大而减少。经拟合发现实验结果更符合Yoon-Nelson模型,且相关系数都在0.9以上。
基金supported by National Natural Science Foundation of China(No.51177007)Ministry of Science and Technology of China(No.2009AA064101-4)
文摘The oxidation of elemental mercury （Hg~） by dielectric barrier discharge reactors was studied at room temperature, where concentric cylinder discharge reactor （CCDR） and surface discharge plasma reactor （SDPR） were employed. The parameters （e.g. Hg^0 oxidation efficiency, energy constant, energy yield, energy consumption, and O3 concentration） were discussed. From comparison of the two reactors, higher Hg^0 oxidation efficiency and energy constant in the SDPR system were obtained by using lower specific energy density. At the same applied voltage, energy yield in the SDPR system was larger than that in the CCDR system, and energy consumption in the SDPR system was much less. Additionally, more 03 was generated in the SDPR system. The experimental results showed that 98% of Hg^0 oxidation efficiency, 0.6 J·L^-1 of energy constant, 13.7 μg·J^-1 of energy yield, 15.1 eV·molecule^-1 of energy consumption, and 12.7 μg·J^-1 of O3 concentration were achieved in the SDPR system. The study reveals an alternative and economical technology for Hg^0 oxidation in the coal-fired flue gas.
