基于脉冲整形的激发双重态间的相干布局操控

为了实现红外飞秒脉冲的整形及调控,采用4f系统相位控制技术,实验搭建了脉冲整形装置,并利用整形脉冲对铷原子体系中激发双重态间的相干布居转移进行操控。结果表明,控制抽运脉冲的附加相位,可实现双重态中上激发态的饱和布居,通过修改附加相位函数可将上、下激发态的布居数反转。整形脉冲同样适用于其它的原子和分子系统的相干布居转移的操控。

Control of molecular excitation during the plasma generation of a femtosecond laser pulse

From a classical dynamic simulation,we find the kinetic energy of the electrons generated during laser plasma generation depends on the laser polarization and intensity.The electron kinetic energy reaches its maximum with a fixed laser intensity for circularly polarized laser pulse.The fluorescence spectra at 380.4 nm from N2 and 391.3 nm from N2^＋ are measured;these are generated by both the direct excitation and electron collision excitation.The electron collision excitation is determined by the electron energy and reaches the maximal with a circularly polarized pulse.