A cationic gemini surfactant 10-2-10, 1,2-ethane bis(decyl dimethyl ammonium bromide) was synthesized, and the interactions in a mixture of the cationic gemini surfactant with a water-soluble polymer polyvinyl alcohol...A cationic gemini surfactant 10-2-10, 1,2-ethane bis(decyl dimethyl ammonium bromide) was synthesized, and the interactions in a mixture of the cationic gemini surfactant with a water-soluble polymer polyvinyl alcohol(PVA) were investigated by means of viscosity, electric conductivity, surface tension and ultraviolet spectrum measurements. The results showed that PVA displays viscosity behavior of polyelectrolyte-electroviscous effect in an aqueous solution with gemini surfactant 10-2-10 due to the molecular interaction between the polymer and the surfactant. The maximum UV absorption wavelength of polymer-surfactant solution shifted to higher wavelength compared with that of the surfactant, and the conductivity of polymer-surfactant solution increased with increase in concentration of PVA in a certain surfactant concentration. In addition, surface tension of gemini surfactant 10-2-10 solution decreased in the presence of PVA and its critical micelle concentration decreased from 5.9 mmol/L to 4.8 mmol/L in the presence of 1.25×10^-3 g/mL PVA.展开更多
We demonstrate a high-energy and high-power pulse laser on a xenon lamp-pumped Er:YAP crystal. The laser performance and thermal focal lengths under different working frequencies are discussed. The results show that t...We demonstrate a high-energy and high-power pulse laser on a xenon lamp-pumped Er:YAP crystal. The laser performance and thermal focal lengths under different working frequencies are discussed. The results show that the thermal lens effect is gradually aggravated with the increase of working frequencies, and even working at 100 Hz, a single pulse energy of 234 m J can be achieved. A maximum average power of 41.5 W is achieved with a working frequency of 20 Hz and slope efficiency of 2.82%. This output power is much higher than other xenon lamp-pumped erbium laser devices.A Q-switched laser is demonstrated by using the TeO2crystal, the maximum output energies of 11.5 m J and 3.5 m J are obtained at 50 and 100 Hz, the corresponding peak powers are 93.4 k W and 17.2 kW, respectively.The laser wavelengths and beam quality factors are also characterized in the free-running and Q-switched modes. A higher pulse energy and peak power laser could be achieved further by improving the damage threshold of TeO2acousto-optical Q-switching. All the experimental results illustrate that the xenon lamp-pumped Er:YAP laser is a promising candidate for high-power and high-frequency mid-infrared laser devices.展开更多
A comparative study on the laser performance between bonding and non-bonding Er,Pr:GYSGG rods side-pumped by 970-nm laser diodes(LDs) is conducted for the thermal lensing compensation. The analyses of the thermal dist...A comparative study on the laser performance between bonding and non-bonding Er,Pr:GYSGG rods side-pumped by 970-nm laser diodes(LDs) is conducted for the thermal lensing compensation. The analyses of the thermal distribution and thermal focal length show that the bonding rod possesses a high cooling efficiency and weak thermal lensing effect compared with the conventional Er,Pr:GYSGG rod. Moreover, the laser characteristics of maximum output power, slope efficiency, and laser beam quality of the bonding rod with concave end-faces operated at 2.79 μm are improved under the high-repetition-rate operation. A maximum output power of 13.96 W is achieved at 150-Hz and 200-μs pulse width,corresponding to a slope efficiency of 17.7% and an electrical-to-optical efficiency of 12.9%. All results suggest that the combination of thermal bonding and concave end-face is a suitable structure for thermal lensing compensation.展开更多
We demonstrate the spectroscopic and laser performance before and after 100 Mrad gamma-ray irradiation on an Er,Pr:GYSGG crystal grown by the Czochralski method. The additional absorption of Er,Pr:GYSGG crystal is c...We demonstrate the spectroscopic and laser performance before and after 100 Mrad gamma-ray irradiation on an Er,Pr:GYSGG crystal grown by the Czochralski method. The additional absorption of Er,Pr:GYSGG crystal is close to zero in the 968 nm pumping and 2.7-3 μm laser wavelength regions. The lifetimes of the upper and lower levels show faint decreases after gamma-ray irradiation. The maximum output powers of 542 and 526 mW with the slope efficiencies of 17.7% and 17.0% are obtained, respectively, on the GYSGG/Er,Pr:GYSGG composite crystal before and after the gammaray irradiation. These results suggest that Er,Pr:GYSGG crystal as a laser gain medium possesses a distinguished antiradiation ability for application in space and radiant environments.展开更多
文摘A cationic gemini surfactant 10-2-10, 1,2-ethane bis(decyl dimethyl ammonium bromide) was synthesized, and the interactions in a mixture of the cationic gemini surfactant with a water-soluble polymer polyvinyl alcohol(PVA) were investigated by means of viscosity, electric conductivity, surface tension and ultraviolet spectrum measurements. The results showed that PVA displays viscosity behavior of polyelectrolyte-electroviscous effect in an aqueous solution with gemini surfactant 10-2-10 due to the molecular interaction between the polymer and the surfactant. The maximum UV absorption wavelength of polymer-surfactant solution shifted to higher wavelength compared with that of the surfactant, and the conductivity of polymer-surfactant solution increased with increase in concentration of PVA in a certain surfactant concentration. In addition, surface tension of gemini surfactant 10-2-10 solution decreased in the presence of PVA and its critical micelle concentration decreased from 5.9 mmol/L to 4.8 mmol/L in the presence of 1.25×10^-3 g/mL PVA.
