用推广的量子轨迹蒙特卡罗方法研究强场光电子全息

强场光电子全息因其二维光电子动量谱中携带着电子和离子的时空动力学信息,所以在实验中被发现后迅速成为近年来强场超快物理中的一个热点研究领域.本文主要介绍一种推广的量子轨迹蒙特卡罗计算方法.利用这种方法可在更广泛的实验条件下探讨原子分子光电子全息现象背后深层次的物理机理.与含时薛定谔方程的对比发现利用推广的量子轨迹蒙特卡罗方法计算的光电子全息干涉结构的截止能量位置能清楚地反映非绝热隧穿电离效应.而且,我们发现了深隧穿电离条件下一种新颖的圆环干涉结构.这一圆环状干涉结构遮蔽了光电子全息条纹,因此,这一结果表明:深隧穿区并非是形成光电子全息的有利实验条件.在非绝热隧穿区,长程库仑势对于光电子全息的形成起着至关重要的作用.

Vibrational transition spectra of H_2^+ in a strong magnetic field

Vibrational transition spectra of H2＋ in an ultra-strong magnetic field are determined. The validity of Born- Oppenheimer approximation is analyzed based on one-center method and B-spline basis sets. It is shown that Born- Oppenheimer approximation is reliable for the investigation on the ground state and low excited states of H2＋ subjected to the strong magnetic field. Furthermore, it is found that the vibrational transition spectra from lσg, lπu, and 1δg states lie in infrared, visible, and ultraviolet ranges with increasing magnetic field strength.

Effect of electron correlation on high-order harmonic generation in helium model atom

High-order harmonic generation （HHG） of a helium model atom in an intense laser field has been numerically investigated. The influence of electron correlation on HHG is analysed by changing the strength between the electrons. The numerical results show that as the electron interaction strength becomes small, the first ionization energy increases rapidly, which results in the decrease in ionization. So the conversion efficiency of the high harmonic lying in the plateau decreases greatly, while the cutoff harmonic order in the harmonic spectrum increases.

Alignment-Dependent Ionization of CO_(2)in the Intense Laser Fields:Single-Active-Electron Approach

We perform Hartree–Fock calculations to obtain occupied orbitals for triatomic molecule CO_(2),based on one-center method and B-splines to deal with cusps and speed up convergence.Both the orbital energies and charge distribution are in good accordance with the reference data.The valence orbital is propagated with single-active-electron approximation,and the alignment-dependent ionization yield peaks about 40°.However,there are discrepancies between our results and the experimental data,and many-electron effects may need to be exploited further to describe them.

Nonadiabatic Effect on the Rescattering Trajectories of Electrons in Strong Laser Field Ionization Process

The important features of the rescattering trajectories in strong field ionization process such as the cutoff of the return energy at 3.17Up and that of the final energy at 10Up are obtained, based on the adiabatic approximation in which the initial momentum of the electron is assumed to be zero. We theoretically study the nonadiabatic effect by assuming a nonzero initial momentum on the rescattering trajectories based on the semiclassical simpleman model. We show that the nonzero initial momentum will modify both the maximal return energy at collision and the final energy after backward scattering, but in different ways for odd and even number of return trajectories. The energies are increased for even number of returns but are decreased for odd number of returns when the nonzero （positive or negative） initial momentum is applied.

Controlling Rydberg excitation process with shaped intense ultrashort laser pulses

We perform a theoretical investigation on the control over the atomic excitation of Rydberg states with shaped intense ultrashort laser pulses.By numerically solving the time-dependent Schrodinger equation(TDSE),we systematically study the dependence of the population of the Rydberg states on theπphase step position in the frequency spectra of the laser pulse for different intensities,central wavelengths and pulse durations.Our results show that the Rydberg excitation process can be effectively modulated using shaped intense laser pulses with the laser intensity as high as 1×10^14 W/cm^2.Our work also have benefit to the future investigation to find out the dominant mechanism behind the excitation of Rydberg states in strong laser fields.

Controlling Three-Dimensional Electron-Electron Correlation via Elliptically Polarized Intense Laser Field

The three-dimensional electron-electron correlation in an elliptically polarized laser field is investigated based on a semiclassical model. Asymmetry parameter α of the correlated electron momentum distribution is used to quantitatively describe the electron-electron correlation. The dependence of α on elliptieity e is totally different in three directions. For the z direction （maJor polarization direction）, α first increases and reaches a maximum at ε = 0.275, then it decreases quickly. For the y direction in which the laser field is always absent, the ellipticity has a minor effect, and the asymmetry parameter fluctuates around α = -0.15. However, for the x direction （minor polarization direction）, α increases monotonously with ellipticity though starts from the same value as in the y direction when ε = 0. The behavior of α in the x direction actually indicates a transformation from the Coulomb interaction dominated correlation to the laser field dominated correlation. Therefore, our work provides an efficient way to control the three-dimensional electron electron correlation via an elliptically polarized intense laser field.

Time-energy analysis of the photoionization process in a double-XUV pulse combined with a few-cycle IR field

We calculate the time-energy distribution(TED)and ionization time distribution(ITD)of photoelectrons emitted by a doubleextreme-ultraviolet(XUV)pulse and a two-color XUV-IR pulse using the Wigner distribution-like function based on the strong field approximation.For a double-XUV pulse,besides two identical broad distributions generated by two XUV pulses,many interference fringes resulting from the interference between electrons generated,respectively,by two pulses appear in the TED.After adding an IR field,the TED intuitively exhibits the effect of the IR field on the electron dynamics.The ITDs during two XUV pulses are no longer the same and show the different changes for the different two-color fields,the origin of which is attributed to the change of the electric field induced by the IR field.Our analysis shows that the emission time of electrons ionized during two XUV pulses mainly depends on the electric field of the combined XUV pulse and IR pulse.