Utilizing a polarization sensitive terahertz detection method where the detector is rotated by either 0° or 90°to measure the electric field Ep,8 (t) of each polarization component, we have characterized t...Utilizing a polarization sensitive terahertz detection method where the detector is rotated by either 0° or 90°to measure the electric field Ep,8 (t) of each polarization component, we have characterized the properties of split ring res- onators. The strong polarization dependence of the bianisotropic-circular-current-driven and linear-polarization-induced resonances is in excellent agreement with the simulation when the p-polarized terahertz transmission is measured. How- ever, these electromagnetic responses vanish when the s-polarized terahertz transmission is measured. There is only a transmission minimum at 1.64 THz and the terahertz polarization rotation angle of about 90° is observed. The polarized terahertz transmission amplitudes and spectra detected at orthogonal orientations show that these behaviours are probably attributed to the birefringent effect of the sample.展开更多
The spatiotemporal and spectral characteristics of ultrawide-band terahertz pulses after passing through a Fresnel lens are studied by using the scalar diffraction theory. The simulation shows that the transmitted ter...The spatiotemporal and spectral characteristics of ultrawide-band terahertz pulses after passing through a Fresnel lens are studied by using the scalar diffraction theory. The simulation shows that the transmitted terahertz waveforms compress with increasing propagation distance, and the multi-frequency focusing phenomenon at different focal points is observed. Additionally, the distribution of terahertz fields in a plane perpendicular to the axis is also discussed, and it is found that the diffraction not only induces focusing on-axis but also inhibits focusing at off-axis positions. Therefore, the Fresnel lens may be a useful alternative approach to being a terahertz filter. Moreover, the terahertz pulses travelling as a basic mode of a Gaussian beam are discussed in detail.展开更多
Femtosecond pump-terahertz probe studies of carrier dynamics in semi-insulating CaAs have been investigated in detail for various pump powers. It is observed that, at high pump powers, the reflection peaks flip to the...Femtosecond pump-terahertz probe studies of carrier dynamics in semi-insulating CaAs have been investigated in detail for various pump powers. It is observed that, at high pump powers, the reflection peaks flip to the opposite polarity and dramatically enhance as the pump arrival time approaches the reflected wave of the terahertz pulse. The abnormal polarity-flip and enhancement can be interpreted by the pump-induced enhancement in the photoconductivity of GaAs and half-wave loss. Moreover, the carrier relaxation processes and surface states filling in GaAs are also studied in these measurements.展开更多
This paper investigates the ultrafast carrier dynamics and surface photoconductivity of unbiased semi-insulating GaAs in detail by using a terahertz pump-emission technique. Based on theoretical modelling, it finds th...This paper investigates the ultrafast carrier dynamics and surface photoconductivity of unbiased semi-insulating GaAs in detail by using a terahertz pump-emission technique. Based on theoretical modelling, it finds that transient photoconductivity plays a very important role in the temporal waveform of terahertz radiation pulse. Anomalous enhancement in both terahertz radiation and transient photoconductivity is observed after the excitation of pump pulse and we attribute these phenomena to carrier capture in the EL2 centers. Moreover, the pump power- and temperature- dependent measurements are also performed to verify this trapping model.展开更多
The optical properties of four kinds of lubricating greases (urea, lithium, extreme pressure lithium, molybdenum disulfide lithium greases) with different NLGL (National Lubricant Grease Institute of America) numb...The optical properties of four kinds of lubricating greases (urea, lithium, extreme pressure lithium, molybdenum disulfide lithium greases) with different NLGL (National Lubricant Grease Institute of America) numbers were investigated using terahertz time-domain spectroscopy. Greases with different NLGL grades have unique spectral features in the terahertz range. Comparison of the experimental data with predictions based on Lorentz Lorenz theory exhibited that the refractive indices of each kind of lubricating grease were dependent on the their consistency. In addition, molybdenum disullfide (MoS2) aa a libricant additive shows strong absorption from 0.2 to 1.4 THz, leading to higher absorption of MoS2-1ithium grease than that of lithium grease.展开更多
The quantitative analysis of zinc isopropyl-isooctyl-dithiophosphate (T204) mixed with lube base oil from Korea with viscosity index 70 (T204-Korea70) is presented by using terahertz time-domain spectroscopy (THz-TDS)...The quantitative analysis of zinc isopropyl-isooctyl-dithiophosphate (T204) mixed with lube base oil from Korea with viscosity index 70 (T204-Korea70) is presented by using terahertz time-domain spectroscopy (THz-TDS).Compared with the middle-infrared spectra of zinc n-butyl-isooctyl-dithiophosphate (T202) and T204,THz spectra of T202 and T204 show the weak broad absorption bands.Then,the absorption coefficients of the T204-Korea70 system follow Beer's law at the concentration from 0.124 to 4.024%.The experimental absorption spectra of T204-Korea70 agree with the calculated ones based on the standard absorption coefficients of T204 and Korea70.The quantitative analysis enables a strategy to monitor the formulation of lubricating oil in real time.展开更多
