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Optimization and evaluation of reduced graphene oxide hydrogel composite as a demulsifier for heavy crude oil-in-water emulsion 被引量:1
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作者 Kin Kit Fong Inn Shi Tan +3 位作者 Henry Chee Yew Foo Man Kee Lam adrian chiong yuh tiong Steven Lim 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2021年第5期297-305,共9页
The rising production of produced water from oilfields had been proven to bring detrimental environmental effects.In this study,an efficient,recyclable,and environmental-friendly reduced graphene oxide immobilizedκ-C... The rising production of produced water from oilfields had been proven to bring detrimental environmental effects.In this study,an efficient,recyclable,and environmental-friendly reduced graphene oxide immobilizedκ-Carrageenan hydrogel composite(κCaGO)was fabricated as an alternative sorbent for crude oil-in-water demulsification.Polyethyleneimine(PEI)was employed to form a stable hydrogel composite.The conditions for the immobilization of graphene oxide(GO)on PEI-modifiedκ-Carrageenan(κC)beads were optimized appropriately.An immobilization yield of 77%was attained at 2%PEI,2 h immobilization activation time,and pH 6.5.Moreover,the synthesizedκCaGO is capable of demulsification with an average demulsification efficiency of 70%.It was found that the demulsification efficiency increases with salinity andκCaGO dosage,and it deteriorates under alkaline condition.These phenomena can be attributed to the interfacial interactions betweenκCaGO and the emulsion.Furthermore,theκCaGO can be recycled to use for up to six cycles without significant leaching and degradation.As such,the synthesizedκCaGO could be further developed as a potential sorbent substitute for the separation of crude oil from produced water. 展开更多
关键词 Graphene OXIDE Κ-CARRAGEENAN Adsorbents DEMULSIFICATION Composites WASTE water
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