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Exploration of optimal reaction conditions on lactic acid production from glucose photoreforming over carbon nitride 被引量:1
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作者 Heng Zhao Xiao Wang +6 位作者 Xingxing Wu Jiu Wang Na Zhong ali seifitokaldani Stephen Larter Md Golam Kibria Jinguang Hu 《Resources Chemicals and Materials》 2023年第2期111-116,共6页
Biomass valorization by photoreforming approach provides a promising and alternative strategy to generate value-added chemicals and fuels.In this work,we demonstrate the selective production of lactic acid from glu-co... Biomass valorization by photoreforming approach provides a promising and alternative strategy to generate value-added chemicals and fuels.In this work,we demonstrate the selective production of lactic acid from glu-cose photoreforming over pristine graphitic carbon nitride(g-C_(3) N_(4))photocatalyst.Control experiments screen the best condition for the highest yield of lactic acid,including modulating pH,catalyst loading,and reaction time.100%glucose conversion is achieved along with almost 100%lactic acid yield under the optimized con-dition.Density functional theory(DFT)calculations reveal that the rate-determining step(RDS)of the overall reaction on g-C_(3) N_(4) is the conversion of pyruvaldehyde,where an electron transfer takes place.This present work provides experimental insights and theoretical understanding for selective lactic acid production from biomass photoreforming. 展开更多
关键词 Lactic acid Glucose photoreforming Carbon nitride DFT Reaction mechanism
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