This paper reports that terahertz time-domain spectroscopy is used to measure the optical properties of CuS nanoparticles in composite samples. The complex conductivity of pure CuS nanoparticles is extracted by applyi...This paper reports that terahertz time-domain spectroscopy is used to measure the optical properties of CuS nanoparticles in composite samples. The complex conductivity of pure CuS nanoparticles is extracted by applying the Bruggeman effective medium theory. The experimental data are consistent with the Drude-Smith model of conductivity in the range of 0.2 1.5 THz. The results demonstrate that carriers become localized with a backscattering behaviour in small-size nanostructures. In addition, the time constant for the carrier scattering is obtained and is only 64.3 fs due to increased electron interaction with interfaces and grain boundaries.展开更多
The ultrafast optical modulation properties of split ring resonators are characterized by utilizing optical pump-terahertz probe spectroscopy.The experimental results show that when the terahertz electric vector is pe...The ultrafast optical modulation properties of split ring resonators are characterized by utilizing optical pump-terahertz probe spectroscopy.The experimental results show that when the terahertz electric vector is perpendicular to the gap of the split ring resonator,resonant absorption can be quenched significantly under high pump excitation.However,when the terahertz electric vector is parallel to the gap,the resonant absorption is less sensitive to pump excitation due to the structural properties of the metamaterial.Our numerical simulations also demonstrate that the pump pulse significantly influences the split ring resonator current by generating carriers in the substrate.展开更多
基金Project supported by the National Basic Research Program of China (Grant No.2007CB310408)the National Natural Science Foundation of China (Grant Nos.10804077,10904098 and 11011120242)+2 种基金the Fund of Beijing Municipal Commission of Education,China (Grant Nos.KM200910028006 and KM201110028004)the Key Program of Ministry of Education,China (Grant No.210002)the Beijing Nova Program,China and the Fund for Academic Human Resources Development in Institutions of Higher Learning under the Jurisdiction of Beijing Municipality,China
文摘Utilizing a polarization sensitive terahertz detection method where the detector is rotated by either 0° or 90°to measure the electric field Ep,8 (t) of each polarization component, we have characterized the properties of split ring res- onators. The strong polarization dependence of the bianisotropic-circular-current-driven and linear-polarization-induced resonances is in excellent agreement with the simulation when the p-polarized terahertz transmission is measured. How- ever, these electromagnetic responses vanish when the s-polarized terahertz transmission is measured. There is only a transmission minimum at 1.64 THz and the terahertz polarization rotation angle of about 90° is observed. The polarized terahertz transmission amplitudes and spectra detected at orthogonal orientations show that these behaviours are probably attributed to the birefringent effect of the sample.
基金Project supported by the National Basic Research Program of China (Grant Nos 2007CB310408 and 2006CB302901)the National Natural Science Foundation of China (Grant No 10804077)+2 种基金Beijing Municipal Commission of Education (Grant No KM200910028006)Funding Project for Academic Human Resources Development in Institutions of Higher Learning under the Jurisdiction of Beijing Municipalitythe State Key Laboratory of Functional Materials for Informatics,Shanghai Institute of Microsystem and Information Technology,Chinese Academy of Sciences
文摘The spatiotemporal and spectral characteristics of ultrawide-band terahertz pulses after passing through a Fresnel lens are studied by using the scalar diffraction theory. The simulation shows that the transmitted terahertz waveforms compress with increasing propagation distance, and the multi-frequency focusing phenomenon at different focal points is observed. Additionally, the distribution of terahertz fields in a plane perpendicular to the axis is also discussed, and it is found that the diffraction not only induces focusing on-axis but also inhibits focusing at off-axis positions. Therefore, the Fresnel lens may be a useful alternative approach to being a terahertz filter. Moreover, the terahertz pulses travelling as a basic mode of a Gaussian beam are discussed in detail.
基金Project supported by the National Basic Research Program of China (973 Program) (Grant Nos 2007CB310408 and2006CB302901)the National Natural Science Foundation of China (Grant No 10804077)+2 种基金Science Foundation of Beijing Municipal Commission of Education (Grant No KM200910028006)Funding Project for Academic Human Resources Development in Institutions of Higher Learning under the Jurisdiction of Beijing Municipalitysupported by State Key Laboratory of Functional Materials for Informatics,Shanghai Institute of Microsystem and Information Technology,the Chinese Academy of Sciences
文摘Femtosecond pump-terahertz probe studies of carrier dynamics in semi-insulating CaAs have been investigated in detail for various pump powers. It is observed that, at high pump powers, the reflection peaks flip to the opposite polarity and dramatically enhance as the pump arrival time approaches the reflected wave of the terahertz pulse. The abnormal polarity-flip and enhancement can be interpreted by the pump-induced enhancement in the photoconductivity of GaAs and half-wave loss. Moreover, the carrier relaxation processes and surface states filling in GaAs are also studied in these measurements.
