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Impacts of pollution heterogeneity on population exposure in dense urban areas using ultra-fine resolution air quality data
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作者 Wenwei Che Yumiao Zhang +3 位作者 Changqing Lin Yik Him Fung Jimmy C.H.Fung alexis khlau 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2023年第3期513-523,共11页
Traditional air quality data have a spatial resolution of 1 km or above, making it challenging to resolve detailed air pollution exposure in complex urban areas. Combining urban morphology, dynamic traffic emission, r... Traditional air quality data have a spatial resolution of 1 km or above, making it challenging to resolve detailed air pollution exposure in complex urban areas. Combining urban morphology, dynamic traffic emission, regional and local meteorology, physicochemical transformations in air quality models using big data fusion technology, an ultra-fine resolution modeling system was developed to provide air quality data down to street level. Based on one-year ultra-fine resolution data, this study investigated the effects of pollution heterogeneity on the individual and population exposure to particulate matter(PM_(2.5)and PM_(10)),nitrogen dioxide(NO_(2)), and ozone(O_(3)) in Hong Kong, one of the most densely populated and urbanized cities. Sharp fine-scale variabilities in air pollution were revealed within individual city blocks. Using traditional 1 km average to represent individual exposure resulted in a positively skewed deviation of up to 200% for high-end exposure individuals. Citizens were disproportionally affected by air pollution, with annual pollutant concentrations varied by factors of 2 to 5 among 452 District Council Constituency Areas(DCCAs) in Hong Kong, indicating great environmental inequities among the population. Unfavorable city planning resulted in a positive spatial coincidence between pollution and population, which increased public exposure to air pollutants by as large as 46% among districts in Hong Kong. Our results highlight the importance of ultra-fine pollutant data in quantifying the heterogeneity in pollution exposure in the dense urban area and the critical role of smart urban planning in reducing exposure inequities. 展开更多
关键词 Particulate matter Nitrogen dioxide OZONE Pollution heterogeneity Urban area
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粤港澳大湾区PM2.5本地与非本地污染来源解析 被引量:8
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作者 王怡然 袁自冰 +9 位作者 赵恺辉 张舒 张夏夏 李文石 谢岩 杨雷峰 刘启汉 郁建珍 岳玎利 谭振威 《环境科学学报》 CAS CSCD 北大核心 2020年第5期1560-1574,共15页
粤港澳大湾区(简称“大湾区”)建设是我国新时代重大国家战略之一.虽然大湾区空气质量在我国处于领先地位,但与世界先进湾区相比还有较大差距.制定大湾区PM2.5精细化防控策略,需要在识别大湾区各城市PM2.5污染来源的基础上,量化PM2.5本... 粤港澳大湾区(简称“大湾区”)建设是我国新时代重大国家战略之一.虽然大湾区空气质量在我国处于领先地位,但与世界先进湾区相比还有较大差距.制定大湾区PM2.5精细化防控策略,需要在识别大湾区各城市PM2.5污染来源的基础上,量化PM2.5本地和非本地贡献及时空变化规律.基于此,本研究首次在大湾区15个站点同步开展持续一年的PM2.5采样和组分分析,并将正定矩阵因子分析模型与后向轨迹结合,建立一种定量识别PM2.5本地与非本地贡献的新方法.通过对大湾区不同季节所属空气域进行划分,厘清大湾区各城市PM2.5本地与非本地贡献的动态化特征.结果发现,在2015年,大湾区15个站点共解析出9种PM2.5污染源,分别为机动车、重油、老化海盐、扬尘源、二次硫酸盐、二次硝酸盐、金属冶炼、生物质燃烧和新鲜海盐.其中,二次硫酸盐和机动车是大湾区最主要的两个PM2.5污染源.不同站点非本地贡献占比为51%~72%,表明外来传输是大湾区PM2.5污染的主要来源.内陆和沿海站点污染源的本地与非本地贡献差异较为显著,主要原因是气象条件和排放特征的差异.值得注意的是,2015年大湾区超过一半的时间处于同一个空气域,而有43%的时间处于两个不同空气域.进一步在每个季节划分空气域,发现大湾区处于两个空气域时,秋、冬季节沿海站点易形成单独的空气域,此时非本地贡献较强(68%~72%);春季内陆站点易形成单独的空气域,此时本地贡献较强(94%).基于对PM2.5本地和非本地贡献变化情况的定量识别,能够为大湾区各城市制定动态的PM2.5排放控制策略提供科学支撑. 展开更多
关键词 PM2.5 正定矩阵因子分析 本地和非本地贡献 空气域 粤港澳大湾区(GBA)
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