As one of the most important steps in wastewater treatment, limited study on plasma discharge process is a key challenge in the development of plasma applications. In this study, we focus on the plasma discharge proce...As one of the most important steps in wastewater treatment, limited study on plasma discharge process is a key challenge in the development of plasma applications. In this study, we focus on the plasma discharge process of a pulsed diaphragm discharge system. According to the analysis, the pulsed diaphragm discharge proceeds in seven stages： （1） Joule heating and heat exchange stage; （2） nucleated site formation; （3） plasma generation （initiation of the breakdown stage）; （4） avalanche growth and plasma expansion; （5） plasma contraction; （6） termination of the plasma discharge; and （7） heat exchange stage. From this analysis, a critical voltage criterion for breakdown is obtained. We anticipate this finding will provide guidance for a better application of plasma discharges, especially diaphragm plasma discharges.展开更多
A synergistic photocatalysis combined pulsed diaphragm discharge（PDD）system with TiO_2 nanofilm deposited on the surface of quartz diaphragm is developed for the first time for phenol degradation in an aqueous solut...A synergistic photocatalysis combined pulsed diaphragm discharge（PDD）system with TiO_2 nanofilm deposited on the surface of quartz diaphragm is developed for the first time for phenol degradation in an aqueous solution.It is observed that the decomposition efficiency of phenol in the TiO_2 combined PDD system is higher than that of the single PDD system under the same conditions,indicating a successful collaboration between the photocatalysis and the plasma decomposition in the present system.Analysis of the solution＇s pH value confirms this collaboration and further reveals that the photocatalytic enhancement effect of phenol degradation is strong at a relatively low supplied voltage.The present TiO_2 combined PDD system exhibits improved efficiencies of pollutant degradation and energy utilization,suggesting a good candidate for wastewater treatment.展开更多
基金supported by National Natural Science Foundation of China(Nos.11205202,21203204 and 11175214)Natural Science Foundation of Anhui Province,China (No.1308085QA09)
文摘As one of the most important steps in wastewater treatment, limited study on plasma discharge process is a key challenge in the development of plasma applications. In this study, we focus on the plasma discharge process of a pulsed diaphragm discharge system. According to the analysis, the pulsed diaphragm discharge proceeds in seven stages： （1） Joule heating and heat exchange stage; （2） nucleated site formation; （3） plasma generation （initiation of the breakdown stage）; （4） avalanche growth and plasma expansion; （5） plasma contraction; （6） termination of the plasma discharge; and （7） heat exchange stage. From this analysis, a critical voltage criterion for breakdown is obtained. We anticipate this finding will provide guidance for a better application of plasma discharges, especially diaphragm plasma discharges.
基金supported by National Natural Science Foundation of China(Nos.11205202,21203204 and 11175214)National Natural Science Foundation of Anhui Province(No.1308085QA09)
文摘A synergistic photocatalysis combined pulsed diaphragm discharge（PDD）system with TiO_2 nanofilm deposited on the surface of quartz diaphragm is developed for the first time for phenol degradation in an aqueous solution.It is observed that the decomposition efficiency of phenol in the TiO_2 combined PDD system is higher than that of the single PDD system under the same conditions,indicating a successful collaboration between the photocatalysis and the plasma decomposition in the present system.Analysis of the solution＇s pH value confirms this collaboration and further reveals that the photocatalytic enhancement effect of phenol degradation is strong at a relatively low supplied voltage.The present TiO_2 combined PDD system exhibits improved efficiencies of pollutant degradation and energy utilization,suggesting a good candidate for wastewater treatment.
