Palladium-based hydrogen sensors have been typically studied due to the dielectric function that changes with the hydrogen concentration. However, the development of a reliable, integral, and widely applicable hydroge...Palladium-based hydrogen sensors have been typically studied due to the dielectric function that changes with the hydrogen concentration. However, the development of a reliable, integral, and widely applicable hydrogen sensor requires a simple readout mechanism and an optimization of the fast detection of hydrogen. In this work, optical fiber hydrogen sensing platforms are developed using an optimized metasurface, which consists of a layer of palladium nanoantennas array suspended above a gold mirror layer. Since the optical properties of these palladium nanoantennas differ from the traditional palladium films, a high reflectance difference can be achieved when the sensor based on the metasurface is exposed to the hydrogen atmosphere. Finally, the optimized reflectance difference ΔR of ~0.28 can be obtained when the sensor is exposed in the presence of hydrogen. It is demonstrated that this integrated system architecture with an optimized palladium-based metasurface and a simple optical fiber readout system provides a compact and light platform for hydrogen detection in various working environments.展开更多
基金This work was partially supported by the National Natural Science Foundation of China(NSFC)(No.92050117)China Postdoctoral Science Foundation(No.2020M680370)Beijing Institute of Technology Research Fund Program for Young Scholars(No.XSQD-201904005).
文摘Palladium-based hydrogen sensors have been typically studied due to the dielectric function that changes with the hydrogen concentration. However, the development of a reliable, integral, and widely applicable hydrogen sensor requires a simple readout mechanism and an optimization of the fast detection of hydrogen. In this work, optical fiber hydrogen sensing platforms are developed using an optimized metasurface, which consists of a layer of palladium nanoantennas array suspended above a gold mirror layer. Since the optical properties of these palladium nanoantennas differ from the traditional palladium films, a high reflectance difference can be achieved when the sensor based on the metasurface is exposed to the hydrogen atmosphere. Finally, the optimized reflectance difference ΔR of ~0.28 can be obtained when the sensor is exposed in the presence of hydrogen. It is demonstrated that this integrated system architecture with an optimized palladium-based metasurface and a simple optical fiber readout system provides a compact and light platform for hydrogen detection in various working environments.