基金supported by the Natural Science Foundation of Anhui Province (Grant No. 2208085QF217)the National Natural Science Foundation of China (Grant No. 52102012)the Hefei Institutes of Physical Science (HFIPS) Director’s Fund (Grant No. YZJJ2022QN08)。
文摘We demonstrate a high-energy and high-power pulse laser on a xenon lamp-pumped Er:YAP crystal. The laser performance and thermal focal lengths under different working frequencies are discussed. The results show that the thermal lens effect is gradually aggravated with the increase of working frequencies, and even working at 100 Hz, a single pulse energy of 234 m J can be achieved. A maximum average power of 41.5 W is achieved with a working frequency of 20 Hz and slope efficiency of 2.82%. This output power is much higher than other xenon lamp-pumped erbium laser devices.A Q-switched laser is demonstrated by using the TeO2crystal, the maximum output energies of 11.5 m J and 3.5 m J are obtained at 50 and 100 Hz, the corresponding peak powers are 93.4 k W and 17.2 kW, respectively.The laser wavelengths and beam quality factors are also characterized in the free-running and Q-switched modes. A higher pulse energy and peak power laser could be achieved further by improving the damage threshold of TeO2acousto-optical Q-switching. All the experimental results illustrate that the xenon lamp-pumped Er:YAP laser is a promising candidate for high-power and high-frequency mid-infrared laser devices.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.51872290,51702322,and 51802307)the National Key Research and Development Program of China(Grant No.2016YFB1102301)
文摘A comparative study on the laser performance between bonding and non-bonding Er,Pr:GYSGG rods side-pumped by 970-nm laser diodes(LDs) is conducted for the thermal lensing compensation. The analyses of the thermal distribution and thermal focal length show that the bonding rod possesses a high cooling efficiency and weak thermal lensing effect compared with the conventional Er,Pr:GYSGG rod. Moreover, the laser characteristics of maximum output power, slope efficiency, and laser beam quality of the bonding rod with concave end-faces operated at 2.79 μm are improved under the high-repetition-rate operation. A maximum output power of 13.96 W is achieved at 150-Hz and 200-μs pulse width,corresponding to a slope efficiency of 17.7% and an electrical-to-optical efficiency of 12.9%. All results suggest that the combination of thermal bonding and concave end-face is a suitable structure for thermal lensing compensation.
基金Project supported by the National Key Research and Development Program of China(Grant No.2016YFB1102301)the National Natural Science Foundation of China(Grant Nos.51272254,61405206,and 51502292)the Open Research Fund of the State Key Laboratory of Pulsed Power Laser Technology,Electronic Engineering Institute,China(Grant No.SKL2015KF01)
文摘We demonstrate the spectroscopic and laser performance before and after 100 Mrad gamma-ray irradiation on an Er,Pr:GYSGG crystal grown by the Czochralski method. The additional absorption of Er,Pr:GYSGG crystal is close to zero in the 968 nm pumping and 2.7-3 μm laser wavelength regions. The lifetimes of the upper and lower levels show faint decreases after gamma-ray irradiation. The maximum output powers of 542 and 526 mW with the slope efficiencies of 17.7% and 17.0% are obtained, respectively, on the GYSGG/Er,Pr:GYSGG composite crystal before and after the gammaray irradiation. These results suggest that Er,Pr:GYSGG crystal as a laser gain medium possesses a distinguished antiradiation ability for application in space and radiant environments.