基金Project supported by the National Basic Research Program (973 Program) (Grant Nos 2007CB310408 and 2006CB302901)the National Natural Science Foundation of China (Grant No 10804077)+1 种基金Funding Project for Academic Human Resources Development in Institutions of Higher Learning under the Jurisdiction of Beijing Municipalitysupported by State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciencs
文摘This paper investigates the ultrafast carrier dynamics and surface photoconductivity of unbiased semi-insulating GaAs in detail by using a terahertz pump-emission technique. Based on theoretical modelling, it finds that transient photoconductivity plays a very important role in the temporal waveform of terahertz radiation pulse. Anomalous enhancement in both terahertz radiation and transient photoconductivity is observed after the excitation of pump pulse and we attribute these phenomena to carrier capture in the EL2 centers. Moreover, the pump power- and temperature- dependent measurements are also performed to verify this trapping model.
基金Project supported by the New Century Excellent Talents in University(Grant No.NCET-08-0841)the National Natural Science Foundation of China(Grant Nos.60778034,60877038,and10804077)+2 种基金the Beijng Natural Science Foundation(Grant No.4082026)the Research Fund for the Doctoral Program of Higher Education(Grant No.200804250006)the State KeyLaboratory of Heavy Oil Processing,China University of Petroleum(Grant No.2008-14)
文摘The optical properties of four kinds of lubricating greases (urea, lithium, extreme pressure lithium, molybdenum disulfide lithium greases) with different NLGL (National Lubricant Grease Institute of America) numbers were investigated using terahertz time-domain spectroscopy. Greases with different NLGL grades have unique spectral features in the terahertz range. Comparison of the experimental data with predictions based on Lorentz Lorenz theory exhibited that the refractive indices of each kind of lubricating grease were dependent on the their consistency. In addition, molybdenum disullfide (MoS2) aa a libricant additive shows strong absorption from 0.2 to 1.4 THz, leading to higher absorption of MoS2-1ithium grease than that of lithium grease.
基金Supported by the Program for New Century Excellent Talents in University(No NCET-08-0841)the Beijing Natural Science Foundation(No 4122064)the Foresight Fund Program from China University of Petroleum(Beijing)(No QZDX-2010-01).
文摘The quantitative analysis of zinc isopropyl-isooctyl-dithiophosphate (T204) mixed with lube base oil from Korea with viscosity index 70 (T204-Korea70) is presented by using terahertz time-domain spectroscopy (THz-TDS).Compared with the middle-infrared spectra of zinc n-butyl-isooctyl-dithiophosphate (T202) and T204,THz spectra of T202 and T204 show the weak broad absorption bands.Then,the absorption coefficients of the T204-Korea70 system follow Beer's law at the concentration from 0.124 to 4.024%.The experimental absorption spectra of T204-Korea70 agree with the calculated ones based on the standard absorption coefficients of T204 and Korea70.The quantitative analysis enables a strategy to monitor the formulation of lubricating oil in real time.
基金Project supported by the Research Foundation of the State Ethnic Affairs Commission of People’s Repulic of China (Grant No. 09ZY012)the National Natural Science Foundation of China (Grant No. 10904176)+1 种基金the "Project 985"the "Project 211" of Minzu University of China
文摘This paper reports that terahertz time-domain spectroscopy is used to measure the optical properties of CuS nanoparticles in composite samples. The complex conductivity of pure CuS nanoparticles is extracted by applying the Bruggeman effective medium theory. The experimental data are consistent with the Drude-Smith model of conductivity in the range of 0.2 1.5 THz. The results demonstrate that carriers become localized with a backscattering behaviour in small-size nanostructures. In addition, the time constant for the carrier scattering is obtained and is only 64.3 fs due to increased electron interaction with interfaces and grain boundaries.
基金Project supported by the National Basic Research Program of China(Grant No.2007CB310408)the National Natural Science Foundation of China(Grant Nos.10804077,10904098 and 11011120242)+2 种基金the Beijing Municipal Commission of Education,China (Grant No.KM200910028006)the Foundation for Key Program of Ministry of Education,China(Grant No.210002)the Beijing Nova Program,and the Funding Project for Academic Human Resources Development in Institutions of Higher Learning Under the Jurisdiction of Beijing Municipality,China
文摘The ultrafast optical modulation properties of split ring resonators are characterized by utilizing optical pump-terahertz probe spectroscopy.The experimental results show that when the terahertz electric vector is perpendicular to the gap of the split ring resonator,resonant absorption can be quenched significantly under high pump excitation.However,when the terahertz electric vector is parallel to the gap,the resonant absorption is less sensitive to pump excitation due to the structural properties of the metamaterial.Our numerical simulations also demonstrate that the pump pulse significantly influences the split ring resonator current by generating carriers in the substrate.