The interference between two dissociating wave packets of the I2 molecule driven by femtosecond laser pulses is theoretically studied by using the time-dependent quantum wave packet method.Both the internuclear distan...The interference between two dissociating wave packets of the I2 molecule driven by femtosecond laser pulses is theoretically studied by using the time-dependent quantum wave packet method.Both the internuclear distanceand velocity-dependent density functions are calculated and discussed.It is demonstrated that the interference pattern is determined by the phase difference and the delay time between two pump pulses.With two identical pulses with a delay time of 305 fs and a FWHM of 20 fs,more interference fringes can be observed,while with two pump pulses with a delay time of 80 fs and a FWHM of 20 fs,only a few interference fringes can be observed.展开更多
基金Li-hang Li thanks Dr. Yin Huang for assistance. The project is supported by the Specialized Research Fund for the Doctoral Program of Higher Education (No.20130041120053), SRF for ROCS, SEM, the Sci- ence and Technology Research Funds of the Depart- ment of Education of Liaoning Province (L2013014), the National Magnetic Confinement Fusion Science Pro- gram (No.2013GB109005), the Fundamental Research Funds for the Central Universities (DUT12RC(3)60), and the NationM Natural Science Foundation of China (No.21473018, No.10974024, and No.11274056).
基金Project supported by the National Natural Science Foundation of China (Grant Nos 10674022 and 20633070)
文摘The interference between two dissociating wave packets of the I2 molecule driven by femtosecond laser pulses is theoretically studied by using the time-dependent quantum wave packet method.Both the internuclear distanceand velocity-dependent density functions are calculated and discussed.It is demonstrated that the interference pattern is determined by the phase difference and the delay time between two pump pulses.With two identical pulses with a delay time of 305 fs and a FWHM of 20 fs,more interference fringes can be observed,while with two pump pulses with a delay time of 80 fs and a FWHM of 20 fs,only a few interference fringes can be observed.